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arXiv:2208.00045 · Physical Review Applied

Complete Unitary Qutrit Control in Ultracold Atoms

Joseph Lindon, Arina Tashchilina, Logan Cooke, Lindsay J. LeBlanc

Published Mar 28, 2023• 31 citations
arXivHTMLPDF

Abstract

Physical quantum systems are commonly composed of more than two levels and offer the capacity to encode information in higher-dimensional spaces beyond the qubit, starting with the three-level qutrit. Here, we encode neutral-atom qutrits in an ensemble of ultracold ${}^{87}\mathrm{Rb}$ and demonstrate arbitrary single-qutrit SU(3) gates. We generate a full set of gates using only two resonant microwave tones, including synthesizing a gate that effects a direct coupling between the two disconnected levels in the three-level $\mathrm{\ensuremath{\Lambda}}$-scheme. Using two different gate sets, we implement and characterize the Walsh-Hadamard Fourier transform, and find similar final-state fidelity and purity from both approaches. This work establishes the ultracold neutral-atom qutrit as a promising platform for qutrit-based quantum information processing, extensions to $d$-dimensional qudits, and explorations in multilevel quantum state manipulations with nontrivial geometric phases.

DOI
10.1103/physrevapplied.19.034089

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Physical quantum systems are commonly composed of more than two levels and offer the capacity to encode information in higher-dimensional spaces beyond the qubit, starting with the three-level qutrit. Here, we encode neutral-atom qutrits in an ensemble of ultracold 87Rb{}^{87}\mathrm{Rb}87Rb and demonstrate arbitrary single-qutrit SU(3) gates. We generate a full set of gates using only two resonant microwave tones, including synthesizing a gate that effects a direct coupling between the two disconnected levels in the three-level \ensuremathΛ\mathrm{\ensuremath{\Lambda}}\ensuremathΛ-scheme. Using two different gate sets, we implement and characterize the Walsh-Hadamard Fourier transform, and find similar final-state fidelity and purity from both approaches. This work establishes the ultracold neutral-atom qutrit as a promising platform for qutrit-based quantum information processing, extensions to ddd-dimensional qudits, and explorations in multilevel quantum state manipulations with nontrivial geometric phases.
We present a theoretical framework for universal single-qutrit control in asymmetric-top molecules, advancing molecular quantum information processing. In this approach, the qutrit is encoded in three rotational eigenstates, with an auxiliary state providing independent phase control within the computational manifold. We explore an analytic protocol for arbitrary single-qutrit gates, combining directly addressable SU(2) rotations with auxiliary-state-mediated phase operations. To support this, we derive a multilevel pulse-area theorem that provides an explicit analytic mapping between gate parameters and control fields, enabling systematic design of high-fidelity microwave pulse sequences. Numerical simulations with 1,2-propanediol confirm the robustness of our approach, achieving Walsh-Hadamard gates with minimal leakage from the computational subspace. We further examine four SU(2) decomposition strategies and find that phase-error sensitivity depends on the decomposition sequence, while amplitude errors propagate along specific coherence pathways. Our results establish asymmetric-top molecules as a viable platform for qutrit-based quantum operations and offer an analytical method for precise quantum control of complex multilevel systems.
Quantum devices comprised of elementary components with more than two stable levels—so-called qudits—enrich the accessible Hilbert space, enabling applications ranging from fault-tolerant quantum computing to simulating complex many-body models. While several quantum platforms are built from local elements that are equipped with a rich spectrum of stable energy levels, schemes for the efficient control and entanglement of qudits are scarce. Importantly, no experimental demonstration of multiqudit control has been achieved to date in neutral atom arrays. Here, we propose a general scheme for controlling and entangling qudits and perform a full analysis for the case of qutrits, encoded in ground and metastable states of alkaline earth atoms. We find an efficient implementation of single-qudit gates via the simultaneous driving of multiple transition frequencies. For entangling operations, we provide a concrete and intuitive recipe for the controlled- Z ( C Z ) gate for any local dimension d , realized through alternating single qudit and entangling pulses that simultaneously drive up to two Rydberg transitions. We further prove that two simultaneous Rydberg tones are, in general, the minimum necessary for implementing the C Z gate with a global drive. The pulses we use are optimally controlled, smooth, and robust to realistic experimental imperfections, as we demonstrate using extensive noise simulations. This amounts to a minimal, resource-efficient, and practical protocol for realizing a universal set of gates. Our scheme for the native control of qudits in a neutral atom array provides a high-fidelity route toward qudit-based quantum computation, ready for implementation on near-term devices.
Although only two quantum states of a physical system are often used to encode quantum information in the form of qubits, many levels can in principle be used to obtain qudits and increase the information capacity of the system. To take advantage of the additional levels, a parameterization of unitary transformations in terms of experimentally realizable operations is needed. Many parameterizations of unitary 3 * 3 matrices (U(3)) exist. One decomposition of a general unitary matrix can be expressed as the product of an exponential of a diagonal matrix and an exponential of an off-diagonal matrix. This decomposition is relevant for controlling superconducting qutrits using fixed-frequency resonant control pulses. This decomposition is numerically confirmed to allow the parameterization of any element in U(3). It is shown that a simple setting of parameter ranges of parameters can easily lead to an over-parameterization, in the sense that several different sets of values for the parameters produce the same element in U(3). This fact is demonstrated using the Walsh-Hadamard (WH) matrix as an example, which is also a special qutrit gate of practical interest. The different decompositions are shown to be related, and the relationships between them are presented using general methods. The shortest path needed for the implementation of a qutrit gate is found. Other parameterizations obtained by other analytic means, which can be advantageous for various reasons, are also discussed.
We have implemented a Walsh-Hadamard gate, which performs a quantum Fourier transform, in a superconducting qutrit. The qutrit is encoded in the lowest three energy levels of a capacitively shunted flux device, operated at the optimal flux-symmetry point. We use an efficient decomposition of the Walsh-Hadamard gate into two unitaries, generated by off-diagonal and diagonal Hamiltonians, respectively. The gate implementation utilizes simultaneous driving of all three transitions between the three pairs of energy levels of the qutrit, one of which is implemented with a two-photon process. The gate has a duration of 35 ns and an average fidelity over a representative set of states, including preparation and tomography errors, of 99.2%, characterized with quantum-state tomography. Compensation of ac-Stark and Bloch-Siegert shifts is essential for reaching high gate fidelities.
Hybrid qubits have recently drawn intense attention in quantum computing. We here propose a method to implement a universal controlled-phase gate of two hybrid qubits via two three-dimensional (3D) microwave cavities coupled to a superconducting flux qutrit. For the gate considered here, the control qubit is a microwave photonic qubit (particle-like qubit), whose two logic states are encoded by the vacuum state and the single-photon state of a cavity, while the target qubit is a cat-state qubit (wave-like qubit), whose two logic states are encoded by the two orthogonal cat states of the other cavity. During the gate operation, the qutrit remains in the ground state; therefore, decoherence from the qutrit is greatly suppressed. The gate realization is quite simple, because only a single basic operation is employed and neither classical pulse nor measurement is used. Our numerical simulations demonstrate that with current circuit quantum electrodynamics technology, this gate can be realized with a high fidelity. The generality of this proposal allows implementing the proposed gate in a wide range of physical systems, such as two 1D or 3D microwave or optical cavities coupled to a natural or artificial three-level atom. Finally, this proposal can be applied to create a novel entangled state between a particle-like photonic qubit and a wave-like cat-state qubit.
Unitary transformations are the fundamental building blocks of gates and operations in quantum information processing, allowing the complete manipulation of quantum systems in a coherent manner. In the case of photons, optical elements that can perform unitary transformations are readily available only for some degrees of freedom, e.g., wave plates for polarization. However, for high-dimensional states encoded in the transverse spatial modes of light, performing arbitrary unitary transformations remains a challenging task for both theoretical proposals and actual implementations. Following the idea of multi-plane light conversion, we show that it is possible to perform a broad variety of unitary operations at high quality by using only a few phase modulation planes. More importantly, we experimentally implement several high-dimensional quantum gates for up to five-dimensional states encoded in the full-field mode structure of photons. In particular, we realize cyclic and quantum Fourier transformations, known as Pauli X ^ -gates and Hadamard H ^ -gates, respectively, with an average visibility of more than 90%. In addition, we demonstrate near-perfect “unitarity” by means of quantum process tomography, unveiling a process purity of 99%. Last, we demonstrate the benefit of the two independent spatial degrees of freedom, i.e., azimuthal and radial, and implement a two-qubit controlled-NOT quantum operation on a single photon. Thus, our demonstrations open up new paths to implement high-dimensional quantum operations, which can be applied to various tasks in quantum communication, computation, and sensing schemes.