A class of systems exists in which dissipation, external drive and interactions compete and give rise to non equilibrium phases that would not exist without the drive. There, phase transitions could occur without the breaking of any symmetry, yet with a local order parameter, in contrast with the Landau theory of phase transitions at equilibrium. One of the simplest driven dissipative quantum systems consists of two-level atoms enclosed in a volume smaller than the wavelength of the atomic transition cubed, driven by a light field. The competition between collective coupling of the atoms to the driving field and their cooperative decay should lead to a transition between a phase where all the atomic dipoles are phaselocked and a phase governed by superradiant spontaneous emission. Here, we realize this model using a pencil-shaped cloud of laser cooled atoms in free space, optically excited along its main axis, and observe the predicted phases. Our demonstration is promising in view of obtaining free-space superradiant lasers or to observe new types of time crystals.
A class of systems exists in which dissipation, external drive and interactions compete and give rise to non equilibrium phases that would not exist without the drive. There, phase transitions could occur without the breaking of any symmetry, yet with a local order parameter, in contrast with the Landau theory of phase transitions at equilibrium. One of the simplest driven dissipative quantum systems consists of two-level atoms enclosed in a volume smaller than the wavelength of the atomic transition cubed, driven by a light field. The competition between collective coupling of the atoms to the driving field and their cooperative decay should lead to a transition between a phase where all the atomic dipoles are phaselocked and a phase governed by superradiant spontaneous emission. Here, we realize this model using a pencil-shaped cloud of laser cooled atoms in free space, optically excited along its main axis, and observe the predicted phases. Our demonstration is promising in view of obtaining free-space superradiant lasers or to observe new types of time crystals.
We observe a non-equilibrium phase transition in a driven dissipative quantum system consisting of an pencil-shape cloud of up to N≈2000 laser-cooled atoms in free space, optically excited along its main axis. We find that our data are well reproduced by the Driven Dicke model, which assumes a sub-wavelength sample volume, by simply using an effective atom number. By measuring the excited state population of the atoms and the light emitted in the superradiant mode, we characterize the dynamics of the system and its steady-state properties. In particular, we observe the characteristic N2 scaling of the photon emission rate in the superradiant phase, thus demonstrating steady-state superradiance in free space. Finally, we observe a modification of the statistics of the superradiant light as we cross the phase transition.
Atomic ensembles strongly interacting with light constitute rich quantum-optical many-body systems, with the potential for observing cooperative effects and dissipative nonequilibrium phase transitions. We theoretically analyze the conditions under which a driven atomic ensemble in free space, characterized by strong dipole-dipole interactions and large spatial extent, can undergo a superradiant phase transition, also known as cooperative resonance fluorescence. In an atomic array, stationary states that conserve the collective pseudospin exhibit completely cooperative decay and undergo a second-order phase transition in the large atom number limit. In contrast, decay mechanisms on longer timescales that fail to conserve pseudospin can lead to discontinuous first-order phase transition at a critical finite atom number, disrupting cooperation despite sharing many similar observable characteristics. A hallmark of the superradiant phase transition is an abrupt shift from total light reflection off the atoms to rapidly increasing transmission, accompanied by significant quantum fluctuations, as a function of light intensity.
Driven-dissipative many-body systems are ubiquitous in nature and a fundamental resource for quantum technologies. However, they are also complex and hard to model because they cannot be described by the standard tools in equilibrium statistical mechanics. Probing nonequilibrium critical phenomena in pristine setups can illuminate fresh perspectives on these systems. Here, we use an ensemble of cold 88 Sr atoms coupled to a driven high-finesse cavity to study the cooperative resonance fluorescence (CRF) model, a classic driven-dissipative model describing coherently driven dipoles superradiantly emitting light. We observe its nonequilibrium phase diagram characterized by a second-order phase transition. Below a critical drive strength, the atoms quickly reach the so-called superradiant steady state featuring a macroscopic dipole moment; above the critical point, the atoms undergo persistent Rabi-like oscillations. At longer times, spontaneous emission transforms the second-order transition into a discontinuous first-order transition. Our observations pave the way for harnessing robust entangled states and exploring boundary time crystals in driven-dissipative systems.
Ultracold atomic systems are among the most promising platforms that have the potential to shed light on the complex behavior of many-body quantum systems. One prominent example is the case of a dense ensemble illuminated by a strong coherent drive while interacting via dipole-dipole interactions. Despite being subjected to intense investigations, this system retains many open questions. A recent experiment carried out in a pencil-shaped geometry [Ferioli Nat. Phys. 19, 1345 (2023)] has reported measurements that have seemed consistent with the emergence of strong collective effects in the form of a “superradiant” phase transition in free space, when looking at the light-emission properties in the forward direction. Motivated by the experimental observations, we carry out a systematic theoretical analysis of the steady-state properties of the system as a function of the driving strength and atom number N . We observe signatures of collective effects in the weak-driving regime, which disappear with increasing drive strength as the system evolves into a single-particle-like mixed state comprised of randomly aligned dipoles. Although the steady state features some similarities to the reported superradiant-to-normal nonequilibrium transition, also known as cooperative resonance fluorescence, we observe significant qualitative and quantitative differences, including a different scaling of the critical drive parameter (from N to N ). We validate the applicability of a mean-field treatment to capture the steady-state dynamics under currently accessible conditions. Furthermore, we develop a simple theoretical model that explains the scaling properties by accounting for interaction-induced inhomogeneous effects and spontaneous emission, which are intrinsic features of interacting disordered arrays in free space. Published by the American Physical Society 2024
The driven Dicke model, wherein an ensemble of atoms is driven by an external field and undergoes collective spontaneous emission due to coupling to a leaky cavity mode, is a paradigmatic example of a system exhibiting a driven-dissipative phase transition as a function of driving strength. Recently, a similar phenomenon was experimentally observed, not in a cavity setting, but rather in a free-space atomic ensemble. The reason why similar behavior should emerge in free space is not obvious, as the system interacts with a continuum of optical modes, which encodes light-propagation effects. Here, we present and solve a simple model to explain the behavior of the free-space system, based on the one-dimensional Maxwell-Bloch equations. On one hand, we show that a free-space ensemble at a low optical depth can exhibit similar behavior as the cavity system, as spatial propagation effects are negligible. On the other hand, in the thermodynamic limit of large atom number, we show that certain observables such as the transmittance or the atomic excited population exhibit nonanalytic behavior as a function of the driving intensity, reminiscent of a phase transition. However, a closer analysis reveals that the atomic properties are highly inhomogeneous in space, and based on this we argue that the free-space system does not undergo a phase transition but rather a “phase separation,” roughly speaking, between saturated and unsaturated regions.
Atoms strongly interacting with light constitute rich quantum-optical systems with the potential for observing cooperative effects and dissipative nonequilibrium phase transitions. We analyze the conditions under which a driven atomic array, characterized by strong dipole–dipole interactions and a large spatial extent, can undergo a superradiant phase transition, also known as cooperative resonance fluorescence. We find that the array can exhibit completely cooperative decay that conserves the collective pseudospin, resulting in a second-order quantum phase transition, with a key hallmark being an abrupt shift from total light reflection by the atoms to rapidly increasing transmission and significant quantum fluctuations. We compare the results with decay mechanisms that fail to conserve pseudospin, leading to a discontinuous first-order phase transition at a critical finite atom number.