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arXiv:2207.05512 · Physical Review Letters

Observation of a Superradiant Phase Transition with Emergent Cat States

Ri‐Hua Zheng, Wen Ning, Ye‐Hong Chen, Jiahao Lu, Li-Tuo Shen, Kai Xu, Yu-Ran Zhang, Da Xu, Hekang Li, Yan Xia, Fan Wu, Zhen‐Biao Yang, Adam Miranowicz, Neill Lambert, Dongning Zheng, Heng Fan, Franco Nori, Shi‐Biao Zheng

Published Sep 11, 2023• 58 citations
arXivHTMLPDF

Abstract

Superradiant phase transitions (SPTs) are important for understanding light-matter interactions at the quantum level, and play a central role in criticality-enhanced quantum sensing. So far, SPTs have been observed in driven-dissipative systems, but the emergent light fields did not show any nonclassical characteristic due to the presence of strong dissipation. Here we report an experimental demonstration of the SPT featuring the emergence of a highly nonclassical photonic field, realized with a resonator coupled to a superconducting qubit, implementing the quantum Rabi model. We fully characterize the light-matter state by Wigner matrix tomography. The measured matrix elements exhibit quantum interference intrinsic of a photonic mesoscopic superposition, and reveal light-matter entanglement.

DOI
10.1103/physrevlett.131.113601

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Superradiant phase transitions (SPTs) are important for understanding light-matter interactions at the quantum level, and play a central role in criticality-enhanced quantum sensing. So far, SPTs have been observed in driven-dissipative systems, but the emergent light fields did not show any nonclassical characteristic due to the presence of strong dissipation. Here we report an experimental demonstration of the SPT featuring the emergence of a highly nonclassical photonic field, realized with a resonator coupled to a superconducting qubit, implementing the quantum Rabi model. We fully characterize the light-matter state by Wigner matrix tomography. The measured matrix elements exhibit quantum interference intrinsic of a photonic mesoscopic superposition, and reveal light-matter entanglement.
The ground state of the quantum Rabi model (QRM) exhibits rich nonclassical states including the squeezed state, cat state, and entangled state in different parameter regimes. In this paper, we first use the polaron picture with high precision and fidelity to figure out the process of the superradiant phase transition (SPT) in view of the nonclassical states. The squeezing effect is considered to be a result of the higher-order excitations and important in order to understand the fundamental quantum physics of the SPT in the QRM. According to the polaron wave functions, the squeezed state extends across the entire range of parameters. Based on the squeezing and superradiance, a classification of the coupling strength for the nonclassical states containing the ground state is presented; the system sequentially goes through the vacuum states, the squeezed vacuum states, the squeezed cat states, and the cat states as the coupling strength increases. The process of the SPT is also demonstrated by the photon number distribution in Fock space, and then the novel behavior of parity chains for the SPT is revealed. Additionally, the nonclassical states can be intuitively characterized by the Wigner functions with analytical expressions in the polaron picture, and the Wigner negativity is evaluated to measure the nonclassicality. We find that a small but nonzero weighted antipolaron is necessary to form novel semicat states. Our paper provides guidance for preparing nonclassical states in experiments based on the light-matter interaction.
The ground state of quantum Rabi model (QRM) exhibits rich nonclassical states including squeezed state, cat state, and entangled state in different parameter regimes. In this paper, we firstly use the polaron picture to figure out the process of superradiant phase transition (SPT) in view of the nonclassical states. According to the polaron wave functions, the squeezed state extends to whole parameter regimes, and a small but non-zero weighted antipolaron is necessary to form novel semi-cat states. Moreover, the behavior of superradiance in the QRM can be viewed as the same displacement of the cat states from zero to a finite value, while the ground state becomes entangled state resulting from the emergence of spin-up state. On the other hand, the nonclassical states can be intuitively characterized by the Wigner functions with analytical expressions in the polaron picture, and the Wigner negativity is also evaluated to measure the nonclassicality. Based on the squeezing and superradiance, a classification of the coupling strength for the nonclassical states containing in the ground state is presented, and the process of the SPT is also revealed by the photon number distribution in Fock space, which is important to understand the fundamental quantum physics in the QRM. Our work provides a guidance for preparing the nonclassical states in experiments based on the QRM.
We theoretically study the superradiant phase transition (SPT) in an indirect Rabi model, where both a two-level system and a single-mode bosonic field couple to an auxiliary bosonic field. We find that the indirect spin-field coupling induced by the virtual excitation of the auxiliary field can allow the occurrence of a SPT at a critical point, and the influence of the so-called A2{A}^{2}A2 term in the normal Rabi model is naturally avoided. In the large detuning regime, we present the analytical expression of quantum critical point in terms of the original system parameters. The critical atom-field coupling strength is tunable, which will loosen the conditions on realizing the SPT. Considering a hybrid magnon-cavity-qubit system, we predict the squeezed cat state of magnon generated with feasible experimental parameters, which has potential applications in quantum metrology and quantum information processing.
Recently, a superradiant phase transition first predicted theoretically in the quantum Rabi model (QRM) has been verified experimentally. This further stimulates the interest in the study of the process of phase transition and the nature of the superradiant phase since the fundamental role of the QRM in describing the interaction of light and matter, and more importantly, the QRM contains rich physics deserving further exploration despite its simplicity. Here we propose a scheme consisting of two successive diagonalizations to accurately obtain the ground-state and excited states wavefunctions of the QRM in full parameter regime ranging from weak to deep-strong couplings. Thus, one is able to see how the phase transition occurs and how the photons populate in Fock space of the superradiant phase. We characterize the photon populations by borrowing the distribution concept in random matrix theory and find that the photon population follows a Poissonian-like distribution once the phase transition takes place and further exhibits the statistics of Gaussian unitary ensemble with increasing coupling strength. More interestingly, the photons in the excited states behave even like the statistics of Gaussian orthogonal ensemble. Our results not only deepen understanding on the superradiant phase transition but also provide an insight on the nature of the superradiant phase of the QRM and related models.
The Dicke-Ising model, one of the few paradigmatic models of matter-light interaction, exhibits a superradiant quantum phase transition above a critical coupling strength. However, in natural optical systems, its experimental validation is hindered by a “no-go theorem.” Here, we propose a digital-analog quantum simulator for this model based on an ensemble of interacting qubits coupled to a single-mode photonic resonator. We analyze the system's free-energy landscape using field-theoretical methods and develop a digital-analog quantum algorithm that disentangles qubit and photon degrees of freedom through a parity-measurement protocol. This disentangling enables the emulation of a photonic Schrödinger cat state, which is a hallmark of the superradiant ground state in finite-size systems and can be unambiguously probed through the Wigner tomography of the resonator's field.
The simple resonant Rabi oscillation of a two-level system in a single-mode coherent field reveals complex features at the mesoscopic scale, with oscillation collapses and revivals. Using slow circular Rydberg atoms interacting with a superconducting microwave cavity, we explore this phenomenon in an unprecedented range of interaction times and photon numbers. We demonstrate the efficient production of cat states, which are the quantum superposition of coherent components with nearly opposite phases and sizes in the range of few tens of photons. We measure cuts of their Wigner functions revealing their quantum coherence and observe their fast decoherence. This experiment opens promising perspectives for the rapid generation and manipulation of nonclassical states in cavity and circuit quantum electrodynamics.