Exploring non-Hermitian phenomenology is an exciting frontier of modern physics.However, the demonstration of a non-Hermitian phenomenon that is quantum in nature has remained elusive.Here, we predict quantum non-Hermitian phenomena: the fractional quantum Zeno (FQZ) effect and FQZ-induced photon antibunching.We consider a quantum optics platform with reservoir engineering, where nonlinear emitters are coupled to a bath of decaying bosonic modes whose own decay rates form band structures.By engineering the dissipation band, the spontaneous emission of emitters can be suppressed by strong dissipation through an algebraic scaling with fractional exponents-the FQZ effect.This fractional scaling originates uniquely from the divergent dissipative density of states near the dissipation band edge, different from the traditional closed-bath context.We find FQZ-induced strong photon antibunching in the steady state of a driven emitter even for weak nonlinearities.Remarkably, we identify that the sub-Poissonian quantum statistics of photons, which has no classical analogs, stems here from the key role of non-Hermiticity.Our setup is experimentally feasible with the techniques used to design lattice models with dissipative couplings.
Exploring non-Hermitian phenomenology is an exciting frontier of modern physics.However, the demonstration of a non-Hermitian phenomenon that is quantum in nature has remained elusive.Here, we predict quantum non-Hermitian phenomena: the fractional quantum Zeno (FQZ) effect and FQZ-induced photon antibunching.We consider a quantum optics platform with reservoir engineering, where nonlinear emitters are coupled to a bath of decaying bosonic modes whose own decay rates form band structures.By engineering the dissipation band, the spontaneous emission of emitters can be suppressed by strong dissipation through an algebraic scaling with fractional exponents-the FQZ effect.This fractional scaling originates uniquely from the divergent dissipative density of states near the dissipation band edge, different from the traditional closed-bath context.We find FQZ-induced strong photon antibunching in the steady state of a driven emitter even for weak nonlinearities.Remarkably, we identify that the sub-Poissonian quantum statistics of photons, which has no classical analogs, stems here from the key role of non-Hermiticity.Our setup is experimentally feasible with the techniques used to design lattice models with dissipative couplings.
Collective quantum phenomena are fascinating, as they repeatedly challenge our comprehension of nature and its underlying mechanisms. The qualification ``quantum'' can be attributed to a generic many-body system whenever the interference effects related to the underlying wave nature of its elementary constituents can not be neglected anymore, and a naive classical description in terms of interacting billiard balls fails to catch its most essential features. This interference phenomenon called ``quantum degeneracy'' which occurs at weak temperatures, leads to spectacular collective behaviours such as the celebrated Bose-Einstein Condensation (BEC) phase transition, where a macroscopic fraction of a bosonic system of particles collapses below a critical temperature T_c on a single-particle state. Quantum coherence, when combined with inter-particle interactions, gives rise to highly non-classical frictionless hydrodynamic behaviours such as superfluidity (SF) and superconductivity (SC). \nEven more exotic quantum phases emerge in presence of important interactions as matter reaches a ``strongly correlated regime'' dominated by quantum fluctuations, where each particle is able to affect significantly the surrounding fluid: characteristic examples are the so-called Mott-Insulator (MI) quantum phase where particles are localized on a lattice due to a strong interaction-induced blockade, along with the Tonks-Girardeau (TG) gas where impenetrable bosons in one-dimension acquire effective fermionic statistics up to a unitary transformation, and the Fractional Quantum Hall (FQH) effect which occurs in presence of a gauge field, and features a special type of elementary excitation possessing a fractional charge and obeying to fractional statistics called `anyon'. \nThese quantum many-body effects were explored in a first place in systems well isolated from the external environment such as ultra-cold atomic gases or electrons in solid-state systems, within a physical context well described by ``equilibrium statistical mechanics''. Yet, over the last two decades a broad community has started investigating the possibility of stabilizing interacting quantum phases in novel nonlinear quantum optics architectures, where interacting photons have replaced their atomic and electronic counterpart. Thanks to their high level of controllability and flexibility, and the possibility of reaching the quantum degeneracy regime at exceptionally high temperatures, these platforms appear as extremely promising candidates for the ``quantum simulation'' of the most exotic many-body quantum problems: while the precursors experiments in semiconductor exciton-polariton already allow to reach the Bose-Einstein Condensation and superfluid regimes, novel platforms such as superconducting circuits, coupled cavity arrays or photons coupled to Rydberg EIT (Electromagnetically induced Transparency) atoms have entered the so-called `photon blockade' where photons behave as impenetrable particles, and open a encouraging pathway toward the future generation of strongly correlated phases with light. \nA specificity of quantum optics devices is their intrinsic ``non-equilibrium'' nature: the interplay between the practically unavoidable radiative and non-radiative losses and the external drive needed to replenish the photon gas leads the many-body system toward a steady-state presenting important non-thermal features. One one hand, an overwhelmingly large quantity of novel quantum phenomena is expected in the non-equilibrium framework, as breaking the thermal equilibrium condition releases severe constraints on the state of a quantum system and on the nature of its surrounding environment. On the other hand, we do not benefit yet of an understanding of non-equilibrium statistical mechanics comparable with its well-established equilibrium counterpart, which relies on strong historical foundations. Understanding how to tame (and possibly exploit) non-equilibrium effects in order to stabilize interesting quantum phases in a controlled manner often reveals a hard challenge. \nIn that prospect, an important conceptual issue in the non-equilibrium physics of strongly interacting photons regards the possibility of stabilizing ``incompressible quantum phases'' such as the Mott-Insulator or Fractional Quantum Hall states, and more generally to stabilize the ground-state of a given particle-number conserving Hamiltonian, in a physical context where dissipative losses can not be neglected. While being able to quantum simulate those emblematic strongly correlated quantum phases in this novel experimental context would strongly benefit to the quantum optics community, gaining such a kind of flexibility would also contribute to fill an important bridge between the equilibrium and the non-equilibrium statistical physics of open quantum systems, allowing to access in a controlled manner a whole new phenomenology at the interface between the two theories. \nIn this thesis I address those questions, which I reformulate in the following manner: \n \n-What are the conditions for the emergence of analogue equilibrium properties in open quantum systems in contact with a non-thermal environment ? \n \n-In particular, is it possible to stabilize strongly correlated quantum phases with a perfectly defined particle number in driven-dissipative photonic platforms, in spite of environment-induced losses and heating effects ? \n \nThe structure of the thesis is the following. \n \n \n[Chapter 1.] We give an overview of the physics of many-body photonic systems. As a first step we address the weakly interacting regime in the physical context of exciton-polaritons: after describing the microscopic aspects of typical experiments, we move to the discussion of non-equilibrium Bose-Einstein Condensation and the various mechanisms related to the emergence of thermal signatures at steady-state. The second part of this Chapter is dedicated to strongly interacting fluids. After drawing a quick overview of several experimental platforms presenting a good potential for the study of such physics in a near future, we discuss the relative performance of several schemes proposed in order to replenish the photonic population \n \n[Chapter 2.] We investigate the potential of a non-Markovian pump scheme with a narrow bandpass (Lorentzian shaped) emission spectrum for the generation of strongly correlated states of light in a Bose-Hubbard lattice. Our proposal can be implemented by mean of embedded inverted two-level emitters with a strong incoherent pumping toward the excited state. Our study confirms in a single cavity the possibility of stabilizing photonic Fock states in a single configuration, and strongly localized n=1 Mott-Insulator states in a lattice with n=1 density. We show that a relatively moderate hopping is responsible for a depletion of the Mott-state, which then moves toward a delocalized state reminiscent of the superfluid regime. Finally, we proceed to a mean-field analysis of the phase diagram, and unveil a Mott-to-Superfluid transition characterized by a spontaneous breaking of the U(1) symmetry and incommensurate density. The results of this Chapter are based on the following publications: \n- J. Lebreuilly, M. Wouters and I. Carusotto, ``Towards strongly correlated photons in arrays of dissipative nonlinear cavities under a frequency-dependent incoherent pumping'', C. R. Phys., 17(8), 836, 2016. \n- A. Biella, F. Storme, J. Lebreuilly, D. Rossini, R. Fazio, I. Carusotto and C. Ciuti, ``Phase diagram of incoherently driven strongly correlated photonic lattice'', Phys. Rev. A, 96, 023839, 2017. \n \n[Chapter 3.] In view of improving the performance of the scheme introduced in last chapter, and reproducing in particular the equilibrium zero temperature phenomenology in driven-dissipative photonic lattices, we develop a fully novel scheme based on the use of non-Markovian reservoirs with tailored broadband spectra which allows to mimick the effect of tunable chemical potential. Our proposal can be implemented by mean of a small number of emitters and absorbers and is accessible to current technologies. \n \nWe first analyse the case of a frequency-dependent emission with a square spectrum and confirm the possibility of stabilizing Mott insulator states with arbitrary integer density. Unlike the previous proposal the Mott state is robust against both losses and tunneling. A sharp transition toward a delocalized superfluid-like state can be induced by strong values of the tunneling or a change in the effective chemical potential. While an overall good agreement is found with the T=0 predictions, our analysis highlights small deviations from the equilibrium case in some parts of the parameters space, which are characterized by a non-vanishing entropy and the kinetic generation of doublon excitations. We finally consider an improved scheme involving additional frequency-dependent losses, and show in that case that the Hamiltonian ground-state is fully recovered for any choice of parameters. Our proposal, whose functionality relies on generic energy relaxation mechanisms and is not restricted to the Bose-Hubbard model, appears as a promising quantum simulator of zero temperature physics in photonic devices. The results of this Chapter are based on the following publication: \n- J. Lebreuilly, A. Biella, F. Storme, D. Rossini, R. Fazio, C. Ciuti and I. Carusotto, ``Stabilizing strongly correlated photon fluids with non-Markovian reservoirs'', Phys. Rev. A 96, 033828 (2017). \n \n[Chapter 4.] We adopt a broader perspective, and analyse the conditions for the emergence of analogous thermal properties in driven-dissipative quantum systems. We show that the impact of an equilibrated environment can be mimicked by several non-Markovian and non-equilibrated reservoirs. Chapter 2 already f
Photon-mediated interaction between quantum emitters in engineered photonic baths is an emerging area of quantum optics. At the same time, non-Hermitian (NH) physics is currently thriving, spurred by the exciting possibility to access new physics in systems ruled by non-trivial NH Hamiltonians—in particular, photonic lattices—which can challenge longstanding tenets such as the Bloch theory of bands. Here, we combine these two fields and study the exotic interaction between emitters mediated by the photonic modes of a lossy photonic lattice described by a NH Hamiltonian. We show in a paradigmatic case study that structured losses in the field can seed exotic emission properties. Photons can mediate dissipative, fully non-reciprocal interactions between emitters with range critically dependent on the loss rate. When this loss rate corresponds to a bare-lattice exceptional point, the effective couplings are exactly nearest neighbor, implementing a dissipative, fully non-reciprocal Hatano–Nelson model. Counterintuitively, this can occur irrespective of the lattice boundary conditions. Thus photons can mediate an effective emitter’s Hamiltonian which is translationally invariant despite the fact that the field is not. We interpret these effects in terms of metastable atom–photon dressed states, which can be exactly localized on only two lattice cells or extended across the entire lattice. These findings introduce a paradigm of light-mediated interactions with unprecedented features such as non-reciprocity, non-trivial dependence on field boundary conditions, and range tunability via a loss rate.
For decades, Hermiticity was considered an immutable axiom of quantum mechanics, essential for ensuring real energies and unitary evolution. This perspective has shifted radically, driven by the realization that non-Hermitian Hamiltonians provide a powerful effective description of open quantum systems, granting access to unique phenomena such as Exceptional Points and the Non-Hermitian Skin Effect. In this Perspective, we chart the trajectory of this field, moving from its established foundations in single-particle, linear models to the emerging frontier of interacting many-body systems. We first clarify the physical origins of non-Hermitian dynamics, distinguishing between mean-field approximations, conditional "no-click" evolution, and exact Liouvillian dynamics. We then focus on the rich phenomenology arising from the interplay of non-Hermiticity and interactions. We discuss interaction-induced topological phases, the generalization of skin effects to the many-body Hilbert space, and the distinct signatures of dissipative quantum chaos and complexity. Finally, we highlight collective phenomena in nonlinear regimes, including skin solitons and dissipative phase transitions. We also comment on measurement-induced entanglement transitions and their relation to non-Hermitian spectra and topology. By synthesizing these diverse developments, we provide a roadmap for the future of non-Hermitian physics.
Abstract We demonstrate the emergence of a topological ordered phase for non-Hermitian systems. Specifically, we elucidate that systems with non-Hermitian two-body interactions show a fractional quantum Hall (FQH) state. The non-Hermitian Hamiltonian is considered to be relevant to cold atoms with dissipation. We conclude the emergence of the non-Hermitian FQH state by the presence of the topological degeneracy and by the many-body Chern number for the ground state multiplet showing Ctot = 1. The robust topological degeneracy against non-Hermiticity arises from the manybody translational symmetry. Furthermore, we discover that the FQH state emerges without any repulsive interactions, which is attributed to a phenomenon reminiscent of the continuous quantum Zeno effect.
Quantum nonlinear optics seeks to harness strong photon-photon interactions for scalable quantum technologies, although dissipative losses still pose a major barrier to near-unity conversion efficiency. Here, we bridge non-Hermitian physics with the quantum nonlinear domain by exploiting perfect absorption to identify and optimize few-photon nonlinear processes. We theoretically investigate two circuit QED systems, operating in the light-matter ultrastrong coupling regime. The first (i) enables simultaneous two-atom excitations by single photons, while the second (ii) realizes the strong coupling between a single-photon and a two-photon Fock states. We demonstrate that, since the strong optical nonlinearities cause quantum spectral features to emerge already at the level of linear response theory, the perfect absorption condition in ∣S11∣ enables near-deterministic single-photon down-conversion into (i) a qubit-qubit-correlated pair and (ii) a two-photon pair. We show that the conversion efficiency can be systematically optimized through experimentally accessible parameters, both linked to the emergence of Hermitian subspaces within the effective non-Hermitian Hamiltonians. These findings position non-Hermitian engineering as a broadly applicable route to optimizing quantum devices at the single-photon level, even beyond circuit-QED platforms.
The Dicke model, which describes the collective interaction between an ensemble of atoms and a single-mode photon field, serves as a fundamental framework for studying light-matter interactions and quantum electrodynamic phenomena. In this work, we investigate the manifestation of non-Hermitian effects in a generalized Dicke model, where two dissipative atom ensembles interact with a single-mode photon field. By applying the Holstein-Primakoff transformation, we explore the system in the semiclassical limit as a non-Hermitian Dicke model, revealing rich exceptional points (EPs) and diabolic points in such a system. We find that, by introducing the nonlinear saturation gain into an atomic ensemble, higher-order EP can be induced, leading to intriguing properties. Furthermore, if the system is extended to a one-dimensional chain, then the band topology will interplay with the non-Hermitian effect. In the quantum regime, we explore the quantum signature of EPs, noting that the conditions for their emergence are influenced by discrete photon numbers. We further study the transition from photon anti-bunching to bunching at a steady state, driven by non-Hermitian dynamics. Our findings deepen the understanding of non-Hermitian physics in light-matter interaction which is instructive for the design of advanced photonic and quantum systems.