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arXiv:2206.08305 · Physical Review A

Collective quantum beats from distant multilevel emitters

Ahreum Lee, Hyok Sang Han, Fredrik K. Fatemi, S. L. Rolston, Kanu Sinha

Published Jan 3, 2023• 14 citations
arXivHTMLPDF

Abstract

We analyze the dynamics of quantum beats in a system of two V-type three-level atoms coupled to a waveguide. We show that quantum beats can be collectively enhanced or suppressed, akin to Dicke super- and subradiance, depending on the interatomic separation and the initial correlations between the atoms. In particular, the interference properties of the collective beats are determined by the distance between the atoms modulo the beat wavelength. We study the collective atomic and field dynamics, illustrating a crossover from a Markovian to a non-Markovian regime as the atomic separation becomes sufficiently large to bring memory effects of the electromagnetic environment into consideration. In such a non-Markovian regime, collective quantum beats can be enhanced beyond the Markovian limit as a result of retardation effects. Our results demonstrate the rich interplay between multilevel and multiatom quantum interference effects arising in a system of distant quantum emitters.

DOI
10.1103/physreva.107.013701

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We analyze the dynamics of quantum beats in a system of two V-type three-level atoms coupled to a waveguide. We show that quantum beats can be collectively enhanced or suppressed, akin to Dicke super- and subradiance, depending on the interatomic separation and the initial correlations between the atoms. In particular, the interference properties of the collective beats are determined by the distance between the atoms modulo the beat wavelength. We study the collective atomic and field dynamics, illustrating a crossover from a Markovian to a non-Markovian regime as the atomic separation becomes sufficiently large to bring memory effects of the electromagnetic environment into consideration. In such a non-Markovian regime, collective quantum beats can be enhanced beyond the Markovian limit as a result of retardation effects. Our results demonstrate the rich interplay between multilevel and multiatom quantum interference effects arising in a system of distant quantum emitters.
We study the collective radiative decay of a system of two two-level emitters coupled to a one-dimensional waveguide in a regime where their separation is comparable to the coherence length of a spontaneously emitted photon. The electromagnetic field propagating in the cavity-like geometry formed by the emitters exerts a retarded backaction on the system leading to strongly non-Markovian dynamics. The collective spontaneous emission rate of the emitters exhibits an enhancement or inhibition beyond the usual Dicke superradiance and subradiance due to self-consistent coherent time-delayed feedback.
Waveguides allow for direct coupling of emitters separated by large distances, offering a path to connect remote quantum systems. However, when facing the distances needed for practical applications, retardation effects due to the finite speed of light are often overlooked. Previous works studied the non-Markovian dynamics of emitters with retardation, but the properties of the radiated field remain mostly unexplored. By considering a toy model of two distant two-level atoms coupled through a waveguide, we study the spectrum of the radiated field that exhibits non-Markovian features such as linewidth broadening beyond standard superradiance, or narrow Fano-resonance-like peaks. We also observe modifications to the energy-exchange dynamics in the presence of retardation. We discuss a proof-of-concept implementation of our results in a superconducting circuit platform.
Abstract This work introduces a theoretical framework to model the collective dynamics of quantum emitters in highly non-Markovian environments, interacting through the exchange of photons with significant retardations. The formalism consists on a set of coupled delay differential equations for the emitter’s raising/lowering operators σ i ± , supplemented by input–output relations that describe the field mediating the interactions. These equations capture the dynamics of both linear (bosonic) and nonlinear (two-level) emitter arrays. It is exact in some limits—e.g. bosonic emitters or generic systems with up to one collective excitation—and can be integrated to provide accurate results for larger numbers of photons. These equations support a study of collective spontaneous emission of emitter arrays in open waveguide-QED environments. This study uncovers an effect we term cascaded super- and sub-radiance, characterized by light-cone-limited propagation and increasingly correlated photon emission across distant emitters. The collective nature of this dynamics for two-level systems is evident both in the enhancement of collective emission rates, as well as in a superradiant burst with a faster than linear growth. While these effects should be observable in existing circuit QED devices or slight generalizations thereof, the formalism put forward in this work can be extended to model other systems such as network of quantum emitters or the generation of correlated photon states.
Atoms coupled to the same environment interfere with each other to yield super- or sub-radiance. Specifically, atoms in subradiant states are promising candidates for long-lifetime qubits and quantum memory because of the immunity to the common environment. However, subradiant states can still be influenced by local environments, which are incoherent for different atoms and cannot be canceled out through interference. Here we propose to break this limit by preparing a waveguide QED system in the non-Markovian regime, where the ultra-small decay rate arises because of the retarded interaction. We further show that similar effect occurs spontaneously by self-interference and can be stressed by cooperative coupling.
We study the impact of destructive interference on the collective dynamics of two distant three-level V-type systems coupled to a waveguide in a strong-coupling regime in which the rotating-wave approximation (RWA) and Markovian approximation are inapplicable. By employing a polaronlike unitary transformation, we derive a transformed RWA Hamiltonian and combine it with the resolvent operator to study the non-Markovian dynamics and derive the condition under which the bound states exist due to the destructive interference, which can be realized by tuning the distance between the two V systems. We use a time-dependent variational approach with the multiple Davydov ansatz to numerically validate the analytical predictions and reveal the dynamical signature of bound states. We illustrate that the populations of symmetric and antisymmetric single-excitation states can be trapped in the long-time limit due to the bound states or possess a long lifetime due to subradiance. Moreover, the excitation probability can exhibit long-lived oscillation due to the coexistence of a bound state and a subradiant state. Our results offer insights into the destructive interference in distant multilevel emitters in a strong-coupling regime.
We analyze the dynamics of a set of two-level atoms coupled to the electromagnetic environment within a waveguide. This problem is often tackled by assuming a weak coupling between the atoms and the environment as well as the associated Markov approximation. We show that the accuracy of such an approximation may be more limited than in the single-atom case and may also be strongly determined by the presence of collective effects produced by atom-atom interactions. To this aim, we solve the full problem with exact diagonalization and also the time-dependent density matrix renormalization group method, and we compare the result to that obtained within a weak-coupling master equation and with the Dicke approximation. Finally, we study the dynamics of the entanglement within the system when considering several interatomic distances and atomic frequencies.