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arXiv:2206.05254 · Nature

Formation of robust bound states of interacting microwave photons

Alexis Morvan, Trond I. Andersen, Xiao Mi, Charles Neill, A. Petukhov, Kostyantyn Kechedzhi, Dmitry A. Abanin, Alexios A. Michailidis, Rajeev Acharya, Frank Arute, Kunal Arya, Abraham T. Asfaw, Juan Atalaya, Joseph C. Bardin, Joao Basso, Andreas Bengtsson, Gina Bortoli, Alexandre Bourassa, Jenna Bovaird, L. Brill, Michael Broughton, Bob B. Buckley, David A. Buell, Tim Burger, Brian Burkett, Nicholas Bushnell, Zidan Chen, B. Chiaro, Roberto Collins, P. Conner, William Courtney, Alexander L. Crook, Ben Curtin, Dripto M. Debroy, Alexander Del Toro Barba, Sean Demura, A. Dunsworth, Daniel Eppens, Catherine Erickson, Lara Faoro, Edward Farhi, Reza Fatemi, Leslie Flores Burgos, Ebrahim Forati, Austin G. Fowler, Brooks Foxen, William Giang, Craig Gidney, Dar Gilboa, Marissa Giustina, Alejandro Grajales Dau, Jonathan A. Gross, Steve Habegger, M. C. Hamilton, Matthew P. Harrigan, Sean David Harrington, M. R. Hoffmann, Sabrina Hong, Trent Huang, Ashley Huff, William J. Huggins, Sergei V. Isakov, Justin Iveland, Evan R. Jeffrey, Z. Jiang, Cody Jones, Pavol Juhás, Dvir Kafri, Tanuj Khattar, Mostafa Khezri, Mária Kieferová, Seon Kim, Alexei Kitaev, Paul V. Klimov, A. R. Klots, Alexander N. Korotkov, Fedor Kostritsa, John Mark Kreikebaum, David Landhuis, Pavel Laptev, K.-M. Lau, Lily Laws, J. Lee, Kenny Lee, Brian Lester, Alexander T. Lill, W. Liu, Aditya Locharla, Fionn D. Malone, Orion Martin, Jarrod R. McClean, Matt McEwen, B. Meurer Costa, Kevin C. Miao, Masoud Mohseni, Shirin Montazeri, Emily Mount, Wojciech Mruczkiewicz, Ofer Naaman, M. Neeley

Published Dec 7, 2022• 75 citations
arXivHTMLPDF

Abstract

Abstract Systems of correlated particles appear in many fields of modern science and represent some of the most intractable computational problems in nature. The computational challenge in these systems arises when interactions become comparable to other energy scales, which makes the state of each particle depend on all other particles1. The lack of general solutions for the three-body problem and acceptable theory for strongly correlated electrons shows that our understanding of correlated systems fades when the particle number or the interaction strength increases. One of the hallmarks of interacting systems is the formation of multiparticle bound states2–9. Here we develop a high-fidelity parameterizable fSim gate and implement the periodic quantum circuit of the spin-½ XXZ model in a ring of 24 superconducting qubits. We study the propagation of these excitations and observe their bound nature for up to five photons. We devise a phase-sensitive method for constructing the few-body spectrum of the bound states and extract their pseudo-charge by introducing a synthetic flux. By introducing interactions between the ring and additional qubits, we observe an unexpected resilience of the bound states to integrability breaking. This finding goes against the idea that bound states in non-integrable systems are unstable when their energies overlap with the continuum spectrum. Our work provides experimental evidence for bound states of interacting photons and discovers their stability beyond the integrability limit.

DOI
10.1038/s41586-022-05348-y

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Abstract Systems of correlated particles appear in many fields of modern science and represent some of the most intractable computational problems in nature. The computational challenge in these systems arises when interactions become comparable to other energy scales, which makes the state of each particle depend on all other particles1. The lack of general solutions for the three-body problem and acceptable theory for strongly correlated electrons shows that our understanding of correlated systems fades when the particle number or the interaction strength increases. One of the hallmarks of interacting systems is the formation of multiparticle bound states2–9. Here we develop a high-fidelity parameterizable fSim gate and implement the periodic quantum circuit of the spin-½ XXZ model in a ring of 24 superconducting qubits. We study the propagation of these excitations and observe their bound nature for up to five photons. We devise a phase-sensitive method for constructing the few-body spectrum of the bound states and extract their pseudo-charge by introducing a synthetic flux. By introducing interactions between the ring and additional qubits, we observe an unexpected resilience of the bound states to integrability breaking. This finding goes against the idea that bound states in non-integrable systems are unstable when their energies overlap with the continuum spectrum. Our work provides experimental evidence for bound states of interacting photons and discovers their stability beyond the integrability limit.
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Integrable models are characterized by the existence of stable excitations that can propagate indefinitely without decaying. This includes multimagnon bound states in the celebrated XXZ spin-chain model and its integrable Floquet counterpart. A recent Google Quantum AI experiment [A. Morvan , Nature , 240 (2022)] realizing the Floquet model has demonstrated the persistence of such collective excitations even when the integrability is broken: this observation is at odds with the expectation of ergodic dynamics in generic nonintegrable systems. Here, we study the spectrum of the model realized in the experiment using exact diagonalization and physical arguments. We find that isolated bands corresponding to the descendants of the exact bound states of the integrable model are clearly observable in the spectrum for a large range of system sizes. However, our numerical analysis of the localization properties of the eigenstates suggests that the bound states become unstable in the thermodynamic limit. A perturbative estimate of the decay rate agrees with the prediction of an eventual instability for large system sizes. Published by the American Physical Society 2024
Harnessing the interaction between light and matter at the quantum level has been a central theme in atomic physics and quantum optics, with applications from quantum computation to quantum metrology. Combining complex interactions with photonic synthetic materials provides an opportunity to investigate novel quantum phases and phenomena, establishing interesting connections to condensed matter physics. Here we explore many-body phenomena with a single artificial atom coupled to the many discrete modes of a photonic crystal. This experiment reaches the ultrastrong light-matter coupling regime using the circuit quantum electrodynamics paradigm, by galvanically coupling a highly nonlinear fluxonium qubit to a tight-binding lattice of microwave resonators. In this regime, the transport of a single photon becomes a many-body problem, owing to the strong participation of multi-photon bound states arising from interactions that break particle number conservation. Exploiting the effective photon-photon interactions mediated by the qubit, the transport of multiple photons leads to complex multimode dynamics that can be employed for generating a continuous reservoir of strongly-correlated photons, an important resource for quantum networks. This work opens exciting prospects for exploring nonlinear quantum optics at the single-photon level and stabilizing entangled many-body phases of light.
Quantum walks are the quantum analogs of classical random walks, which allow for the simulation of large-scale quantum many-body systems and the realization of universal quantum computation without time-dependent control. We experimentally demonstrate quantum walks of one and two strongly correlated microwave photons in a one-dimensional array of 12 superconducting qubits with short-range interactions. First, in one-photon quantum walks, we observed the propagation of the density and correlation of the quasiparticle excitation of the superconducting qubit and quantum entanglement between qubit pairs. Second, when implementing two-photon quantum walks by exciting two superconducting qubits, we observed the fermionization of strongly interacting photons from the measured time-dependent long-range anticorrelations, representing the antibunching of photons with attractive interactions. The demonstration of quantum walks on a quantum processor, using superconducting qubits as artificial atoms and tomographic readout, paves the way to quantum simulation of many-body phenomena and universal quantum computation.
Strong coupling between light and matter has been demonstrated both in classical cavity quantum electrodynamics (QED) systems and in more recent circuit-QED experiments. This enables the generation of strong nonlinear photon-photon interactions at the single-photon level, which is of great interest for the observation of quantum nonlinear optical phenomena, the control of light quanta in quantum information protocols such as quantum networking, as well as the study of strongly correlated quantum many-body systems using light. Recently, strong coupling has also been realized in a variety of one-dimensional (1D) waveguide- QED experimental systems, which in turn makes them promising candidates for quantum information processing. Compared to cavity-QED systems, there are two new features in waveguide-QED: the existence of a continuum of states and the restricted 1D phase space, which together bring in new physical effects, such as the bound-state effects. This thesis consists of two parts: 1) understanding the fundamental interaction between local quantum objects, such as two-level systems and four-level systems, and photons confined in the waveguide; 2) exploring its implications in quantum information processing, in particular photonic quantum computation and quantum key distribution. First, we demonstrate that by coupling a two-level system (TLS) or three/fourlevel system to a 1D continuum, strongly-correlated photons can be generated inside the waveguide. Photon-photon bound states, which decay exponentially as a function of the relative coordinates of photons, appear in multiphoton scattering processes. As a result, photon bunching and antibunching can be observed in the photon-photon correlation function, and nonclassical light source can be generated on demand. In the case of an N-type four-level system, we show that the effective photon-photon interaction mediated by the four-level system, gives rise to a variety of nonlinear optical phenomena, including photon blockade, photon-induced tunneling, and creation of single-photon states and photon pairs with a high degree of spectral entanglement, all in the absence of a cavity. However, to enable greater quantum networking potential using waveguide- QED, it is important to study systems having more than just one TLS/qubit. We develop a numerical Green function method to study cooperative effects in a system of two qubits coupled to a 1D waveguide. Quantum beats emerge in photon-photon correlations, and persist to much longer time scales because of non-Markovian processes. In addition, this system can be used to generate a high-degree of long-distance entanglement when one of the two qubits is driven by an on-resonance laser, further paving the way toward waveguide-QED-based quantum networks. Furthermore, based on our study of light-matter interactions in waveguide- QED, we investigate its implications in quantum information processing. First, we study quantum key distribution using the sub-Possonian single photon source obtained by scattering a coherent state off a two-level system. The rate for key generation is found to be twice as large as for other sources. Second, we propose a new scheme for scalable quantum computation using flying qubits--propagating photons in a one-dimensional waveguide--interacting with matter qubits. Photonphoton interactions are mediated by the coupling to a three- or four-level system, based on which photon-photon -phase gates (Controlled-NOT) can be implemented for universal quantum computation. We show that high gate fidelity is possible given recent dramatic experimental progress in superconducting circuits and photonic-crystal waveguides. The proposed system can be an important building block for future on-chip quantum networks.
Qubits strongly coupled to a photonic crystal give rise to qubit-photon dressed bound states.These bound states, comprising the qubits and spatially localized photonic modes induced around the qubits, are the basis for many exotic physical scenarios.The localization of these states changes with qubit detuning from the photonic crystal band edge, offering an avenue of in situ control of bound-state interaction.Here, we present experimental results from a device with two transmon qubits coupled to a superconducting microwave photonic crystal and realize tunable on-site and interbound state interactions.We observe a fourth-order two-photon virtual process between bound states indicating strong coupling between the photonic crystal and transmon qubits.Because of their localization-dependent interaction, these states offer the ability to realize one-dimensional chains of bound states with tunable and potentially long-range interactions that preserve the qubits' spatial organization.The widely tunable, strong, and robust interactions demonstrated with this system are promising benchmarks towards realizing larger, more complex systems that use bound states to build and study quantum spin models.