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arXiv:2206.01174

Dynamical Planckian scaling of charge response at a particle-hole-asymmetric quantum critical point with Kondo destruction

Ananth Kandala, Haoyu Hu, Qimiao Si A, Kevin Ingersent

Published Jun 2, 2022• 0 citations
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Abstract

Metallic quantum criticality is a central theme in a variety of strongly correlated systems. Recent experiments have raised the fundamental question of how the charge response can be singular in cases where the Landau framework of quantum criticality allows singularity only in the spin channel. Motivated by this emerging issue, we study the particle-hole-asymmetric regime of a Bose-Fermi Anderson model with power-law forms for both the bosonic bath spectrum and the fermionic band density of states. We realize a particle-hole-asymmetric quantum-critical state where quasiparticles are lost due to a critical destruction of Kondo screening, and demonstrate a dynamical Planckian scaling of the charge response. Implications for a new regime of heavy-fermion quantum criticality and for Mott-Hubbard systems are discussed.

DOI
10.48550/arxiv.2206.01174

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Metallic quantum criticality is a central theme in a variety of strongly correlated systems. Recent experiments have raised the fundamental question of how the charge response can be singular in cases where the Landau framework of quantum criticality allows singularity only in the spin channel. Motivated by this emerging issue, we study the particle-hole-asymmetric regime of a Bose-Fermi Anderson model with power-law forms for both the bosonic bath spectrum and the fermionic band density of states. We realize a particle-hole-asymmetric quantum-critical state where quasiparticles are lost due to a critical destruction of Kondo screening, and demonstrate a dynamical Planckian scaling of the charge response. Implications for a new regime of heavy-fermion quantum criticality and for Mott-Hubbard systems are discussed.
Quantum critical points often arise in metals perched at the border of an antiferromagnetic order. The recent observation of singular and dynamically scaling charge conductivity in an antiferromagnetic quantum critical heavy fermion metal implicates beyond-Landau quantum criticality. Here we study the charge and spin dynamics of a Kondo destruction quantum critical point (QCP), as realized in an SU(2)-symmetric Bose-Fermi Kondo model. We find that the critical exponents and scaling functions of the spin and single-particle responses of the QCP in the SU(2) case are essentially the same as those of the large-N limit, showing that 1/N corrections are subleading. Building on this insight, we demonstrate that the charge responses at the Kondo destruction QCP are singular and obey ω/T scaling. This property persists at the Kondo destruction QCP of the SU(2)-symmetric Kondo lattice model.
Quantum criticality that goes beyond the Landau framework of order-parameter fluctuations is playing a central role in elucidating the behavior of strange metals. A prominent case appears in Kondo lattice systems, which have been extensively analysed in terms of an effective Bose-Fermi Kondo model. Here, a spin is simultaneously coupled to conduction electron bands and gapless vector bosons that represent magnetic fluctuations. The Bose-Fermi Kondo model features interacting fixed points of Kondo destruction with such properties as dynamical Planckian (ℏω/kBT\hbar ω/ k_{\rm B} Tℏω/kB​T) scaling and loss of quasiparticles. Here we carry out a renormalization-group analysis of the model with spin isotropy and identify pair-wise annihilations of the fixed points as the spectrum of the bosonic bath evolves. Our analysis not only provides an essentially complete understanding of the previous numerical results of an SU(2)-symmetric model, but also reveals a surprising feature of sequential fixed-point annihilation. Our results lay the foundation for the understanding of quantum criticality in spin-isotropic heavy-fermion metals as well as in doped Mott-Hubbard systems.
We address the phenomenon of critical Kondo destruction in pseudogap Bose-Fermi Anderson and Kondo quantum impurity models. These models describe a localized level coupled both to a fermionic bath having a density of states that vanishes like ${|\ensuremath{\epsilon}|}^{r}$ at the Fermi energy ($\ensuremath{\epsilon}=0$) and, via one component of the impurity spin, to a bosonic bath having a sub-Ohmic spectral density proportional to ${|\ensuremath{\omega}|}^{s}$. Each bath is capable by itself of suppressing the Kondo effect at a continuous quantum phase transition. We study the interplay between these two mechanisms for Kondo destruction using continuous-time quantum Monte Carlo for the pseudogap Bose-Fermi Anderson model with 0<r<120<r<\frac{1}{2}0<r<21​ and $\frac{1}{2}\ensuremath{\le}s<1$, and applying the numerical renormalization group to the corresponding Kondo model. At particle-hole symmetry, the models exhibit a quantum-critical point between a Kondo (fermionic strong-coupling) phase and a localized (Kondo-destroyed) phase. The two solution methods, which are in good agreement in their domain of overlap, provide access to the many-body spectrum, as well as to correlation functions including, in particular, the single-particle Green's function and the static and dynamical local spin susceptibilities. The quantum-critical regime exhibits the hyperscaling of critical exponents and $\ensuremath{\omega}/T$ scaling in the dynamics that characterize an interacting critical point. The (r,s)(r,s)(r,s) plane can be divided into three regions: one each in which the calculated critical properties are dominated by the bosonic bath alone or by the fermionic bath alone, and between these two regions, a third in which the bosonic bath governs the critical spin response but both baths influence the renormalization-group flow near the quantum-critical point.
Quantum criticality in certain heavy-fermion metals is believed to go beyond the Landau framework of order-parameter fluctuations. In particular, there is considerable evidence for Kondo destruction: a disappearance of the static Kondo singlet amplitude that results in a sudden reconstruction of Fermi surface across the quantum critical point and an extra critical energy scale. This effect can be analyzed in terms of a dynamical interplay between the Kondo and RKKY interactions. In the Kondo-destroyed phase, a well-defined Kondo resonance is lost, but Kondo singlet correlations remain at nonzero frequencies. This dynamical effect allows for mass enhancement in the Kondo-destroyed phase. Here, we elucidate the dynamical Kondo effect in Bose-Fermi Kondo/Anderson models, which unambiguously exhibit Kondo-destruction quantum critical points. We show that a simple physical quantity---the expectation value ⟨Sf⋅sc⟩\langle {\bf S}_{f} \cdot {\bf s}_{c} \rangle⟨Sf​⋅sc​⟩ for the dot product of the local (fff) and conduction-electron (ccc) spins---varies continuously across such quantum critical points. A nonzero ⟨Sf⋅sc⟩\langle {\bf S}_{f} \cdot {\bf s}_{c} \rangle⟨Sf​⋅sc​⟩ manifests the dynamical Kondo effect that operates in the Kondo-destroyed phase. Implications are discussed for the stability of Kondo-destruction quantum criticality as well as the understanding of experimental results in quantum critical heavy-fermion metals.
Quantum dissipation induces a critical destruction of a Kondo screened state, which is of interest in the contexts of quantum critical heavy fermion metals and magnetic nanostructures. The sub-ohmic Bose-Fermi Kondo model provides a setting to study this effect. We find that this many-body problem is exactly solvable when the spectrum of the dissipative bosonic bath, J(ω), is singular, corresponding to J(τ)=const.. We determine the local spin correlation functions, showing that the singular LONGITUDINAL fluctuations of the bosonic bath dominate over the transverse ones. Our results provide evidence that the local quantum critical solution, derived within the extended dynamical mean field approach to the Kondo lattice model, has a zero residual entropy.
Strange metals appear in a wide range of correlated materials. Electronic localization-delocalization and the expected loss of quasiparticles characterize beyond-Landau metallic quantum critical points and the associated strange metals. Typical settings involve local spins. Systems that contain entwined degrees of freedom offer new platforms to realize unusual forms of quantum criticality. Here, we study the fate of an SU(4) spin-orbital Kondo state in a multipolar Bose-Fermi Kondo model, which provides an effective description of a multipolar Kondo lattice, using a renormalization-group method. We show that at zero temperature, a generic trajectory in the model's parameter space contains two quantum critical points, which are associated with the destruction of Kondo entanglement in the orbital and spin channels, respectively. Our asymptotically exact results reveal an overall phase diagram, provide the theoretical basis to understand puzzling recent experiments of a multipolar heavy fermion metal, and point to a means of designing different forms of quantum criticality and strange metallicity in a variety of strongly correlated systems.