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arXiv:2206.00490 · npj Quantum Information

Spectroscopic characterization of the quantum linear-zigzag transition in trapped ions

Jie Zhang, B. T. Chow, Sara Ejtemaee, P. C. Haljan

Published Jul 13, 2023• 8 citations
arXivHTMLPDF

Abstract

Abstract While engineered quantum systems are a general route to the manipulation of multipartite quantum states, access in a physical system to a continuous quantum phase transition under sufficient control offers the possibility of an intrinsic source of entangled states. To this end we realize the quantum version of the linear-zigzag structural transition for arrays of up to five ground state-cooled ions held in a linear Paul trap and we demonstrate several of the control requirements towards entangled-state interferometry near the critical point. Using in situ spectroscopy we probe the energy level structure and occupation of the soft mode associated with the structural transition, and show a stable critical point and majority ground state occupation crossing the transition. We resolve biases arising from trap electrode asymmetries that change the nature of the transition, show that they can be suppressed by varying the ion number, and demonstrate control of the transition bias using optical dipole forces.

DOI
10.1038/s41534-023-00741-5

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•Jan 1, 2021•138 citations
Abstract While engineered quantum systems are a general route to the manipulation of multipartite quantum states, access in a physical system to a continuous quantum phase transition under sufficient control offers the possibility of an intrinsic source of entangled states. To this end we realize the quantum version of the linear-zigzag structural transition for arrays of up to five ground state-cooled ions held in a linear Paul trap and we demonstrate several of the control requirements towards entangled-state interferometry near the critical point. Using in situ spectroscopy we probe the energy level structure and occupation of the soft mode associated with the structural transition, and show a stable critical point and majority ground state occupation crossing the transition. We resolve biases arising from trap electrode asymmetries that change the nature of the transition, show that they can be suppressed by varying the ion number, and demonstrate control of the transition bias using optical dipole forces.
Laser-cooled, trapped ions are a highly controlled experimental system that allows one to engineer novel quantum states of both fundamental and practical interest.For a string of ions in a linear radio frequency (RF) Paul trap, the linear-zigzag structural phase transition is an intriguing system to investigate quantum dynamics near the critical point of a prototype second-order phase transition, including the preparation of superposition states of different structural configurations.This thesis focuses on two technological improvements required for studying the linear-zigzag structural phase transition in the quantum regime.The first is the development of a compact and cost-effective RF synthesizer setup to provide multiple modulation sources for the laser manipulation of ion strings.The functionality and limitations of a prototype design, based on Direct Digital Synthesizer (DDS) development boards with a microcontroller interface, are evaluated and future improvements are identified.The second part of this thesis focuses on the stabilization of the secular trap frequencies in a linear Paul trap, which is necessary to obtain a stable critical point for the studies of the linear-zigzag transition.To this end, this thesis presents the implementation of a Ramsey spectroscopic technique to measure the secular frequencies and presents the preliminary results from the stability tests.
Laser-cooled ions held in a linear Paul trap with strong transverse confinement organize into a one-dimensional (1-D) linear crystal. If the transverse confinement is relaxed, the linear ion crystal undergoes a continuous, structural phase transition to a 2-D zigzag configuration. We study the dynamics near the critical point of the linear-zigzag transition. In the first part of this thesis, we study the spontaneous nucleation and dynamics of topological kink defects, formed as a result of a rapid quench across the linear-zigzag transition. The experimental results are compared to the Kibble-Zurek mechanism, which provides an intuitive model of defect formation and predicts a power-law scaling for the number of defectsformed as a function of transition quench rate. The second part of this thesis is focused on one of the key requirements for investigations of the near-transition dynamics in the quantum regime. To achieve an efficient ground state cooling of the zigzag vibrational mode, we demonstrate 3-D polarization-gradient cooling of strings of 1-4 trapped ions as an intermediate step between Doppler and sideband cooling, and study the polarization-gradient cooling rate and cooling limit as a function of the cooling beam intensity in and near the Lamb-Dicke regime. The results of this thesis pave the way towards our future experiments aimed at assessing the coherence time of a zigzag superposition state through measurements of tunneling oscillations.
An array of ions in a linear radio-frequency (RF) Paul trap is a good candidate for investigating structural phase transitions, such as the linear-to-zigzag (LZ) transition, due to the convenient control provided by modification of the trap confinement strength. In such studies, the trap secular frequencies are a key factor that limits the stability of the critical point (CP). In this paper, we implement secular-frequency stabilization, including active feedback stabilization of the RF voltage near the trap electrodes, and achieve a stability of better than 5~ppm over 200~s for both transverse and axial potentials. To evaluate the combined long-term stability of the trap potential in both directions, we measure the zigzag (ZZ) mode frequency near the CP, where the effect of instability in both trap directions is substantially amplified. The short-term noise within a limited spectral window is also suppressed by this scheme, as inferred from decoherence rates of the ZZ mode measured at different frequencies with Ramsey fringes. We also identify that the limitation of the secular frequency stability is mainly from the imperfect temperature insensitivity of voltage dividers and RF detectors, and as a result improvement of lab temperature stability is of great help for stabilizing the trap frequency.
A quasi-one-dimensional system of trapped, repulsively interacting atoms (e.g., an ion chain) exhibits a structural phase transition from a linear chain to a zigzag structure, tuned by reducing the transverse trap potential or increasing the particle density. Since it is a one-dimensional transition, it takes place at zero temperature and therefore quantum fluctuations dominate. In Fishman et al. [Phys. Rev. B 77, 064111 (2008)] it was shown that the system close to the linear-zigzag instability is described by a ${\ensuremath{\phi}}^{4}$ model. We propose a mapping of the ${\ensuremath{\phi}}^{4}$ field theory to the well-known Ising chain in a transverse field, which exhibits a quantum critical point. Based on this mapping, we estimate the quantum critical point in terms of the system parameters. This estimate gives the critical value of the transverse trap frequency for which the quantum phase transition occurs and which has a finite, measurable deviation from the critical point evaluated within the classical theory. A measurement is suggested for atomic systems which can probe the critical trap frequency at sufficiently low temperatures TTT. We focus in particular on a trapped-ion system and estimate the implied limitations on TTT and on the interparticle distance. We conclude that the experimental observation of the quantum critical behavior is, in principle, accessible.
A string of trapped ions at zero temperature exhibits a structural phase transition to a zigzag structure, tuned by reducing the transverse trap potential or the interparticle distance. The transition is driven by transverse, short wavelength vibrational modes. We argue that this is a quantum phase transition, which can be experimentally realized and probed. Indeed, by means of a mapping to the Ising model in a transverse field, we estimate the quantum critical point in terms of the system parameters, and find a finite, measurable deviation from the critical point predicted by the classical theory. A measurement procedure is suggested which can probe the effects of quantum fluctuations at criticality. These results can be extended to describe the transverse instability of ultracold polar molecules in a one-dimensional optical lattice.
Abstract Quantum phase transitions (QPTs) are usually associated with many-body systems in the thermodynamic limit when their ground states show abrupt changes at zero temperature with variation of a parameter in the Hamiltonian. Recently it has been realized that a QPT can also occur in a system composed of only a two-level atom and a single-mode bosonic field, described by the quantum Rabi model (QRM). Here we report an experimental demonstration of a QPT in the QRM using a 171Yb+ ion in a Paul trap. We measure the spin-up state population and the average phonon number of the ion as two order parameters and observe clear evidence of the phase transition via adiabatic tuning of the coupling between the ion and its spatial motion. An experimental probe of the phase transition in a fundamental quantum optics model without imposing the thermodynamic limit opens up a window for controlled study of QPTs and quantum critical phenomena.