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arXiv:2205.14621 · Physical Review Applied

Facilitation-Induced Transparency and Single-Photon Switch with Dual-Channel Rydberg Interactions

Yao Ding, Zhengyang Bai, Guoxiang Huang, Weibin Li

Published Jan 5, 2023• 4 citations
arXivHTMLPDF

Abstract

We investigate facilitation-induced transparency (FIT) enabled by strong and long-range Rydberg atom interactions between two spatially separated optical channels. In this setting, the resonant two-photon excitation of Rydberg states in a target channel is conditioned by a single Rydberg excitation in a control channel. Through the contactless coupling enabled by the Rydberg interaction, the optical transparency of the target channel can be actively manipulated by steering the optical detuning in the control channel. By adopting a dressed-state picture, we identify two different interference pathways, in which one corresponds to Rydberg blockade and an emergent one results from facilitation. We show that the FIT is originated from the Rydberg interaction and the quantum interference effect between the two pathways, which is different from conventional electromagnetically induced transparency realized by single-body laser-atom coupling. We find that the FIT in such a dual-channel setting is rather robust, insensitive to changes of systemic parameters, and can be generalized to multichannel settings. Moreover, we demonstrate that such a FIT permits the realization of controllable single-photon switches, which also paves a route to detect Rydberg facilitation by using optical absorption spectra. Our study contributes to current efforts in probing correlated many-body dynamics and developing single-photon quantum devices based on Rydberg atom ensembles.

DOI
10.1103/physrevapplied.19.014017

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We investigate facilitation-induced transparency (FIT) enabled by strong and long-range Rydberg atom interactions between two spatially separated optical channels. In this setting, the resonant two-photon excitation of Rydberg states in a target channel is conditioned by a single Rydberg excitation in a control channel. Through the contactless coupling enabled by the Rydberg interaction, the optical transparency of the target channel can be actively manipulated by steering the optical detuning in the control channel. By adopting a dressed-state picture, we identify two different interference pathways, in which one corresponds to Rydberg blockade and an emergent one results from facilitation. We show that the FIT is originated from the Rydberg interaction and the quantum interference effect between the two pathways, which is different from conventional electromagnetically induced transparency realized by single-body laser-atom coupling. We find that the FIT in such a dual-channel setting is rather robust, insensitive to changes of systemic parameters, and can be generalized to multichannel settings. Moreover, we demonstrate that such a FIT permits the realization of controllable single-photon switches, which also paves a route to detect Rydberg facilitation by using optical absorption spectra. Our study contributes to current efforts in probing correlated many-body dynamics and developing single-photon quantum devices based on Rydberg atom ensembles.
We discuss electromagnetically induced transparency in a cold ensemble of atoms optically excited to the Rydberg states. Strong dipole-dipole or van der Waals interactions between the atomic Rydberg states translate into large nonlocal nonlinearities for a propagating probe field. In the case of weak quantum fields, this can be used to attain a conditional phase shift of π between pairs of single photons realizing a deterministic photonic phase gate. For stronger fields, long-range interactions between the atoms constrain the medium to behave as a collection of superatoms, each comprising a blockade volume that can accommodate at most one Rydberg excitation. The propagation of a probe field is affected by its two-photon correlations within the blockade distance, which are strongly damped due to low saturation threshold of the superatoms. Our calculations reproduce and interpret the results of recent experiments.
Interacting Rydberg excitations in cold atomic ensembles can exhibit large quantum nonlinearities that enable engineering of strong interactions between individual photons. Consequently, Rydberg ensembles are a promising platform for quantum information applications and the study of more fundamental physics of few- and many-body phenomena with interacting photons. This thesis presents a series of experiments that study and exploit different regimes of Rydberg-mediated interactions. We report the realization of an efficient on-demand single-photon source. The strong long-range Rydberg interactions allow the excitation of only a single collective Rydberg state within the entire atomic medium. The collective excitation can be subsequently retrieved as a single-photon. We use this scheme to generate highly pure and highly indistinguishable photons, which are suitable for scalable quantum information applications. These photons can be compatible with other atomic systems due to their narrow bandwidth, which makes building practical hybrid quantum systems feasible. Here, we demonstrate high visibility two-photon quantum interference between our Rydberg-produced photons, and photons emitted by a remote single-trapped ion. We also study Rydberg atoms under electromagnetically induced transparency conditions, where coherent superpostions of photons and Rydberg excitations propagate through the atomic medium as lossless dark-state polaritons. In the experiment, we use the external control fields to tune the interactions to a many-body regime where we can observe resonant scattering of dark-state polaritons to lossy channels. We show that the enhanced scattering process arises as a pure three-body effect.
High optical nonlinearities can be achieved at the single photon level by coupling the photon states to strongly interacting Rydberg excitations under the conditions of electromagnetically induced transparency. The nonlinear response in Rydberg quantum optics comes as a direct result of the long range dipole-dipole interactions via Rydberg blockade and interaction induced dephasing. In this thesis, Rydberg quantum optics experiments are performed with two spatially separated mediums with a nonlinear response at the single photon level. Two ultracold rubidium atomic clouds are tightly confined by a pair of in-vacuo aspheric lenses such that only a few Rydberg excitations can exist in each one of the clouds simultaneously. The long range character of the dipole-dipole interactions leads to the generation of quantum states of light. The effective photon-photon interactions are directly observed as an anti-correlation in the simultaneous photon retrieval as a result of the non resonant van der Waals interactions. The collective Rydberg excitations, stored in the non-overlapping mediums, experience an additional spatial non-uniform phase. In addition, we experimentally characterize the cooperative optical response of a cold atomic medium at a single photon level. This aims to exploit the enhancement of the spontaneous emissions decay rate (superradiance) as a dependence of the number of atoms involved in the ensemble. The observed atomic response in two different regimes gives a further understanding of the system dynamics and unlocks a promising potential route towards the implementation in scalable, multichannel quantum optical devices.
We predict a resonant enhancement of the nonlinear optical response of an interacting Rydberg gas under conditions of electromagnetically induced transparency. The enhancement originates from a two-photon process which resonantly couples electronic states of a pair of atoms dressed by a strong control field. We calculate the optical response for the three-level system by explicitly including the dynamics of the intermediate state. We find an analytical expression for the third-order susceptibility for a weak classical probe field. The nonlinear absorption displays the strongest resonant behavior on two-photon resonance where the detuning of the probe field equals the Rabi frequency of the control field. The nonlinear dispersion of the medium exhibits various spatial shapes depending on the interaction strength. Based on the developed model, we propose a realistic experimental scenario to observe the resonance by performing transmission measurements.
We study electromagnetically induced transparency in a three-level ladder type configuration in ultracold atomic gases, where the upper level is an electronically highly excited Rydberg state. An effective distance dependent two-body dephasing can be induced in a regime where dipole-dipoles interaction couple nearly degenerate Rydberg pair states. We show that strong two-body dephasing can enhance the excitation blockade of neighboring Rydberg atoms. Due to the dissipative blockade, transmission of the probe light is reduced drastically by the two-body dephasing in the transparent window. The reduction of transmission is accompanied by a strong photon-photon anti-bunching. Around the Autler-Townes doublets, the photon bunching is amplified by the two-body dephasing, while transmission is largely unaffected. Besides relevant to the ongoing Rydberg atom studies, our study moreover provides a setting to explore and understand two-body dephasing dynamics in many-body systems.
Dynamic control of atomic dressing to the highly excited Rydberg state in multilevel systems has special appeals owing to the development of flexible and precise measurement. In this study we develop an experimentally accessible proposal to robustly control the dressing probability via a three-step cascaded excitation with double electromagnetically induced transparency (EIT) technique. The system can function as an optical switch where the third addressing laser serving as the control knob can switchably engineer the dressing probability with time. Differing from a conventional two-photon EIT, this scheme facilitates a maximal dressing probability determined by a relative strength between two strong coupling fields, entirely relaxing their absolute values. The collective feature caused by the interactions of a few atoms is also studied leading to an enhanced dressing probability as well as reduced response times. Our work offers the opportunity to a coherent dynamic control of Rydberg excitation and to realize sizable Rydberg-Rydberg interactions in weakly driven multilevel quantum systems.