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arXiv:2205.08832

Loss compensated and enhanced mid-infrared interaction-free sensing with undetected photons

Nathan R. Gemmell, Jefferson Flórez, Emma J. Pearce, Olaf Czerwinski, Chris C. Phillips, Rupert F. Oulton, Alex S. Clark

Published May 18, 2022• 1 citation
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Abstract

Sensing with undetected photons enables the measurement of absorption and phase shifts at wavelengths different from those detected. Here, we experimentally map the balance and loss parameter space in a non-degenerate nonlinear interferometer, showing the recovery of sensitivity despite internal losses at the detection wavelength. We further explore an interaction-free operation mode with a detector-to-sample incident optical power ratio of >200. This allows changes in attowatt levels of power at 3.4 $μ$m wavelength to be detected at 1550 nm, immune to the level of thermal black-body background. This reveals an ultra-sensitive infrared imaging methodology capable of probing samples effectively `in the dark'.

DOI
10.48550/arxiv.2205.08832

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Sensing with undetected photons enables the measurement of absorption and phase shifts at wavelengths different from those detected. Here, we experimentally map the balance and loss parameter space in a non-degenerate nonlinear interferometer, showing the recovery of sensitivity despite internal losses at the detection wavelength. We further explore an interaction-free operation mode with a detector-to-sample incident optical power ratio of >200. This allows changes in attowatt levels of power at 3.4 μμμm wavelength to be detected at 1550 nm, immune to the level of thermal black-body background. This reveals an ultra-sensitive infrared imaging methodology capable of probing samples effectively `in the dark'.
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Mid-infrared (mid-IR) light scatters much less than shorter wavelengths, allowing greatly enhanced penetration depths for optical imaging techniques such as optical coherence tomography (OCT). However, both detection and broadband sources in the mid-IR are technologically challenging. Interfering entangled photons in a nonlinear interferometer enables sensing with undetected photons, making mid-IR sources and detectors obsolete. Here we implement mid-IR frequency-domain OCT based on ultra-broadband entangled photon pairs spanning from 3.3 to 4.3 µm. We demonstrate 10 µm axial and 20 µm lateral resolution 2D and 3D imaging of strongly scattering ceramic and paint samples. By intrinsically being limited only by shot noise, we observe times more sensitivity per integration time and power of the probe light. Together with the vastly reduced footprint and technical complexity, our technique can outperform conventional approaches with classical mid-IR light sources.
Sensing with undetected photons has become a vibrant, application-driven research domain with a special focus on the mid-infrared (mid-IR) wavelength region. Since the mid-IR contains spectral bands with highly specific and strong molecular absorbance signatures, often referred to as fingerprints, a multitude of different samples and their compositions can be detected and quantified spectroscopically. Enhancing this spectroscopic method with imaging capabilities leads to a powerful technique for environmental monitoring and biomedical applications that enables automated diagnostics while omitting time-consuming and non-reversible labeling steps. To evade the shortcomings of state-of-the-art instruments for mid-IR hyperspectral microscopy—namely cost, complexity, power consumption, and performance, which stem from technological challenges in mid-IR detection and light sources—we construct a proof-of-concept nonlinear interferometer in a wide-field imaging arrangement. This nominally narrowband imaging technique is then expanded to acquire broadband spectral information through capturing images for varying interferometer displacement and applying a pixelwise Fourier-transform of the resulting interferograms, yielding high-resolution infrared spectra for each camera pixel. For the broadband range of 2300−3100cm −1 , covering the important CH-stretch band, we perform hyperspectral imaging that simultaneously resolves 3500 spatial modes, each with a spectral resolution of 10cm −1 , leveraging in total around 10 5 spatio-spectrally entangled photon modes. Our image acquisition uses a commercial sCMOS camera, while a medium-power and compact continuous-wave pump laser is the only necessary light source. For a moderate speed of 360 voxel/s, we obtain a predominantly shot-noise-influenced signal-to-noise ratio (SNR) of 50. We further demonstrate the practicality of our novel hyperspectral imaging technique for microplastics detection and bio-imaging tasks and outline engineering solutions to increase its speed by several orders of magnitude. This shows that our quantum imaging technique is highly promising for applications requiring compact, cost-effective label-free analyses.
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