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arXiv:2205.07738 · Physical Review Research

Optical magnetism and wavefront control by arrays of strontium atoms

Kyle E. Ballantine, David Wilkowski, Janne Ruostekoski

Published Sep 27, 2022• 12 citations
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Abstract

By analyzing the parameters of electronic transitions, we show how bosonic Sr atoms in planar optical lattices can be engineered to exhibit optical magnetism and other higher-order electromagnetic multipoles that can be harnessed for wavefront control of incident light. Resonant $\ensuremath{\lambda}\ensuremath{\simeq}2.6\phantom{\rule{4pt}{0ex}}\ensuremath{\mu}\mathrm{m}$ light for the $^{3}D_{1}\ensuremath{\rightarrow}{}^{3}{P}_{0}$ transition mediates cooperative interactions between the atoms while the atoms are trapped in a deeply subwavelength optical lattice. The atoms then exhibit collective excitation eigenmodes, e.g., with a strong cooperative magnetic response at optical frequencies, despite individual atoms having negligible coupling to the magnetic component of light. We provide a detailed scheme to utilize excitations of such cooperative modes consisting of arrays of electromagnetic multipoles to form an atomic Huygens' surface, with complete $2\ensuremath{\pi}$ phase control of transmitted light and almost no reflection, allowing nearly arbitrary wavefront shaping. In the numerical examples, this is achieved by controlling the atomic level shifts of Sr with off-resonant ${^{3}P}_{J}\ensuremath{\rightarrow}{^{3}D}_{1}$ transitions, which results in a simultaneous excitation of arrays of electric dipoles and electric quadrupoles or magnetic dipoles. We demonstrate the wavefront engineering for a Sr array by realizing the steering of an incident beam and generation of a baby-Skyrmion texture in the transmitted light via a topologically nontrivial transition of a Gaussian beam to a Poincar\'e beam, which contains all possible polarizations in a single cross-section.

DOI
10.1103/physrevresearch.4.033242

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Abstract Natural materials typically interact weakly with the magnetic component of light which greatly limits their applications. This has led to the development of artificial metamaterials and metasurfaces. However, natural atoms, where only electric dipole transitions are relevant at optical frequencies, can cooperatively respond to light to form collective excitations with strong magnetic, as well as electric, interactions together with corresponding electric and magnetic mirror reflection properties. By combining the electric and magnetic collective degrees of freedom, we show that ultrathin planar arrays of atoms can be utilized as atomic lenses to focus light to subwavelength spots at the diffraction limit, to steer light at different angles allowing for optical sorting, and as converters between different angular momentum states. The method is based on coherently superposing induced electric and magnetic dipoles to engineer a quantum nanophotonic Huygens’ surface of atoms, giving full 2π phase control over the transmission, with close to zero reflection.
We show how to achieve single-photon control via a synthesized optical magnetic response without metamaterials, using quantum-mechanical electric dipole transitions of naturally occurring atoms. We demonstrate how arrays of atoms can be designed to absorb, store, and emit single photons and realize a quantum atomic Huygens' surface that allows for extreme wavefront engineering. The response can be further controlled by the quantum state of an optical cavity, generating entanglement between the cavity and the array, and hence the cavity and transmitted light.
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We show that atoms in an optical lattice can respond cooperatively to resonant incident light and that such a response can be employed for precise control and manipulation of light on a subwavelength scale. Specific collective excitation modes of the system that result from strong light-mediated dipole-dipole interactions can be addressed by tailoring the spatial phase profile of the incident light. We demonstrate how the collective response can be used to produce optical excitations at well-isolated sites on the lattice.