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arXiv:2205.00685 · Physical Review A

Motion-selective coherent population trapping for subrecoil cooling of optically trapped atoms outside the Lamb-Dicke regime

Hyun Gyung Lee, Sooyoung Park, Meung Ho Seo, D. Cho

Published Aug 31, 2022• 5 citations
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Abstract

We propose a scheme that combines velocity-selective coherent population trapping (CPT) and Raman sideband cooling (RSC) for subrecoil cooling of optically trapped atoms outside the Lamb-Dicke regime. This scheme is based on an inverted $\mathsf{Y}$ configuration in an alkali-metal atom. It consists of a $\mathrm{\ensuremath{\Lambda}}$ formed by two Raman transitions between the ground hyperfine levels and the $D$ transition, allowing RSC along two paths and formation of a CPT dark state. Using the state-dependent difference in vibration frequency of the atom in a circularly polarized trap, we can tune the $\mathrm{\ensuremath{\Lambda}}$ to make only the motional ground state a CPT dark state. We call this scheme motion-selective coherent population trapping (MSCPT). We write the master equations for RSC and MSCPT and solve them numerically for a $^{87}\mathrm{Rb}$ atom in a one-dimensional optical lattice when the Lamb-Dicke parameter is 1. Although MSCPT reaches the steady state slowly compared with RSC, the former consistently produces colder atoms than the latter. The numerical results also show that subrecoil cooling by MSCPT outside the Lamb-Dicke regime is possible under a favorable, yet experimentally feasible, condition. We explain this performance quantitatively by calculating the relative darkness of each motional state. Finally, we discuss the application of the MSCPT scheme to an optically trapped diatomic polar molecule whose Stark shift and vibration frequency exhibit large variations depending on the rotational quantum number.

DOI
10.1103/physreva.106.023324

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We propose a scheme that combines velocity-selective coherent population trapping (CPT) and Raman sideband cooling (RSC) for subrecoil cooling of optically trapped atoms outside the Lamb-Dicke regime. This scheme is based on an inverted Y\mathsf{Y}Y configuration in an alkali-metal atom. It consists of a \ensuremathΛ\mathrm{\ensuremath{\Lambda}}\ensuremathΛ formed by two Raman transitions between the ground hyperfine levels and the DDD transition, allowing RSC along two paths and formation of a CPT dark state. Using the state-dependent difference in vibration frequency of the atom in a circularly polarized trap, we can tune the \ensuremathΛ\mathrm{\ensuremath{\Lambda}}\ensuremathΛ to make only the motional ground state a CPT dark state. We call this scheme motion-selective coherent population trapping (MSCPT). We write the master equations for RSC and MSCPT and solve them numerically for a 87Rb^{87}\mathrm{Rb}87Rb atom in a one-dimensional optical lattice when the Lamb-Dicke parameter is 1. Although MSCPT reaches the steady state slowly compared with RSC, the former consistently produces colder atoms than the latter. The numerical results also show that subrecoil cooling by MSCPT outside the Lamb-Dicke regime is possible under a favorable, yet experimentally feasible, condition. We explain this performance quantitatively by calculating the relative darkness of each motional state. Finally, we discuss the application of the MSCPT scheme to an optically trapped diatomic polar molecule whose Stark shift and vibration frequency exhibit large variations depending on the rotational quantum number.
We report our experiment on sideband cooling with two Raman transitions in a $\mathrm{\ensuremath{\Lambda}}$ configuration that allows selective coherent population trapping (CPT) of the low-lying motional states. The cooling method is applied to 87Rb^{87}\mathrm{Rb}87Rb atoms in a circularly polarized one-dimensional optical lattice. Owing to the vector polarizability, the vibration frequency of a trapped atom depends on its Zeeman quantum number and the CPT resonance for a pair of bound states in the $\mathrm{\ensuremath{\Lambda}}$ configuration depends on their vibrational quantum numbers. We call this scheme motion-selective coherent population trapping (MSCPT) and it is a trapped-atom analog of the velocity-selective CPT developed for free He atoms. We observe a pronounced dip in temperature near a detuning for the Raman beams to satisfy the CPT resonance condition for the motional ground state. Although the lowest temperature we obtain is ten times the recoil limit owing to the heat load from motion along an axis, which is left uncooled, and the large Lamb-Dicke parameter of 2.3 in our apparatus, the experiment demonstrates that MSCPT enhances the effectiveness of Raman sideband cooling and enlarges the range of its application. Discussions of design parameters optimized for MSCPT on 87Rb^{87}\mathrm{Rb}87Rb atoms and opportunities provided by diatomic polar molecules, whose Stark shift shows a strong dependence on the rotational quantum number, are included.
We form a 1D optical lattices for Cs atoms using light tuned a few thousand linewidths below the 6S1/2(F equals 4) yields 6P3/2(F' equals 5) transition at 852 nm. In this far-off- resonance lattice the time scale for damping of motional coherences and kinetic energy can be orders of magnitude longer than the vibrational oscillation period for atoms trapped in the lattice potential wells. Atoms are loaded directly into deeply bound states, by adiabatic transfer from a superimposed, near-resonance optical lattice. This yields a mean vibrational excitation n approximately equals 0.3, and localization (Delta) z approximately (lambda) /20 deep in the Lamb-Dicke regime. Light scattering subsequently heats the atoms, but the initial rate is only of order 10-3 vibrational quanta per oscillation period. Low vibrational excitation, localization in the Lamb-Dicke regime and low heating rates make these atoms good candidates for resolved- sideband Raman cooling, and for the generation and study of non-classical states of center-of-mass motion. We propose a scheme for resolved-sideband Raman cooling and quantum state preparation; the scheme employs Raman coupling between magnetic sublevels induced by the lattice light field itself.
We report our study on coherent population trapping (CPT) in a $\ensuremath{\Lambda}$ configuration coupled by magnetic dipole interactions. The $\ensuremath{\Lambda}$ configuration is formed by bichromatic radio-frequency fields coupling a pair of Zeeman sublevels in one hyperfine level of an alkali-metal atom to another sublevel in the other hyperfine level. The Zeeman sublevel at the apex is coupled to a state in the nPnPnP manifold via an optical transition on one of the spectroscopic DDD lines to induce optical pumping to a dark state. The configuration is closed without leakage to other Zeeman sublevels. We use lithium atoms in an optical trap for our experimental study. The system allows independent control of the main parameters characterizing CPT, which include the upper-state decay rate and the decoherence rate as well as the Rabi frequencies. By turning off the applied fields, the system is frozen so that its quantum state can be measured precisely. We studied the line shapes and dynamics of the CPT system, and measured the phase relation of the dark superposition state to find excellent agreement with theory. The possible application of the scheme as a method to cool optically trapped atoms below the recoil limit in a manner analogous to velocity-selective coherent population trapping is discussed.
We report Raman sideband cooling of a single sodium atom to its three-dimensional motional ground state in an optical tweezer. Despite a large Lamb-Dicke parameter, high initial temperature, and large differential light shifts between the excited state and the ground state, we achieve a ground-state population of 93.5(7)% after 53 ms of cooling. Our technique includes addressing high-order sidebands, where several motional quanta are removed by a single laser pulse, and fast modulation of the optical tweezer intensity. We demonstrate that Raman sideband cooling to the three-dimensional motional ground state is possible, even without tight confinement and low initial temperature.
Summary form only given. The preparation of quantum systems in pure states is a prerequisite for coherent control. In this context laser cooling of trapped particles to the ground state of the confining potential is a powerful tool for preparing e.g. ions for quantum logic. In particular sideband cooling has been demonstrated to be the most efficient technique, allowing to achieve more than 99% of occupation of the ground state of the trap. This cooling technique relies on two conditions: the Lamb-Dicke regime, and the strong confinement regime. This latter condition, which allows the spectral resolution of individual sidebands of the motion, is however a limitation on the cooling time. We propose a model for cooling single ions inside a trap as an alternative to sideband cooling. The scheme uses electromagnetically induced transparency (EIT) in a /spl Lambda/-level scheme, where one of the transitions is dressed by a strong laser field. For detuning of the dressing laser, the absorption spectrum for the transition shows EIT when the cooling (probe) laser has detuning. Then, by tuning the cooling laser on the dark resonance (or EIT), for a suitable set of parameters and in the Lamb-Dicke regime the atoms are cooled to the ground state by the sideband transitions which are resonantly excited. The scheme achieves efficient ground state cooling and fast cooling rates using a continuous driving, instead of a pulsed one as in Raman sideband cooling schemes. An example is illustrated, where the average vibrational number is plotted as a function of the cooling time, and the final probability of occupation is plotted as a function of the vibrational state. This method may also be applied to reduce phase errors in coherent manipulations of trapped ions for quantum logic.
We present the results of simulations of optical sideband cooling of atomic ions in a trap with a shallow potential well. In such traps, an ion cannot be Doppler cooled near to the Lamb-Dicke regime $\mathrm{[}{\ensuremath{\eta}}^{2}(2\ensuremath{\langle}n\ensuremath{\rangle}+1)\ensuremath{\ll}1]$. Outside the Lamb-Dicke regime, the sideband cooling dynamics are altered by the existence of various Fock states with weak coupling where the cooling becomes very slow. A 40Ca+^{40}\mathrm{Ca}^{+}40Ca+ ion trapped in our Penning trap realizes such a situation; hence single stage cooling is inefficient to prepare the ion in the motional ground state. For these systems, it is necessary to study the cooling dynamics in detail and we show that it is possible to implement an optimized cooling sequence to achieve efficient ground-state cooling. We also present the simulated cooling dynamics of two ions trapped in a Penning trap, where the presence of an additional motional mode requires a complicated cooling sequence in order to cool both axial modes to the ground state simultaneously. Additionally, we demonstrate the dissipative preparation of Fock states outside the Lamb-Dicke regime by sideband heating a single ion in a Penning trap.