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arXiv:2204.09609 · Physical Review A

Controlling atomic spin mixing via multiphoton transitions in a cavity

Ming Xue, Xiangliang Li, Wenhao Ye, Junjie Chen, Zhi-Fang Xu, Li You

Published Sep 19, 2022• 3 citations
arXivHTMLPDF

Abstract

We propose to control spin-mixing dynamics in a gas of spinor atoms, via the combination of two off-resonant Raman transition pathways, enabled by a common cavity mode and a bichromatic pump laser. The mixing rate, which is proportional to the synthesized spin-exchange interaction strength, and the effective atomic quadratic Zeeman shift (QZS), can both be tuned by changing the pump laser parameters. Quench and driving dynamics of the atomic collective spin are shown to be controllable on a faster timescale than in existing experiments based on inherent spin-exchange collision interactions. The results we present open a promising avenue for exploring spin-mixing physics of atomic ensembles accessible in current experiments.

DOI
10.1103/physreva.106.033708

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We propose a method for engineering spin dynamics in ensembles of integer-spin atoms confined within a high-finesse optical cavity. Our proposal uses cavity-assisted Raman transitions to engineer a Dicke model for integer-spin atoms, which, in a dispersive limit, reduces to effective atom-atom interactions within the ensemble. This scheme offers a promising and flexible new avenue for the exploration of a wide range of spinor many-body physics. As an example of this, we present results showing that this method can be used to generate spin-nematic squeezing in an ensemble of spin-1 atoms. With realistic parameters the scheme should enable substantial squeezing on time scales much shorter than current experiments with spin-1 Bose-Einstein condensates.
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We propose a method to prepare the spin singlet in an ensemble of integer-spin atoms confined within a high-finesse optical cavity. Using a cavity-assisted Raman transition to produce an effective Tavis-Cummings model, we show that a high-fidelity spin singlet can be produced probabilistically, although with low efficiency, heralded by the absence of photons escaping the cavity. In a different limit, a similar configuration of laser and cavity fields can be used to engineer a model that emulates spinor collisional dynamics. Borrowing from techniques used in spinor Bose-Einstein condensates, we show that adiabatic transformation of the system Hamiltonian (via a time-dependent, effective quadratic Zeeman shift) can be used to produce a low-fidelity spin singlet. Then, by following this method with the aforementioned heralding technique, we show that it is possible to prepare the singlet state with both high fidelity and good efficiency for a large ensemble.