Abstract Although photon Bose–Einstein condensates have already been used for studying many interesting effects, the precise role of the photon–photon interaction is not fully clarified up to now. In view of this, it is advantageous that these systems allow measuring both the intensity of the light leaking out of the cavity and its spectrum at the same time. Therefore, the photon–photon interaction strength can be determined once via analysing the condensate broadening and once via examining the interaction-induced modifications of the cavity modes. As the former method depends crucially on the concrete shape of the trapping potential and the spatial resolution of the used camera, interferometric methods promise more precise measurements. To this end, the present paper works out the impact of the photon–photon interaction upon the cavity modes. A quantum mechanical description of the photon–photon interaction, including the thermal cloud, builds the theoretical backbone of the method. An exact diagonalisation approach introduced here exposes how the effective photon–photon interaction modifies both the spectrum and the width of the photon gas. A comparison with a variational approach based on the Gross–Pitaevskii equation quantifies the contribution of the thermal cloud in the respective applications.
Abstract Although photon Bose–Einstein condensates have already been used for studying many interesting effects, the precise role of the photon–photon interaction is not fully clarified up to now. In view of this, it is advantageous that these systems allow measuring both the intensity of the light leaking out of the cavity and its spectrum at the same time. Therefore, the photon–photon interaction strength can be determined once via analysing the condensate broadening and once via examining the interaction-induced modifications of the cavity modes. As the former method depends crucially on the concrete shape of the trapping potential and the spatial resolution of the used camera, interferometric methods promise more precise measurements. To this end, the present paper works out the impact of the photon–photon interaction upon the cavity modes. A quantum mechanical description of the photon–photon interaction, including the thermal cloud, builds the theoretical backbone of the method. An exact diagonalisation approach introduced here exposes how the effective photon–photon interaction modifies both the spectrum and the width of the photon gas. A comparison with a variational approach based on the Gross–Pitaevskii equation quantifies the contribution of the thermal cloud in the respective applications.
Abstract Thermo-optic interaction significantly differs from the usual particle-particle interactions in physics, as it is retarded in time. A prominent platform for realising this kind of interaction are photon Bose–Einstein condensates, which are created in dye-filled microcavities. The dye solution continually absorbs and re-emits these photons, causing the photon gas to thermalize and to form a Bose–Einstein condensate. Because of a non-ideal quantum efficiency, these cycles heat the dye solution, creating a medium that provides an effective thermo-optic photon–photon interaction. So far, only a mean-field description of this process exists. This paper goes beyond by working out a quantum mechanical description of the effective thermo-optic photon–photon interaction. To this end, the self-consistent modelling of the temperature diffusion builds the backbone of the modelling. Furthermore, the manyfold experimental timescales allow for deriving an approximate Hamiltonian. The resulting quantum theory is applied in the perturbative regime to both a harmonic and a box potential for investigating its prospect for precise measurements of the effective photon–photon interaction strength.
Abstract Although for photon Bose–Einstein condensates the main mechanism of the observed photon–photon interaction has already been identified to be of a thermo-optic nature, its influence on the condensate dynamics is still unknown. Here a mean-field description of this effect is derived, which consists of an open-dissipative Schrödinger equation for the condensate wave function coupled to a diffusion equation for the temperature of the dye solution. With this system at hand, the lowest-lying collective modes of a harmonically trapped photon Bose–Einstein condensate are calculated analytically via a linear stability analysis. As a result, the collective frequencies and, thus, the strength of the effective photon–photon interaction turn out to strongly depend on the thermal diffusion in the cavity mirrors. In particular, a breakdown of the Kohn theorem is predicted, i.e. the frequency of the centre-of-mass oscillation is reduced due to the thermo-optic photon–photon interaction.
Abstract Since the advent of experiments with photon Bose–Einstein condensates (phBECs) in dye-filled microcavities in 2010, many investigations have focussed upon the emerging effective photon–photon interaction. Despite its smallness, it can be identified to stem from two physically distinct mechanisms. On the one hand, a Kerr nonlinearity of the dye medium yields a photon–photon contact interaction. On the other hand, a heating of the dye medium leads to an additional thermo-optic interaction, which is both delayed and non-local. The latter turns out to represent the leading contribution to the effective interaction for the current 2D experiments. Here we analyse theoretically how the effective photon–photon interaction increases when the system dimension is reduced from 2D to 1D. To this end, we consider an anisotropic harmonic trapping potential and determine via a variational approach how the properties of the phBEC in general, and both aforementioned interaction mechanisms in particular, change with increasing anisotropy. We find that the thermo-optic interaction strength increases at first linearly with the trap aspect ratio and later on saturates at a certain value of the trap aspect ratio. Furthermore, in the strong 1D limit the roles of both interactions get reversed as the thermo-optic interaction remains saturated and the contact Kerr interaction becomes the leading interaction mechanism. Finally, we discuss how the predicted effects can be measured experimentally.
We review recent experiments on the Bose-Einstein condensation of photons in a dye-filled optical microresonator. The most well-known example of a photon gas, photons in blackbody radiation, does not show Bose-Einstein condensation. Instead of massively populating the cavity ground mode, photons vanish in the cavity walls when they are cooled down. The situation is different in an ultrashort optical cavity imprinting a low-frequency cutoff on the photon energy spectrum that is well above the thermal energy. The latter allows for a thermalization process in which both temperature and photon number can be tuned independently of each other or, correspondingly, for a nonvanishing photon chemical potential. We here describe experiments demonstrating the fluorescence-induced thermalization and Bose-Einstein condensation of a two-dimensional photon gas in the dye microcavity. Moreover, recent measurements on the photon statistics of the condensate, showing Bose-Einstein condensation in the grand-canonical ensemble limit, will be reviewed. Introduction Quantum statistical effects become relevant when a gas of particles is cooled, or its density is increased, to the point where the associated de Broglie wavepackets spatially overlap. For particles with integer spin (bosons), the phenomenon of Bose-Einstein condensation (BEC) then leads to macroscopic occupation of a single quantum state at finite temperatures [1]. Bose-Einstein condensation in the gaseous case was first achieved in 1995 by laser and subsequent evaporative cooling of a dilute cloud of alkali atoms [2, 3, 4], as detailed in Chapter 3 of this volume. The condensate atoms can be described by a macroscopic singleparticle wavefunction, similar to the case of liquid helium [1]. Bose-Einstein condensation has also been observed for exciton-polaritons, which are hybrid states of matter and light [5, 6, 7] (see Chapter 4), magnons [8] (see Chapter 25), and other physical systems. Other than material particles, photons usually do not show Bose-Einstein condensation [9]. In blackbody radiation, the most common Bose gas, photons at low temperature disappear, instead of condensing to a macroscopically occupied ground-state mode. In this system, photons have a vanishing chemical potential, meaning that the number of photons is determined by the available thermal energy and cannot be tuned independently from temperature.
The experimental realization of a Bose-Einstein condensate of photons, first achieved in 2010 at Bonn University, allowed for new ways to probe the properties of condensates. For thermal light in free space the chemical potential is zero and condensation is not possible. By confining light to a microcavity, the transverse degrees of freedom behave as massive bosons which can have nonzero chemical potential. The gas of thermal photons can be brought to thermalize with a fluorescent dye though absorption and emission cycles. By pumping the dye molecules with a laser, the chemical potential can be increased and the photons will condense. \nWe have built a setup with which we can spatially and spectrally resolve the photon distribution in such a dye-filled microcavity. This allows us to study the shape and occupation of the low energy transverse modes of the cavity. We use this to investigate the thermalization process of the photon gas. A rate equation model is presented and qualitatively compared to experimental data. We find that the photon gas is not in thermal equilibrium.\nWe also investigate effective photon-photon interactions by measuring the spatial extent of the condensate. We find an effective interaction in the form of thermal lensing. As the thermal lensing depends on the interaction between the photon gas and the dye, we find that the model used for thermalization can also make good predictions about effective photon-photon interactions.
Bose-Einstein condensation (BEC) is the transition to a macroscopic occupation of the ground state of a system of bosonic particles. In 1995 the first experimental realization of BEC was achieved by condensing a dilute atomic gas [1,2]. It was long thought only massive particles could undergo BEC. However, in 2010 it was shown that photon BEC was achieved in an optical dye-filled microcavity [3]. In 2015, we became the second group to successfully repeat these experiments.\n\nBEC is a phase transition and thus it occurs at thermal equilibrium. To achieve a thermal photon gas the cavity is filled with a fluorescent dye solution. The dye molecules thermalize the photons by means of repeated absorption-emission cycles. We optically pump the cavity. With the pump we determine the number of photons absorbed by the dye, consequently defining a nonvanishing chemical potential. This ensures a conserved photon number. The photons are trapped by the harmonic potential induced by the concave cavity mirrors. Due to the cutoff energy determined by the cavity length, the trapped photons have a dispersion similar to that of a massive particle in a quantum harmonic oscillator. The cavity length is tuned such that the free spectral range is larger than the bandwidth of the dye. Therefore, only one longitudinal mode fits inside the cavity, making the photon gas effectively two-dimensional. We end up with a thermalized two-dimensional photon gas that has the eigenenergies of a quantum harmonic oscillator. The Bose-Einstein distribution function predicts a critical photon number. Pumping the thermal photon gas beyond this critical number will lead to photon BEC.\n\nWe measure the spectral- and spatial distributions of our two-dimensional photon gas. In both distributions we observe photon BEC. Results show the characteristics of a phase transition: the appearance of a sharp peak on top of the thermal cloud that coincides with a converging chemical potential to zero. Both the spectral- and spatial distribution are in agreement with the theoretical distribution of photons with an effective mass in a quantum harmonic oscillator. Expansion of the condensate has been measured. This could indicate nonlinear optical effects such as thermal lensing or repulsive photon-photon interactions.