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arXiv:2204.05293 · PRX Quantum

Enriching the Quantum Toolbox of Ultracold Molecules with Rydberg Atoms

Kenneth Wang, Conner P. Williams, Lewis R. B. Picard, Norman Y. Yao, Kang-Kuen Ni

Published Sep 16, 2022• 36 citations
arXivHTMLPDF

Abstract

A quantum information architecture consisting of a hybrid array of optically trapped molecules and Rydberg atoms is developed to realize both high-fidelity submicrosecond entangling gates and nondestructive molecule detection.
DOI
10.1103/prxquantum.3.030339

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We show that an array of polar molecules interacting with Rydberg atoms is a promising hybrid system for scalable quantum computation.Quantum information is stored in long-lived hyperfine or rotational states of molecules, which interact indirectly through resonant dipole-dipole interactions with Rydberg atoms.A two-qubit gate based on this interaction has a duration of 1 μs and an achievable fidelity of 99.9%.The gate has little sensitivity to the motional states of the particles-the molecules can be in thermal states, the atoms do not need to be trapped during Rydberg excitation, the gate does not heat the molecules, and heating of the atoms has a negligible effect.Within a large, static array, the gate can be applied to arbitrary pairs of molecules separated by tens of micrometres, making the scheme highly scalable.The molecule-atom interaction can also be used for rapid qubit initialization and efficient, nondestructive qubit readout, without driving any molecular transitions.Single-qubit gates are driven using microwave pulses alone, exploiting the strong electric dipole transitions between rotational states.Thus, all operations required for large-scale quantum computation can be done without moving the molecules or exciting them out of their ground electronic states.
We propose high-fidelity controlled-NOT (CNOT) gates in a hybrid system of polar molecules and Rydberg atoms based on the unconventional Rydberg pumping mechanism. By combining the rich internal structure of polar molecules with the strong dipole-dipole interactions of Rydberg atoms, we realize both two-to-one and one-to-two gate configurations. Numerical simulations show that the gate performance is robust against spontaneous emission from Rydberg states. The approach naturally extends to larger systems, as demonstrated by four-qubit implementations achieving three-to-one and one-to-three CNOT gates with fidelities exceeding 99\%. These results highlight hybrid molecule-Rydberg atom architectures as a promising platform for scalable quantum information processing.