Arrays of Rydberg atoms constitute a highly tunable, strongly interacting venue for the pursuit of exotic states of matter. We develop a strategy for accessing a family of fractionalized phases known as quantum spin liquids in two-dimensional Rydberg arrays. We specifically use effective field theory methods to study arrays assembled from Rydberg chains tuned to an Ising phase transition that famously hosts emergent fermions propagating within each chain. This highly entangled starting point allows us to naturally access spin liquids familiar from Kitaev's honeycomb model---albeit from an entirely different framework. In particular, we argue that finite-range repulsive Rydberg interactions, which frustrate nearby symmetry-breaking orders, can enable coherent propagation of emergent fermions between the chains in which they were born. Delocalization of emergent fermions across the full two-dimensional Rydberg array yields a gapless
Z2 spin liquid with a single massless Dirac cone. Here, the Rydberg occupation numbers exhibit universal power-law correlations that provide a straightforward experimental diagnostic of this phase. We further show that explicitly breaking symmetries perturbs the gapless spin liquid into gapped, topologically ordered descendants: Breaking lattice symmetries generates toric-code topological order, whereas introducing Floquet-mediated chirality generates non-Abelian Ising topological order. In the toric-code phase, we analytically construct microscopic incarnations of non-Abelian defects, which can be created and transported by dynamically controlling the atom positions in the array. Our work suggests that appropriately tuned Rydberg arrays provide a cold-atoms counterpart of solid-state ``Kitaev materials'' and, more generally, it spotlights a different angle for pursuing experimental platforms for Abelian and non-Abelian fractionalization.
Interactions among atoms can lead to emergent phenomena, one of the most fascinating being topological order. Topological phases are important in understanding high-temperature superconductors and fault-tolerant quantum computing. Quantum spin liquids, a key example of topologically ordered phases, exhibit unique properties such as long-range entanglement in the ground state and support of anyonic excitations, making them an exciting focus in the study of strongly correlated systems. This thesis explores the detection and learning of topological phases in quantum many-body systems, including quantum spin models, cuprate superconductors and ultracold atomic platform of Rydberg atom arrays. Guided by the experiments on Kitaev materials, we begin by using spinon mean-field theory of quantum spin liquids to explain the transition from a quantized thermal Hall effect to an unquantized values. Making closer connections to experiments in cuprates, we include additional interactions with phonons present in the system. We examine how spinon-phonon interactions, characterized by symmetry analysis, give rise to a chiral phonon Hall viscosity and can also contribute to the thermal Hall effect. In the second part, we turn to Rydberg atom arrays, which have recently been shown to realize a
Z2 quantum spin liquid phase—an elusive state in conventional solid-state materials. We study how Rydberg interactions and lattice geometries lead to the emergence of
Z2 gauge theories and distinct classes of topological quantum spin liquids. Finally, we study a variational tensor network tomography method for learning topological states from randomized measurements on Rydberg atom arrays. We demonstrate its efficiency in characterizing complex two-dimensional states that could be realized in future experiments.
Abstract Programmable quantum simulators based on neutral atom arrays today offer powerful platforms for studying strongly correlated phases of quantum matter. Here, we employ the projective symmetry group framework to describe the symmetry fractionalization patterns in a topologically ordered
Z2 Z 2 quantum spin liquid (QSL) synthesized in such a Rydberg array on the ruby lattice. By systematically comparing the static structure factors of all possible mean-field Ansätze against density-matrix renormalization group calculations, we identify a promising candidate for the precise
Z2 Z 2 QSL realized microscopically. We also present detailed analyses of the dynamical structure factors as a reference for future experiments and showcase how these spin correlations can differentiate between varied QSL Ansätze .
We investigate the nature of quantum phases arising in chiral interacting Hamiltonians recently realized in Rydberg atom arrays. We classify all possible fermionic chiral spin liquids with
U(1) global symmetry using parton construction on the honeycomb lattice. The resulting classification includes six distinct classes of gapped quantum spin liquids: the corresponding variational wavefunctions obtained from two of these classes accurately describe the Rydberg many-body ground state at
1/2 and
1/4 particle density. Complementing this analysis with tensor network simulations, we conclude that both particle filling sectors host a spin liquid with the same topological order of a $\ensuremath{\nu}\phantom{\rule{0.16em}{0ex}}=\phantom{\rule{0.16em}{0ex}}1/2$ fractional quantum Hall effect. At density
1/2, our results clarify the phase diagram of the model, while at density
1/4, they provide an explicit construction of the ground-state wavefunction with almost unit overlap with the microscopic one. These findings pave the way to the use of parton wavefunctions to guide the discovery of quantum spin liquids in chiral Rydberg models.
Quantum spin liquids are exotic phases of matter whose low-energy physics is described as the deconfined phase of an emergent gauge theory. With recent theory proposals and an experiment showing preliminary signs of Z 2 topological order [G. Semeghini , ], Rydberg atom arrays have emerged as a promising platform to realize a quantum spin liquid. In this work, we propose a way to realize a U(1) quantum spin liquid in three spatial dimensions, described by the deconfined phase of U(1) gauge theory in a pyrochlore lattice Rydberg atom array. We study the ground state phase diagram of the proposed Rydberg system as a function of experimentally relevant parameters. Within our calculation, we find that by tuning the Rabi frequency, one can access both the confinement-deconfinement transition driven by a proliferation of “magnetic” monopoles and the Higgs transition driven by a proliferation of “electric” charges of the emergent gauge theory. We suggest experimental probes for distinguishing the deconfined phase from ordered phases. This work serves as a proposal to access a confinement-deconfinement transition in three spatial dimensions on a Rydberg-based quantum simulator.
The physics of strongly interacting particles is often extraordinarily rich, leading to the \textit{emergence} of fundamentally new phases and phenomena that cannot exist in the absence of correlations. This thesis is devoted to the study of different classes of quantum systems with such strong correlations. Programmable quantum simulators based on Rydberg atom arrays have recently emerged as versatile platforms to probe quantum many-body phases and their dynamics. In Chapter 2, we start with theories of quantum phase transitions (QPTs) in one-dimensional chains of Rydberg atoms. We demonstrate the existence of a novel QPT in the universality class of the
Z3 chiral clock model, calculate its critical exponents, and discuss their measurement with the quantum Kibble-Zurek mechanism. Proceeding to two dimensions, Chapter 3 describes the zero-temperature phase diagram of a square-lattice Rydberg atom array, revealing several experimentally realizable density-wave-ordered phases and QPTs. For a different geometry, namely, the kagome lattice studied in Chapter 4, we identify a regime that constitutes a likely candidate for hosting a phase with long-range quantum entanglement and topological order. Based on mappings to dimer models and gauge theories, we argue for the existence of a quantum spin liquid phase that has proved elusive in solid-state materials. In the next part of this thesis, we focus on similarly strongly correlated phases in the realm of quantum materials. Motivated by recent observations of an enhanced thermal Hall response in the high-temperature cuprate superconductors, in Chapter 5, we study the thermal Hall conductivity,
κxy, of chiral spin-liquid ans\"{a}tze on the square lattice, focusing on the contribution from neutral (bosonic or fermionic) spinons. Thereafter, going beyond mean-field theory, we consider the corrections due to emergent gauge fields, which yield a response of opposite sign to that of the fermionic matter. We additionally consider the contribution of phonons to
κxy and establish its relation to the spinon Hall viscosity. Thermal Hall measurements also leave intriguing fingerprints in Kitaev materials like
α-RuCl
3, and in this context, Chapter 6 investigates the unquantized
κxy obtained in a gapless spinon Fermi surface state.