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arXiv:2204.00439 · Nature Communications

Pauli blocking of stimulated emission in a degenerate Fermi gas

Raphaël Jannin, Yuri van der Werf, Kees Steinebach, Hendrick L. Bethlem, K. S. E. Eikema

Published Oct 29, 2022• 10 citations
arXivHTMLPDF

Abstract

Abstract The Pauli exclusion principle in quantum mechanics has a profound influence on the structure of matter and on interactions between fermions. Almost 30 years ago it was predicted that the Pauli exclusion principle could lead to a suppression of spontaneous emission, and only recently several experiments confirmed this phenomenon. Here we report that this so-called Pauli blockade not only affects incoherent processes but also, more generally, coherently driven systems. It manifests itself as an intriguing sub-Doppler narrowing of a doubly-forbidden transition profile in an optically trapped Fermi gas of 3 He. By actively pumping atoms out of the excited state, we break the coherence of the excitation and lift the narrowing effect, confirming the influence of Pauli blockade on the transition profile. This insight into the interplay between quantum statistics and coherent driving is a promising development for future applications involving fermionic systems.

DOI
10.1038/s41467-022-34135-6

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Abstract The Pauli exclusion principle in quantum mechanics has a profound influence on the structure of matter and on interactions between fermions. Almost 30 years ago it was predicted that the Pauli exclusion principle could lead to a suppression of spontaneous emission, and only recently several experiments confirmed this phenomenon. Here we report that this so-called Pauli blockade not only affects incoherent processes but also, more generally, coherently driven systems. It manifests itself as an intriguing sub-Doppler narrowing of a doubly-forbidden transition profile in an optically trapped Fermi gas of 3 He. By actively pumping atoms out of the excited state, we break the coherence of the excitation and lift the narrowing effect, confirming the influence of Pauli blockade on the transition profile. This insight into the interplay between quantum statistics and coherent driving is a promising development for future applications involving fermionic systems.
The Pauli exclusion principle forbids indistinguishable fermions from occupying the same quantum mechanical state. The implications of this are profound; for example, it accounts for the electronic shell structure of atoms. Here, we performed measurements on the scattering of light from ultracold ensembles of atoms. For a Fermi gas in the quantum degenerate regime, we observed a marked suppression in scattering compared with a similarly prepared Bose gas. The observed decrease in fluorescence and the corresponding increase in light transmission results from Pauli blocking, where Fermi-Dirac statistics limits the number of accessible states for a scattering atom in a large Fermi sea. Our work confirms a fundamental result on the optical response of quantum gases and may contribute to cooling and thermometry schemes.
A technique is proposed to cool Fermi gases to the regime of quantum degeneracy based on the expected inhibition of spontaneous emission due to the Pauli principle. The reduction of the linewidth for spontaneous emission originates a corresponding reduction of the Doppler temperature, which under specific conditions may give rise to a runaway process through which fermions are progressively cooled. The approach requires a combination of a magneto-optical trap as a cooling system and an optical dipole trap to enhance quantum degeneracy. This results in expected Fermi degeneracy factors T/TFT/{T}_{F}T/TF​ comparable to the lowest values recently achieved, with potential for a direct implementation in optical lattices. The experimental demonstration of this technique should also indirectly provide a macroscopic manifestation of the Pauli exclusion principle at the atomic physics level.
Pauli blocking of spontaneous emission is responsible for the stability of atoms. Electrons cannot decay to lower-lying internal states that are already occupied. Pauli blocking also occurs when free atoms scatter light elastically (Rayleigh scattering) and the final external momentum states are already populated. This was predicted more than 30 years ago but is challenging to realize experimentally. Here, we report on Pauli blocking of light scattering in a dense quantum-degenerate Fermi gas of ultracold lithium atoms. When the Fermi momentum is larger than the photon recoil, most final momentum states are within the Fermi surface. At low temperature, we find that light scattered even at large angles is suppressed by 37% compared with higher temperatures, where atoms scatter at the single-atom Rayleigh scattering rate.
Spontaneous emission by an excited fermionic atom can be suppressed due to the Pauli exclusion principle if the relevant final states after the decay are already occupied by identical atoms in the ground state. Here we discuss a setup where a single atom is prepared in the first excited state on a single site of an optical lattice under conditions of very tight trapping. We investigate these phenomena in the context of two experimental realizations: (1) with alkali-metal atoms, where the decay rate of the excited state is large, and (2) with alkaline-earth-metal-like atoms, where the decay rate from metastable states can be tuned in experiments. This phenomenon has potential applications towards reservoir engineering and dissipative many-body state preparation in an optical lattice.
Lasing [1, 2] and superradiance [3‐5] phenomena are currently enjoying a renaissance as research topics in atomic physics. Fundamentally based on the interaction of matter with an electromagnetic (light) field, the atomic dipoles in a “lasing medium” collectively emit into selected modes of the electromagnetic field and thereby create an amplified and coherent source of light. Present-day lasers use di erent types of gain media and cover a wide range of output frequencies for application in both, fundamental research and industry. A recent string of papers has reported on superradiance [6, 7] and lasing-type instabilities using Bose gases of various type (thermal atoms [8, 9], photon gases [10] and Bose-Einstein condensed atoms [11‐14]) in optical cavities. Buoyed by experimental control over essentially single excitation quanta of atoms and photons [15‐19] in cavity quantum electrodynamics, these works o er intriguing prospects for the next wave of experiments on strongly interacting light-mattter systems including a new regime where unexpected many-body and quantum fluctuation e ects of the lasing medium may become visible. Bohnet et al. [20] recently operated a superradiant “bad-cavity” laser in the few-photon regime based on coherent oscillations of the inter-atomic, collective dipole of the ultracold atoms in the cavity [21]. In this paper, we point out that a quantum degenerate Fermi gas has remarkable features as a lasing medium in a transversally driven cavity as sketched in Fig. 1. We show that the quantum statistics of the Fermi gas puts the coupled cavity+atoms system generically close to superradiance threshold as a consequence of the Pauli exclusion principle (“Pauli pressure”). Physically, this arises from enhanced scattering of fermions between di erent points on the Fermi surface with radiusjkFj by exchanging relatively large photon momenta Q from the cavity as illustrated in Fig. 1. By changing the power of the pump laser at a given density of the Fermi gas, the lasing transition is concomitant with the spontaneous formation of a charge density wave oscillating with 1=Q in real space. Tuning the ratiojkFj=jQj allows to generate a cavity spectrum with “broadband light” in certain spectral ranges or, for energies outside the particle-hole continuum of the fermions, light with relatively narrow linewidth. The normal mode splitting of the cavity by a single atom is completely replaced by many-body Ω |kF| Q
Pauli blocking of spontaneous emission by a single excited-state atom has been predicted to be dramatic at low temperature when the Fermi energy E F exceeds the recoil energy E R . The photon scattering rate of a ground-state Fermi gas can also be suppressed by occupation of the final states accessible to a recoiling atom; however, suppression is diminished by scattering events near the Fermi edge. We analyse two new approaches to improve the visibility of Pauli blocking in a trapped Fermi gas. Focusing the incident light to excite preferentially the high-density region of the cloud can increase the blocking signature by 14%, and is most effective at intermediate temperature. Spontaneous Raman scattering between imbalanced internal states can be strongly suppressed at low temperature, and is completely blocked for a final state E F > 4 E R in the high imbalance limit.