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arXiv:2203.07257

Optical manipulation of matter waves

Kamran Akbari, Valerio Di Giulio, F. Javier Garcı́a de Abajo

Published Mar 14, 2022• 0 citations
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Abstract

Light is extensively used to steer the motion of atoms in free space, enabling cooling and trapping of matter waves through ponderomotive forces and Doppler-mediated photon scattering. Likewise, light interaction with free electrons has recently emerged as a versatile approach to modulate the electron wave function for applications in ultrafast electron microscopy. Here, we combine these two worlds by theoretically demonstrating that matter waves can be optically manipulated via inelastic interactions with optical fields, allowing us to modulate the translational wave function and produce temporally and spatially compressed atomic beam pulses. Specifically, we realize such modulation through stimulated photon absorption and emission by atoms traversing phase-matching evanescent optical fields generated upon light scattering by a nanostructure, but also via stimulated Compton scattering in free space without any assistance from material media. Our results support optical manipulation of matter waves as a powerful tool for microscopy, spectroscopy, and the exploration of novel fundamental phenomena associated with light-atom interactions.

DOI
10.48550/arxiv.2203.07257

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Light is extensively used to steer the motion of atoms in free space, enabling cooling and trapping of matter waves through ponderomotive forces and Doppler-mediated photon scattering. Likewise, light interaction with free electrons has recently emerged as a versatile approach to modulate the electron wave function for applications in ultrafast electron microscopy. Here, we combine these two worlds by theoretically demonstrating that matter waves can be optically manipulated via inelastic interactions with optical fields, allowing us to modulate the translational wave function and produce temporally and spatially compressed atomic beam pulses. Specifically, we realize such modulation through stimulated photon absorption and emission by atoms traversing phase-matching evanescent optical fields generated upon light scattering by a nanostructure, but also via stimulated Compton scattering in free space without any assistance from material media. Our results support optical manipulation of matter waves as a powerful tool for microscopy, spectroscopy, and the exploration of novel fundamental phenomena associated with light-atom interactions.
Light is used to steer the motion of atoms in free space, enabling cooling and trapping of matter waves through ponderomotive forces and Doppler-mediated photon scattering. Likewise, light interaction with free electrons has recently emerged as a versatile approach to modulate the electron wave function for applications in ultrafast electron microscopy. Here, we combine these two worlds, theoretically demonstrating that matter waves can be optically manipulated via inelastic interactions with optical fields. This allows us to modulate the translational part of the wave function and produce temporally and spatially compressed atomic beam pulses. We realize such modulation through stimulated photon absorption and emission by atoms traversing phase-matching evanescent optical fields generated upon light scattering by a nanostructure and via stimulated Compton scattering in free space without any assistance from material media. Our results support optical manipulation of matter waves as a powerful tool for microscopy, spectroscopy, and exploration of fundamental phenomena associated with light-atom interactions.
Light is routinely used to steer the motion of atoms in free space, enabling cooling and trapping of matter waves through ponderomotive interaction and Doppler-mediated photon scattering. In parallel, optical interaction with free electrons has recently emerged as a powerful way to modulate the electron wave function for applications in ultrafast electron microscopy. Here, we combine these two worlds by theoretically demonstrating that matter waves can be optically manipulated by inelastic interaction with optical fields, allowing us to modulate the translational wave function and produce temporally and spatially compressed atomic beam pulses.
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Controlled interaction of laser light with electron beams is fundamental for ultrafast electron microscopy and electron-based quantum optics, yet their direct coupling is forbidden in free space. Here we use longitudinally polarized light at a thin membrane and show that the emerging focal fields can modulate the electron beam in a direct, coherent and linear way, without the need for nanostructured materials or slanted interaction geometries. Also, we use vectorial polarizations to excite and probe three-dimensional nanophotonic near-fields in metallic mesocrystals by coherent electron energy gain and loss. We find that longitudinal electric fields excite axial near-fields in a direct way while longitudinal magnetic fields excite oscillating ring currents via azimuthal electric fields. These possibilities enable tilt-free, collinear generation of attosecond electron pulses or free-electron qubits and provide novel imaging modes in ultrafast electron microscopy and metamaterial tomography.
The long range goal of this project was the creation of nanostructures using light fields to manipulate atoms. By passing an atomic beam through one or more standing wave light fields, it is possible to create modulations in the atomic density having periods which are a fraction of the period of the standing wave light fields. Patterns having periods as small as lambda/10 were observed using optical masks and clear evidence for matter-wave effects were established. Several theoretical methods for achieving sub-lambda matter wave patterns were developed, Moreover it was shown that it is possible to create optical lattices having reduced periodicity using Raman transitions in a novel atom-field geometry Experiments were carried out in both magneto-optical traps and atomic beams. In both experimental set-ups, pulsed standing wave optical fields were used to excite the atoms. At some later time the atoms were probed by a traveling wave field, revealing the spatial patterns that had evolved as a result of the atom-field interaction.
Temporal light modulation methods which are of great practical importance in optical technology, are emulated with matter waves. This includes generation and tailoring of matter-wave sidebands, using amplitude and phase modulation of an atomic beam. In the experiments atoms are Bragg diffracted at standing light fields, which are periodically modulated in intensity or frequency. This gives rise to a generalized Bragg situation under which the atomic matter waves are both diffracted and coherently shifted in their de Broglie frequency. In particular, we demonstrate creation of complex and non-Hermitian matter-wave modulations. One interesting case is a potential with a time-dependent complex helicity $[V\ensuremath{\propto}\mathrm{exp}(i\ensuremath{\omega}t)],$ which produces a purely lopsided energy transfer between the atoms and the photons, and thus violates the usual symmetry between absorption and stimulated emission of energy quanta. Possible applications range from atom cooling over advanced atomic interferometers to a new type of mass spectrometer.