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arXiv:2202.11085 · Physical Review Letters

Dynamical Scaling as a Signature of Multiple Phase Competition in Yb 2 Ti 2 O 7

Allen O. Scheie, Owen Benton, Mathieu Taillefumier, Ludovic D. C. Jaubert, Gabriele Sala, Niina Jalarvo, S. M. Koohpayeh, Nic Shannon

Published Nov 15, 2022• 13 citations
arXivHTMLPDF

Abstract

Yb_{2}Ti_{2}O_{7} is a celebrated example of a pyrochlore magnet with highly frustrated, anisotropic exchange interactions. To date, attention has largely focused on its unusual, static properties, many of which can be understood as coming from the competition between different types of magnetic order. Here we use inelastic neutron scattering with exceptionally high energy resolution to explore the dynamical properties of Yb_{2}Ti_{2}O_{7}. We find that spin correlations exhibit dynamical scaling, analogous to behavior found near to a quantum critical point. We show that the observed scaling collapse can be explained within a phenomenological theory of multiple-phase competition, and confirm that a scaling collapse is also seen in semiclassical simulations of a microscopic model of Yb_{2}Ti_{2}O_{7}. These results suggest that dynamical scaling may be general to systems with competing ground states.

DOI
10.1103/physrevlett.129.217202

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Yb_{2}Ti_{2}O_{7} is a celebrated example of a pyrochlore magnet with highly frustrated, anisotropic exchange interactions. To date, attention has largely focused on its unusual, static properties, many of which can be understood as coming from the competition between different types of magnetic order. Here we use inelastic neutron scattering with exceptionally high energy resolution to explore the dynamical properties of Yb_{2}Ti_{2}O_{7}. We find that spin correlations exhibit dynamical scaling, analogous to behavior found near to a quantum critical point. We show that the observed scaling collapse can be explained within a phenomenological theory of multiple-phase competition, and confirm that a scaling collapse is also seen in semiclassical simulations of a microscopic model of Yb_{2}Ti_{2}O_{7}. These results suggest that dynamical scaling may be general to systems with competing ground states.
The static scaling laws may be generalized to dynamic phenomena by making assumptions on the behavior of time-dependent correlation functions near the magnetic critical point. At any temperature different from Tc, the correlation functions are assumed to reflect the ``hydrodynamic'' behavior of the system, for sufficiently long wavelengths and low frequencies. As the critical temperature is approached, however, the range ξ of spatial correlations in the system diverges, and the domain of applicability of hydrodynamics is reduced to very small wavenumbers, satisfying the inequality kξ≪1. The dynamic scaling assumptions relate the behavior of the time-dependent correlation functions in the ``hydrodynamic'' (kξ≪1) and ``critical'' (kξ≫1) regions. It is thus possible to predict certain features of the dynamic behavior at Tc, from a knowledge of the behavior away from Tc. Application is made to the spin-correlation function of the isotropic Heisenberg antiferromagnet, which is directly measurable by inelastic neutron scattering. Detailed predictions are presented on the form of the cross section as a function of energy and momentum transfer, and of temperature near Tc.
We report inelastic neutron scattering measurements of the magnetic excitations in Ba2CuTeO6{\mathrm{Ba}}_{2}{\mathrm{CuTeO}}_{6}Ba2​CuTeO6​, proposed by ab initio calculations to magnetically realize weakly coupled antiferromagnetic two-leg spin-12\frac{1}{2}21​ ladders. Isolated ladders are expected to have a singlet ground state protected by a spin gap. Ba2CuTeO6{\mathrm{Ba}}_{2}{\mathrm{CuTeO}}_{6}Ba2​CuTeO6​ orders magnetically, but with a small N\'eel temperature relative to the exchange strength, suggesting that the interladder couplings are relatively small and only just able to stabilize magnetic order, placing Ba2CuTeO6{\mathrm{Ba}}_{2}{\mathrm{CuTeO}}_{6}Ba2​CuTeO6​ close in parameter space to the critical point separating the gapped phase and N\'eel order. Through comparison of the observed spin dynamics with linear spin wave theory and quantum Monte Carlo calculations, we propose values for all relevant intra- and interladder exchange parameters, which place the system on the ordered side of the phase diagram in proximity to the critical point. We also compare high field magnetization data with quantum Monte Carlo predictions for the proposed model of coupled ladders.
In this thesis we examine universal scaling properties of strongly-correlated systems near and far from equilibrium. We discuss quantum phase transitions at vanishing temperature, multicritical and dynamic critical behavior near thermal equilibrium, and scaling properties of nonequilibrium steady states. We employ nonperturbative methods including the functional renormalization group as well as Monte Carlo simulations. A general outline of the functional renormalization group is given in the introductory chapters. \n \nIn the first part of this thesis, we investigate spinless fermions on the honeycomb lattice interacting via short-range repulsive interactions. Such a system can be seen as a simple model for suspended graphene. The short-range interactions control the ground state properties of the system that may lead to a chiral phase transition from the semimetal to the charge density wave (CDW)/Kekulé ordered state. We determine the universal scaling properties at the chiral transition, and establish the presence of large anomalous dimensions indicating the importance of strong fluctuations. \n \nThe competition of two nonvanishing order parameters and their corresponding multicritical behavior are investigated in the subsequent chapter. We characterize the bicritical and tetracritical behavior in the purely bosonic O(N_1) + O(N_2) symmetric model and comment on possible applications to condensed-matter and high-energy physics. \n \nIn the following chapter we discuss the long-time relaxational behavior at criticality of an order parameter with O(N) symmetry coupled to an additional conserved density. We find an anomalous diffusion phase with new dynamic scaling properties. Using the functional renormalization group we determine the complete dynamic critical behavior of the model in 2 < d < 4 dimensions and compare our results to experiments. \n \nFinally, we investigate the scaling properties of stationary states far from equilibrium. At the example of the one-dimensional Burgers’ equation we develop a novel approach to hydrodynamic turbulence using lattice Monte Carlo methods. We apply these techniques to determine the statistical properties of small-scale fluctuations in this model and identify the anomalous scaling behavior. \n
We resolve the nature of the quantum phase transition between antiferromagnetic and valence-bond solid ground states in square-lattice spin-1/2 magnets - the putative deconfined quantum-critical point. Using quantum Monte Carlo simulations of J-Q models, in which Heisenberg exchange J competes with multi-spin interactions Qn formed by n singlet projectors, we demonstrate first-order discontinuities increasing with n. For n=2 and n=3, the first-order signatures are very weak and we extract universal scaling dimensions of a proximate multicritical point. Their values coincide closely with known bounds for an SO(5) symmetric conformal field theory (CFT) containing a relevant SO(5) singlet operator that destabilizes the generic deconfined critical point. We characterize the emergent SO(5) symmetry by its scaling dimensions of the leading irrelevant perturbations. Using the J-Q2-Q6 model, we tune the transition from weak to stronger first-order and find scaling of the coexisting order parameters with a large exponent beta ~ 0.85, in agreement with the relevant scaling dimensions of the multicritical point. The exponent that had previously been identified with the correlation length does not have a corresponding CFT level, and we explain it as pseudo-critical length scale of bubbles of one phase inside the other that are compressed in size by an SO(5)-violating irrelevant repulsive interaction between the two order parameters. The bubble scale reflects a hierarchy of excitation gaps generated by the SO(5) perturbation in the neighborhood of the first-order transition, akin to a Higgs mechanism. We argue that the multicritical point is the tip of a gapless spin liquid phase in frustrated Heisenberg models into which the J-Q models can be deformed, but the spin liquid, and perhaps the multicritical point itself, exist outside the regime amenable to sign-free simulations.
In this PhD thesis, the physics of quantum critical matter and exotic quantum state close to quantum phase transitions is investigated. We will focus on three different examples that highlight some of the interesting phenomena related to quantum phase transitions. Firstly, we discuss the physics of quantum phase transitions in quantum wires as a function of an external gate voltage when new subbands are activated. We find that at these transitions, strong correlations lead to the formation of an impenetrable gas of polarons, and identify criteria for possible instabilities in the spin- and charge sectors of the model. Our analysis is based on the combination of exact resummations, renormalization group techniques and Luttinger liquid approaches. \n \nSecondly, we turn to the physics of multiple divergent time scales close to a quantum critical point. Using an appropriately generalized renormalization group approach, we identify that the presence of multiple dynamics at a quantum phase transition can lead to the emergence of new critical scaling exponents and thus to the breakdown of the ususal scaling schemes. We calculate the critical behavior of various thermodynamic properties and detail how unusual physics can arise. It is hoped that these results might be helpful for the interpretation of experimental scaling puzzles close to quantum critical points. \n \nThirdly, we turn to the physics of topological transitions, and more precisely the physics of Weyl superconductors. The latter are the superconducting variant of the topologically non-trivial Weyl semimetals, and emerge at the quantum phase transition between a topological superconductor and a normal insulator upon perturbing the transition with a time reversal symmetry breaking perturbation, such as magnetism. We characterize the topological properties of Weyl superconductors and establish a topological phase diagram for a particular realization in heterostructures. We discuss the physics of vortices in Weyl superconductors, and establish under which conditions they can trap zero energy Majorana modes. Our disucssion ends with some remarks on possible experimental signatures.
By means of inelastic neutron scattering we investigate finite temperature dynamics in the quantum spin ladder compound (C_{5}H_{12}N)_{2}CuBr_{4} (BPCB) near the magnetic field induced quantum critical point with dynamical exponent z=2. We observe universal finite-temperature scaling of the transverse local dynamic structure factor in spectacular quantitative agreement with long-standing theoretical predictions. At the same time, already at rather low temperatures, we observe strong nonuniversal longitudinal fluctuations. To separate the two, we make use of an intrinsic leg-exchange symmetry of the spin ladder. Complementary measurements of specific heat also reveal striking scaling behavior near the quantum critical point.