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arXiv:2202.03063 · Journal of Mathematical Physics

Proper condensates and long range order

Detlev Buchholz A

Published Aug 1, 2022• 3 citations
arXivHTMLPDF

Abstract

Within the framework of the algebra of canonical commutation relations in position space, a long range order between particles in bounded regions is established in states with a sufficiently large particle number. It occurs whenever homogeneous proper (infinite) condensates form locally in the states in the limit of infinite densities. The condensates are described by eigenstates of the momentum operator, covering also those cases where they are streaming with a constant velocity. The arguments given are model independent and lead to a new criterion for the occurrence of condensates. It makes use of a novel approach to the identification of condensates, based on a characterization of regular and singular wave functions.

DOI
10.1063/5.0087983

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Journal of Mathematical Physics•Jul 1, 1965•29 citations
Within the framework of the algebra of canonical commutation relations in position space, a long range order between particles in bounded regions is established in states with a sufficiently large particle number. It occurs whenever homogeneous proper (infinite) condensates form locally in the states in the limit of infinite densities. The condensates are described by eigenstates of the momentum operator, covering also those cases where they are streaming with a constant velocity. The arguments given are model independent and lead to a new criterion for the occurrence of condensates. It makes use of a novel approach to the identification of condensates, based on a characterization of regular and singular wave functions.
In this article, a novel characterization of Bose–Einstein condensates is proposed. Instead of relying on occupation numbers of a few dominant modes, which become macroscopic in the limit of infinite particle numbers, it focuses on the regular excitations whose numbers stay bounded in this limit. In this manner, subspaces of global, respectively, local regular wave functions are identified. Their orthogonal complements determine the wave functions of particles forming proper (infinite) condensates in the limit. In contrast to the concept of macroscopic occupation numbers, which does not sharply fix the wave functions of condensates in the limit states, the notion of proper condensates is unambiguously defined. It is outlined how this concept can be used in the analysis of condensates in models. The method is illustrated by the example of trapped non-interacting ground states and their multifarious thermodynamic limits, differing by the structure of condensates accompanying the Fock vacuum. The concept of proper condensates is also compared with the Onsager–Penrose criterion based on the analysis of eigenvalues of one-particle density matrices. It is shown that the concept of regular wave functions is also useful in that approach for the identification of wave functions forming proper condensates.
In this article a novel characterization of Bose-Einstein condensates is proposed. Instead of relying on occupation numbers of a few dominant modes, which become macroscopic in the limit of infinite particle numbers, it focuses on the regular excitations whose numbers stay bounded in this limit. In this manner, subspaces of global, respectively local regular wave functions are identified. Their orthogonal complements determine the wave functions of particles forming proper (infinite) condensates in the limit. In contrast to the concept of macroscopic occupation numbers, which does not sharply fix the wave functions of condensates in the limit states, the notion of proper condensates is unambiguously defined. It is outlined, how this concept can be used in the analysis of condensates in models. The method is illustrated by the example of trapped non-interacting ground states and their multifarious thermodynamic limits, differing by the structure of condensates accompanying the Fock vacuum. The concept of proper condensates is also compared with the Onsager-Penrose criterion, based on the analysis of eigenvalues of one-particle density matrices. It is shown that the concept of regular wave functions is useful there as well for the identification of wave functions forming proper condensates.
The existence of a Bose-Einstein condensation in an interacting many-boson system at T = 0°K is proved under certain conditions on the particle density and the interparticle potential. Starting with the tentative assumption that the condensation exists, we study the fluctuation in the occupation number of the condensate with due regard to its interactions (1) with particles outside the condensate as well as (2) with the fluctuation itself. If the condensate fluctuation has a normalizable ground state, then the assumed existence of the condensation is tenable. For the case of the pair-Hamiltonian model satisfying the conditions for condensation, the interactions of the second category are of no importance. In the limit of infinite volume, this Hamiltonian can be diagonalized in an irreducible representation of a Bose-field operatorφ(x), whereφ(x) has nonvanishing ground state expectation value, in accordance with the usual c-number replacement of creation and destruction operators for the condensate particles. The full Hamiltonian for a system of pairwise interacting bosons is studied only in a low-density limit. Bose-Einstein condensation exists when the over-all space integral of the interparticle potential is positive. In this case the interactions of the second category play an important role in ensuring a normalizable ground state for the condensate fluctuation. There is an indication that in the limit of infinite volume the Hamiltonian cannot be diagonalized in any irreducible representation of the field operatorφ. Yet the c-number replacement of the condensate operators is legitimate as far as states of particles outside the condensate are concerned. Some speculations are made as to what may happen for systems of moderate density.
Abstract Finite Bose systems cannot display a genuine Bose–Einstein condensate with infinite long-range order. But, if the number of trapped atoms is sufficiently large, a kind of Bose–Einstein condensation does occur, with the properties of the arising quasi-condensate being very close to the genuine condensate. Although the quasi-condensate does not enjoy long-range order, it has mid-range order. This paper shows that the level of mid-range order in finite Bose systems can be characterized by order indices of density matrices.
The limit states of canonical ensembles of a large number of interacting bosons at a given temperature, which are confined by harmonic forces, are studied in the framework of the resolvent algebra. It is shown that the limits satisfy the KMS condition or are ground states, regardless of the type of interaction. In case of attractive forces, where the ensembles collapse, observables that become meaningless in the limit disappear from the limit representations. For repulsive forces, this can also happen if condensates with an infinite number of particles in the same state (proper condensates) appear in the limit. The resulting structures and their interpretation are illustrated by a simple model. The study of vanishing harmonic forces (thermodynamic limit) involves changes of the dynamics. It is conveniently based on derivations acting on the algebra. They are given by the commutator of the Hamiltonians with the elements of the algebra. To ensure that the images remain in the algebra, the interaction must be regularized. This is accomplished in a manner that has only a minor impact on the dynamics and may be of broader interest. With this input a relation between the strength of the confining harmonic forces and the number of particles in the ensembles is derived from the condition that the limit states are to be stationary (invariant) under the adjoint action of the unconfined, spatially homogeneous limit dynamics. This relation encompasses the conditions that are frequently used in studies of Bose-Einstein condensates.
It is shown for boson systems with periodic boundary conditions that the existence of generalized Bose condensation, of which the simple type typified by the ideal Bose gas is a special case, is equivalent to the existence of off-diagonal long-range order (ODLRO) in the single-particle density matrix ρ1 provided that the two noncomuting limits involved in the criterion for ODLRO are taken in the proper order: first size of system → ∞, then interparticle separation → ∞. It is shown by means of an example that certain assumptions concerning the behavior of the single-particle momentum distribution function involved in proving this equivalence are actually satisfied in thermal equilibrium for some dynamical models. The analysis is generalized to box-enclosure boundary conditions by an extension of an argument due to Schafroth, according to which box-enclosure conditions are equivalent to homogeneous Neumann conditions except for a thermodynamically negligible surface effect, provided that one second-quantizes with respect to Hartree-Fock orbitals rather than free-particle orbitals. A general criterion for generalized Bose condensation in terms of eigenvalues of ρ1 is proposed. On the basis of the behavior of soluble models it is conjectured that for a boson system in thermal equilibrium subject to arbitrary boundary conditions, the existence of such Bose condensation is equivalent to the existence of ODLRO in ρ1. The two-particle density matrix ρ2 is discussed briefly. By means of a simplified model it is shown that for a Bose system generalized condensation implies large eigenvalues of ρ2 and ODLRO of ρ2, just as for ρ1. It is pointed out that the question of the existence or nonexistence of generalized Bose condensation of fermion pairs ought to be investigated.