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arXiv:2202.00306 · Journal of Physics Photonics

Cryogenic electro-optic modulation in titanium in-diffused lithium niobate waveguides

Frederik Thiele, Felix vom Bruch, Julian Brockmeier, Maximilian Protte, Thomas Hummel, Raimund Ricken, Viktor Quiring, Sebastian Lengeling, Harald Herrmann, Christof Eigner, Christine Silberhorn, Tim J. Bartley

Published May 3, 2022• 12 citations
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Abstract

Abstract Lithium niobate is a promising platform for integrated quantum optics. In this platform, we aim to efficiently manipulate and detect quantum states by combining superconducting single photon detectors and modulators. The cryogenic operation of a superconducting single photon detector dictates the optimisation of the electro-optic modulators under the same operating conditions. To that end, we characterise a phase modulator, directional coupler, and polarisation converter at both ambient and cryogenic temperatures. The operation voltage V π / 2 of these modulators increases, due to the decrease in the electro-optic effect, by 74% for the phase modulator, 84% for the directional coupler and 35% for the polarisation converter below 8.5 K . The phase modulator preserves its broadband nature and modulates light in the characterised wavelength range. The unbiased bar state of the directional coupler changed by a wavelength shift of 85 n m while cooling the device down to 5 K . The polarisation converter uses periodic poling to phasematch the two orthogonal polarisations. The phasematched wavelength of the utilised poling changes by 112 n m when cooling to 5 K .

DOI
10.1088/2515-7647/ac6c63

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Abstract Lithium niobate is a promising platform for integrated quantum optics. In this platform, we aim to efficiently manipulate and detect quantum states by combining superconducting single photon detectors and modulators. The cryogenic operation of a superconducting single photon detector dictates the optimisation of the electro-optic modulators under the same operating conditions. To that end, we characterise a phase modulator, directional coupler, and polarisation converter at both ambient and cryogenic temperatures. The operation voltage V π / 2 of these modulators increases, due to the decrease in the electro-optic effect, by 74% for the phase modulator, 84% for the directional coupler and 35% for the polarisation converter below 8.5 K . The phase modulator preserves its broadband nature and modulates light in the characterised wavelength range. The unbiased bar state of the directional coupler changed by a wavelength shift of 85 n m while cooling the device down to 5 K . The polarisation converter uses periodic poling to phasematch the two orthogonal polarisations. The phasematched wavelength of the utilised poling changes by 112 n m when cooling to 5 K .
The realisation of light modulation based on single photon detection events is an important step towards feed-forward-modulation, which is required for many quantum optics protocols. This requires combining detection events with modulation in a device with a small physical footprint, for which integrated optics is ideal. Several platforms for integrated quantum optics have been developed to generate, modulate, and detect quantum features in the light over the last years. Titanium in-diffused waveguides in lithium niobate is a promising candidate for quantum communication applications [1] , [2] , however, single photon detection with superconducting photon detectors (SNSPDs) require cryogenic temperatures. Therefore, optimising the nonlinear optical properties of these waveguides under cryogenic operating conditions is an important task. Previously, we have demonstrated frequency conversion [3] , electro-optical modulation [4] and integrated single photon detection [5] at cryogenic temperatures.
Integrated quantum photonic devices require the combination of quantum light sources, elements for guiding and manipulating the photonic states and detectors [1] . In a fully-integrated platform, the operating conditions for each component must be mutually compatible. Whilst parametric down-conversion (PDC) as a source for photonic states is well-established under ambient conditions [2] , other quantum photonic technologies require cryogenic operation temperatures, in particular superconducting single-photon detectors [3] .
Lithium Niobate On Insulator (LNOI) has recently emerged as a promising platform for the realization of electro-optically reconfigurable waveguides combining small footprint and ultra-low propagation loss. Integration of these components with superconducting nanowire single photon detectors (SNSPDs) opens up the possibility to perform on-chip manipulation and detection of quantum states of light in a physically stable and scalable architecture. Here we report recent theoretical and experimental progress towards the realization of fast electro-optic modulators compatible with cryogenic temperatures and high-performance NbTiN superconducting nanowires single-photon detectors (SNSPDs) monolithically integrated in LNOI waveguides.
Photonic integrated circuits operating at cryogenic temperatures are necessary for many quantum technologies such as quantum transduction, integrated single-photon emitters and detectors, as well as deep-space communication and sensing devices. Thin-film lithium niobate (TFLN) is an emerging platform that is a strong candidate for fully integrated quantum photonics, offering low loss, fast electro-optic reconfigurability, nonlinear quantum light sources, and the ability to host quantum emitters and single-photon detectors. To interface TFLN with technologies that require cryogenic operation, like superconducting single-photon detectors, microwave-to-optical transducers, and solid-state quantum emitters, it is important to study its optical and electrical properties from room temperature down to cryogenic temperatures. Here, we investigate linear and nonlinear photonic devices, including racetrack resonators, Mach-Zehnder modulators and periodically poled waveguides in TFLN using a cryogenic fiber probe station with full temperature control down to 5 K. We quantify a shift in resonances, a 22% increase in electro-optic modulator half-wave voltage, a blue shift of 18 nm for Type-0 phase-matching as well as a red shift of 64 nm for Type-II phase-matching as the sample temperature decreases. Our study of nonlinear processes in a cryogenic environment will contribute towards developing novel devices for inter-platform quantum information processing, secure communication, and enhanced sensing.
Lithium-Niobate-On-Insulator (LNOI) is emerging as a promising platform for integrated quantum photonic technologies because of its high second-order nonlinearity and compact waveguide footprint. Importantly, LNOI allows for creating electro-optically reconfigurable circuits, which can be efficiently operated at cryogenic temperature. Their integration with superconducting nanowire single-photon detectors (SNSPDs) paves the way for realizing scalable photonic devices for active manipulation and detection of quantum states of light. Here we demonstrate integration of these two key components in a low loss (0.2 dB/cm) LNOI waveguide network. As an experimental showcase of our technology, we demonstrate the combined operation of an electrically tunable Mach-Zehnder interferometer and two waveguide-integrated SNSPDs at its outputs. We show static reconfigurability of our system with a bias-drift-free operation over a time of 12 hours, as well as high-speed modulation at a frequency up to 1 GHz. Our results provide blueprints for implementing complex quantum photonic devices on the LNOI platform.
Abstract Lithium niobate has emerged as a promising platform for integrated quantum optics, enabling efficient generation, manipulation, and detection of quantum states of light. However, integrating single-photon detectors requires cryogenic operating temperatures, since the best performing detectors are based on narrow superconducting wires. While previous studies have demonstrated the operation of quantum light sources and electro-optic modulators in LiNbO3 at cryogenic temperatures, the thermal transition between room temperature and cryogenic conditions introduces additional effects that can significantly influence device performance. In this paper, we investigate the generation of pyroelectric charges and their impact on the optical properties of lithium niobate waveguides when changing from room temperature to 25 K, and vice versa. We measure the generated pyroelectric charge flow and correlate this with fast changes in the birefringence acquired through the Sénarmont-method. Both electrical and optical influence of the pyroelectric effect occur predominantly at temperatures above 100 K.