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arXiv:2201.12517 · Physical review. B./Physical review. B

Thermally enhanced Majorana-mediated spin transport in the Kitaev model

Hirokazu Taguchi, Yuta Murakami, Akihisa Koga

Published Mar 28, 2022• 8 citations
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Abstract

We study how stable the Majorana-mediated spin transport in a quantum spin Kitaev model is against thermal fluctuations. Using the time-dependent thermal pure quantum state method, we examine finite-temperature spin dynamics in the Kitaev model. The model exhibits two characteristic temperatures, ${T}_{L}$ and ${T}_{H}$, which correspond to energy scales of the local flux and the itinerant Majorana fermion, respectively. At low temperatures $(T\ensuremath{\ll}{T}_{L})$, an almost flux-free state is realized, and the spin excitation propagates in a similar way to that for the ground state. Namely, after the magnetic pulse is introduced at one of the edges, the itinerant Majorana fermions propagate the spin excitations even through the quantum spin liquid state region, and oscillations in the spin moment appear in the other edge with a tiny magnetic field. When $T\ensuremath{\sim}{T}_{L}$, larger oscillations in the spin moments are induced in the other edge, compared with the results at the ground state. At higher temperatures, excited ${Z}_{2}$ fluxes disturb the coherent motion of the itinerant Majorana fermions, which suppresses the spin propagation. Our results demonstrate a crucial role of thermal fluctuations in the Majorana-mediated spin transport.

DOI
10.1103/physrevb.105.125137

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We study how stable the Majorana-mediated spin transport in a quantum spin Kitaev model is against thermal fluctuations. Using the time-dependent thermal pure quantum state method, we examine finite-temperature spin dynamics in the Kitaev model. The model exhibits two characteristic temperatures, TL{T}_{L}TL​ and TH{T}_{H}TH​, which correspond to energy scales of the local flux and the itinerant Majorana fermion, respectively. At low temperatures (T\ensuremath≪TL)(T\ensuremath{\ll}{T}_{L})(T\ensuremath≪TL​), an almost flux-free state is realized, and the spin excitation propagates in a similar way to that for the ground state. Namely, after the magnetic pulse is introduced at one of the edges, the itinerant Majorana fermions propagate the spin excitations even through the quantum spin liquid state region, and oscillations in the spin moment appear in the other edge with a tiny magnetic field. When T\ensuremath∼TLT\ensuremath{\sim}{T}_{L}T\ensuremath∼TL​, larger oscillations in the spin moments are induced in the other edge, compared with the results at the ground state. At higher temperatures, excited Z2{Z}_{2}Z2​ fluxes disturb the coherent motion of the itinerant Majorana fermions, which suppresses the spin propagation. Our results demonstrate a crucial role of thermal fluctuations in the Majorana-mediated spin transport.
We study the spin transport through the quantum spin liquid (QSL) by investigating the real-time and real-space dynamics of the Kitaev spin system with zigzag edges using the time-dependent Majorana mean-field theory. After the magnetic-field pulse is introduced to one of the edges, spin moments are excited in the opposite edge region although spin moments are never induced in the Kitaev QSL region. This unusual spin transport originates from the fact that the S=1/2 spins are fractionalized into the itinerant and localized Majorana fermions in the Kitaev system. Although both Majorana fermions are excited by the magnetic pulse, only the itinerant ones flow through the bulk regime without spin excitations, resulting in the spin transport in the Kitaev system despite the presence of a nonzero spin gap. We also demonstrate that this phenomenon can be observed in the system with small Heisenberg interactions using the exact diagonalization.
The Kitaev model exhibits a canonical quantum spin liquid as a ground state and hosts two fractional quasiparticles, i.e., itinerant Majorana fermion and localized flux excitation. The former can carry heat and spin modulations in the quantum spin liquid, but the role of the latter remains unknown for the transport phenomena. Here, we focus on spin transport in the presence of excited fluxes and report that they yield strong interference in the propagation of the Majorana fermions, which have a gaugelike potential emergent around the fluxes. We examine the transient spin dynamics triggered by a pulsed magnetic field at an edge. In the absence of excited fluxes, the magnetic-field pulse creates the plane wave of the Majorana fermions, which flows in the quantum spin liquid. Although this wave does not accompany the change of local spin moments in bulk, it induces local moments at the side opposite to the edge under the magnetic-field pulse. We observe the spatial modulation of induced spin moments when fluxes are excited in the bulk region. This behavior is more striking than the case of lattice defects. Moreover, we find that although the amplitude of the spatial change is almost independent of the distance between lattice defects, it is strongly enhanced by increasing the distance for the case of excited fluxes. The difference is understood from the influence on the itinerant Majorana fermions; the lattice defects change the system locally, but flux excitations alter all the transfer integrals on the string connecting them. The present results will provide another route to observing intrinsic flux excitations distinguished from extrinsic effects such as lattice defects.
Thermal Fractionalization of Quantum Spins in a Kitaev Model: Coherent Transport of Majorana Fermions and TTT-linear Specific Heat
Finite-temperature (TTT) properties of a Kitaev model defined on a honeycomb lattice are investigated by a quantum Monte Carlo simulation, from the viewpoint of fractionalization of quantum S=1/2S=1/2S=1/2 spins into two types of Majorana fermions, itinerant and localized. In this system, the entropy is released successively at two well-separated TTT scales, as a clear indication of the thermal fractionalization. We show that the high-TTT crossover, which is driven by itinerant Majorana fermions, is closely related with the development of nearest-neighbor spin correlations. On the other hand, the low-TTT crossover originates in thermal fluctuations of fluxes composed of localized Majorana fermions, by which the spectrum of itinerant Majorana fermions is significantly disturbed. As a consequence, in the intermediate-TTT range, the system exhibits coherent transport of Majorana fermions and TTT-linear behavior in the specific heat, despite the Dirac semimetallic spectrum in the low-TTT limit. We also show that the flux fluctuations affect the gapless-gapped phase boundary. Our results indicate that the fractionalization is experimentally observable in spin correlations, specific heat, and transport properties.
The Kitaev model offers a platform for quantum spin liquids (QSLs) with fractional excitations, itinerant Majorana fermions and localized fluxes. Since these fractional excitations could be utilized for quantum computing, how to create, observe, and control them through the spin degree of freedom is a central issue. Here, we study dynamical spin transport in a wide range of frequencies for the Kitaev-Heisenberg model, by applying an AC magnetic field to an edge of the system. We find that, in the Kitaev QSL phase, spin polarizations at the other edge are resonantly induced in a specific spin component, even though the static spin correlations are vanishingly small. This interedge spin resonance appears around the input frequency over the broad frequency range. Comparing with the dynamical spin correlations, we clarify that the resonance is governed by the itinerant Majorana fermions with a broad continuum excitation spectrum, which can propagate over long distances, although it vanishes for the pure Kitaev model because of accidental degeneracy and requires weak Heisenberg interactions. We also find that the spin polarizations in the other spin components are weakly induced at an almost constant frequency close to the excitation gap of the localized fluxes, irrespective of the input frequency. These results demonstrate that the dynamical spin transport is a powerful probe of the fractional excitations in the Kitaev QSL. Possible experimental realization of the interedge spin resonance is discussed.
We investigate the real-time spin response of the S=1S=1S=1 Kitaev model upon stimuli of a pulsed magnetic field in one of the edges using the exact diagonalization method. It is found that the pulsed magnetic field has no effect on the appearance of the spin moments in the quantum spin liquid region, but induces the spin oscillations in the other edge region with a small magnetic field. This is understood by the existence of the itinerant quasiparticles, which carry the spin excitations without the spin polarization in the quantum spin liquid state. This suggests that the spin fractionalizations occur in the S=1S=1S=1 Kitaev model as well as the exactly solvable S=1/2S=1/2S=1/2 Kitaev one and the fractionalized quasiparticles play an essential role in the spin transport.
The long-sought quantum spin liquid is a quantum-entangled magnetic state leading to the fractionalization of spin degrees of freedom. Quasiparticles emergent from the fractionalization affect not only the ground-state properties but also thermodynamic behavior in a peculiar manner. Here we investigate how the spin dynamics evolves from the high-temperature paramagnet to the quantum spin-liquid ground state, for the Kitaev spin model describing the fractionalization into itinerant matter fermions and localized Z2{Z}_{2}Z2​ fluxes. Beyond the previous studies [J. Yoshitake, J. Nasu, and Y. Motome, Phys. Rev. Lett. 117, 157203 (2016); J. Yoshitake, J. Nasu, Y. Kato, and Y. Motome, Phys. Rev. B 96, 024438 (2017)], in which the mean-field nature of the cluster dynamical mean-field theory prevented us from studying low-temperature properties, we develop a numerical technique by applying the continuous-time quantum Monte Carlo (CTQMC) method to statistical samples generated by the quantum Monte Carlo (QMC) method in a Majorana fermion representation. This QMC+CTQMC method is fully unbiased and enables us to investigate the low-temperature spin dynamics dominated by thermally excited Z2{Z}_{2}Z2​ fluxes, including the unconventional phase transition caused by Z2{Z}_{2}Z2​ flux loops in three dimensions, which was unreachable by the previous methods. We apply this technique to the Kitaev model in both two and three dimensions. Our results clearly distinguish two cases: while the dynamics changes smoothly through the crossover in the two-dimensional honeycomb case, it exhibits singular behaviors at the phase transition in the three-dimensional hyperhoneycomb case. We show that the low-temperature spin dynamics is a sensitive probe for thermally fluctuating Z2{Z}_{2}Z2​ fluxes that behave very differently between two and three dimensions.