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arXiv:2201.09469 · Physical Review Letters

Non-Hermitian Absorption Spectroscopy

Kai Li, Yong Xu

Published Aug 26, 2022• 35 citations
arXivHTMLPDF

Abstract

While non-Hermitian Hamiltonians have been experimentally realized in cold atom systems, it remains an outstanding open question of how to experimentally measure their complex energy spectra in momentum space for a realistic system with boundaries. The existence of non-Hermitian skin effects may make the question even more difficult to address given the fact that energy spectra for a system with open boundaries are dramatically different from those in momentum space; the fact may even lead to the notion that momentum-space band structures are not experimentally accessible for a system with open boundaries. Here, we generalize the widely used radio-frequency spectroscopy to measure both real and imaginary parts of complex energy spectra of a non-Hermitian quantum system for either bosonic or fermionic atoms. By weakly coupling the energy levels of a non-Hermitian system to auxiliary energy levels, we theoretically derive a formula showing that the decay of atoms on the auxiliary energy levels reflects the real and imaginary parts of energy spectra in momentum space. We further prove that measurement outcomes are independent of boundary conditions in the thermodynamic limit, providing strong evidence that the energy spectrum in momentum space is experimentally measurable. We finally apply our non-Hermitian absorption spectroscopy protocol to the Hatano-Nelson model and non-Hermitian Weyl semimetals to demonstrate its feasibility.

DOI
10.1103/physrevlett.129.093001

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While non-Hermitian Hamiltonians have been experimentally realized in cold atom systems, it remains an outstanding open question of how to experimentally measure their complex energy spectra in momentum space for a realistic system with boundaries. The existence of non-Hermitian skin effects may make the question even more difficult to address given the fact that energy spectra for a system with open boundaries are dramatically different from those in momentum space; the fact may even lead to the notion that momentum-space band structures are not experimentally accessible for a system with open boundaries. Here, we generalize the widely used radio-frequency spectroscopy to measure both real and imaginary parts of complex energy spectra of a non-Hermitian quantum system for either bosonic or fermionic atoms. By weakly coupling the energy levels of a non-Hermitian system to auxiliary energy levels, we theoretically derive a formula showing that the decay of atoms on the auxiliary energy levels reflects the real and imaginary parts of energy spectra in momentum space. We further prove that measurement outcomes are independent of boundary conditions in the thermodynamic limit, providing strong evidence that the energy spectrum in momentum space is experimentally measurable. We finally apply our non-Hermitian absorption spectroscopy protocol to the Hatano-Nelson model and non-Hermitian Weyl semimetals to demonstrate its feasibility.
We develop a generalized Aufbau principle for non-Hermitian systems that allows for building up the configurations of indistinguishable particles. The Aufbau rule of non-Hermitian systems is unexpectedly shown to be identical to that developed in Hermitian systems when the real parts of the complex energy levels are considered. We derive full many-body energy spectra of the fermionic and bosonic Hatano-Nelson models as examples by filling single-particle energy levels in the momentum space. For open boundary conditions, we show that many-body non-Hermitian skin effects persist in all many-body eigenstates for both fermions and bosons. Furthermore, we find surprisingly that the ground state of bosons is an anomalous Bose-Einstein condensation with all of the particles simultaneously localizing in both the real and momentum space beyond the Heisenberg uncertainty principle. For periodic boundary conditions, we show that hard-core bosons cannot be mapped to fermions. This work establishes a general framework for understanding the many-body physics of non-Hermitian systems, revealing rich unique non-Hermitian many-body physics.
Non-Hermitian systems generically have complex energies, which may host topological structures, such as links or knots. While there has been great progress in experimentally engineering non-Hermitian models in quantum simulators, it remains a significant challenge to experimentally probe complex energies in these systems, thereby making it difficult to directly diagnose complex-energy topology. Here, we experimentally realize a two-band non-Hermitian model with a single trapped ion whose complex eigenenergies exhibit the unlink, unknot, or Hopf link topological structures. Based on non-Hermitian absorption spectroscopy, we couple one system level to an auxiliary level through a laser beam and then experimentally measure the population of the ion on the auxiliary level after a long period of time. Complex eigenenergies are then extracted, illustrating the unlink, unknot, or Hopf link topological structure. Our work demonstrates that complex energies can be experimentally measured in quantum simulators via non-Hermitian absorption spectroscopy, thereby opening the door for exploring various complex-energy properties in non-Hermitian quantum systems, such as trapped ions, cold atoms, superconducting circuits, or solid-state spin systems.
Non-Hermitian systems exhibit unique spectral properties, including the non-Hermitian skin effect and exceptional points, often influenced by boundary conditions. The modulation of these phenomena by generalized boundary conditions remains unexplored and not understood. Here, we analyze the Hatano-Nelson model with generalized boundary conditions induced by complex hopping amplitudes at the boundary. Using similarity transformations, we determine the conditions yielding real energy spectra and skin effect, and identify the emergence of exceptional points where spectra transition from real to complex. We demonstrate that tuning the boundary hopping amplitudes precisely controls the non-Hermitian skin effect, i.e., the localization of eigenmodes at the lattice edges. These findings reveal the sensitivity of spectral and localization properties to boundary conditions, providing a framework for engineering quantum lattice models with tailored spectral and localization features, with potential applications in quantum devices.
In general, the energy spectrum of a non-Hermitian system turns out to be complex, which is not very satisfactory since the time evolution of eigenstates with complex eigenvalues is either exponentially growing or decaying. Here, we provide a sufficient and necessary condition of the real spectrum under open boundary conditions for one-dimensional non-Hermitian tight-binding Hamiltonians. The necessity is directly related to the fact that the generalized Brillouin zone in one dimension is a closed loop whose origin is in its interior. We also establish the sufficiency by analytically determining when the preimage of the characteristic polynomial contains a loop and showing that this loop is just the generalized Brillouin zone itself, using some simple models first and then general one-band models. We demonstrate our conclusions on various non-Hermitian model examples with longer-range hopping. Our results indicate that real spectra are more common than one may have expected in non-Hermitian systems and are helpful for designing non-Hermitian models with real spectra.
Open systems feature a variety of phenomena that arise from non-Hermitian physics. Recent theoretical studies have offered much insights into these phenomena through the non-Bloch band theory, though many of the theory's key features are experimentally elusive. For instance, the correspondence between complex momenta and non-Hermitian bands, while central to non-Bloch band theory, has so far defied direct experimental observation. Here we experimentally study the non-Hermitian spectral deformation in complex-momentum space, by implementing a non-Hermitian lattice with long-range couplings in the synthetic orbital-angular-momentum (OAM) dimension of photons inside a degenerate cavity. Encoding the complex momenta in the phase and amplitude modulations of the OAM modes, and devising a complex-momentum-resolved projective detection, we reconstruct the spectral deformation in momentum space, where the eigenspectrum on the complex plane morphs through distinct geometries. This enables us to experimentally extract key information of the system under the non-Bloch band theory, including exceptional points in the complex-momentum space, the open-boundary spectra, and the generalized Brillouin zone. Our work demonstrates a versatile platform for exploring non-Hermitian physics and non-Bloch band theory, and opens the avenue for direct experimental investigation of non-Bloch features in the complex-momentum space.
The non-Hermitian skin effect (NHSE), the accumulation of eigen-wave functions at boundaries of open systems, underlies a variety of exotic properties that defy conventional wisdom. While the NHSE and its intriguing impact on band topology and dynamics have been observed in classical or photonic systems, their demonstration in a quantum gas system remains elusive. Here we report the experimental realization of a dissipative Aharonov-Bohm chain-non-Hermitian topological model with NHSE-in the momentum space of a two-component Bose-Einstein condensate. We identify signatures of the NHSE in the condensate dynamics, and perform Bragg spectroscopy to resolve topological edge states against a background of localized bulk states. Our Letter sets the stage for further investigation on the interplay of many-body statistics and interactions with the NHSE, and is a significant step forward in the quantum control and simulation of non-Hermitian physics.