Light-matter interactions that are nonlinear with respect to the photon number reveal the quantum nature of coherent states. We characterize how coherent states depart from Gaussian by the emergence of negative values in their Wigner function during the evolution while maintaining their characteristic Poissonian photon statistics. Such states have nonminimum uncertainty yet present a metrological advantage that can reach the Heisenberg limit. Non-Gaussianity of light arises as a general property of nonlinear interactions, which only requires a polarizable media, resonant or dispersive. Our results highlight how useful quantum features can be extracted from the seemingly most classical states of light, a relevant phenomenon for quantum optics applications.
Light-matter interactions that are nonlinear with respect to the photon number reveal the quantum nature of coherent states. We characterize how coherent states depart from Gaussian by the emergence of negative values in their Wigner function during the evolution while maintaining their characteristic Poissonian photon statistics. Such states have nonminimum uncertainty yet present a metrological advantage that can reach the Heisenberg limit. Non-Gaussianity of light arises as a general property of nonlinear interactions, which only requires a polarizable media, resonant or dispersive. Our results highlight how useful quantum features can be extracted from the seemingly most classical states of light, a relevant phenomenon for quantum optics applications.
Non-Gaussian quantum states of light are essential resources for quantum information processing and precision metrology. Among them, generalized coherent states (GCS), which naturally arise from the evolution of a coherent state with a nonlinear medium, exhibit useful quantum features such as Wigner negativity and metrological advantages [Phys. Rev. Res. 5, 013165 (2023)]. Because these states remain coherent to all orders, their nonclassical character cannot be revealed through standard intensity-intensity correlation measurements. Here, we demonstrate that the intensity-field correlation function alone provides a simple and experimentally accessible witness of nonclassicality. For GCSs, any deviation of this normalized correlation from unity signals nonclassical behavior. We derive analytical results for Kerr-generated states and extend the analysis to statistical mixtures of GCSs. The proposed approach enables real-time, low-complexity detection of quantum signatures in non-Gaussian states, offering a practical tool for experiments across a broad range of nonlinear regimes.
Non-Gaussian states of light are a critical resource for fault-tolerant quantum computing and enhanced metrology, but are typically faint and often obtained via post-selection. Here, we demonstrate the deterministic generation of a bright non-Gaussian state by introducing a Kerr nonlinearity to a macroscopic state of light called bright squeezed vacuum (BSV). To characterize the resulting state, we use a single-shot f-2f interferometer to sample its Husimi function. We observe a clear transformation from a 2D Gaussian distribution to an 'S'-shaped non-Gaussian profile, which is the direct statistical evidence of the intensity-dependent nonlinear phase. The negativity of the Wigner function, which is an intrinsic property of any pure non-Gaussian state, cannot be observed because BSV is a mixed state even under minute optical loss. However, we show that BSV can be considered as a mixture of pure squeezed coherent states, for some of which Kerr-induced Wigner-function negativity is quite tolerant to loss. This work bridges the gap between quantum optics and ultrafast nonlinear optics, opening a path to quantum applications that require high photon flux.
Quantum attributes of light have been related to non-classicality so far, i. e. to incompatibility with mixtures of coherent states. The progress in quantum optics indicates that this feature does not suffice to witness exotic behavior of light. Contrary, quantum non-Gaussianity is starting to appear as a promising and applicable property reflecting interesting states of light that are suitable for quantum protocols. We investigate a newly introduced hierarchy of criteria of quantum non-Gaussianity and predict this attribute can be observed on light emitted from many single photon emitters, even if the light undergoes realistic optical losses. It contrasts negativity of Wigner function, that is unreachable in experimental platforms with losses above fifty percent.
Quantum technologies are powered by platforms to generate complex non-classical states of matter or light to realize applications. We investigate the non-classical properties of high-harmonic generation in semiconductors, an emerging photonic platform. Measuring the click statistics of three double-digit orders, we evaluate witness operators to certify the non-classicality of the generated states. We show that higher-order harmonics driven by a coherent laser are squeezed and entangled. The properties of the emission are well retrieved with an entangled Gaussian state model, obtained by numerical state optimization to multiple observables. Additionally, we perform inter-order heralded measurements to engineer the quantum state of the emission. The heralded states have distinct properties, showing sub-Poissonian photon statistics. Further, we witness the generation of a quantum non-Gaussian state, a resource highly relevant for quantum information. With this, we establish high-harmonic generation as a platform for generating quantum optical resources.
Abstract Since radiation field states are very important in the interaction with the various atomic structures, in this article we introduce a new type of quantum states, which we call ‘Mth nonlinear coherent states’. We define these states based on acting of the number operator M times n ˆ M on a nonlinear coherent state. By analyzing the photon distribution function and its overlap with the nonlinear coherent states, it becomes clear that these states are very similar to the corresponding nonlinear coherent states. We also investigate the nonclassical features of such states for different values of M, and it is determined that the occurrence of sub-Poissonian photon statistics, normal squeezing, and amplitude squared squeezing are considerable nonclassical properties of the Mth nonlinear coherent states. Also, examining the Husimi function shows a local behavior for the introduced states. Furthermore, by calculating the Wigner function, we find out that in some points of the phase space, the value of this function is negative which could be considered as a nonclassical feature for these states.
This review covers recent theoretical and experimental efforts to extend the application of the continuous-variable quantum technology of light beyond "Gaussian" quantum states, such as coherent and squeezed states, into the domain of "non-Gaussian" states with negative Wigner functions. Starting with basic Gaussian nonclassicality associated with single- and two-mode vacuum states produced by means of parametric down-conversion and applying a set of standard tools, such as linear interferometry, coherent state injection, and conditional homodyne and photon number measurements, one can implement a large variety of optical states and processes that are relevant in fundamental quantum physics as well as quantum optical information processing. We present a systematic review of these methods, paying attention to both fundamental and practical aspects of their implementation, as well as a comprehensive overview of the results achieved therewith.