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arXiv:2201.03311 · Nature

Extended Bose–Hubbard model with dipolar excitons

Camille Lagoin, Utso Bhattacharya, Tobias Graß, Ravindra W. Chhajlany, Tymoteusz Salamon, Kirk Baldwin, Loren N. Pfeiffer, Maciej Lewenstein, Markus Holzmann, François Dubin

Published Sep 14, 2022• 52 citations
arXivHTMLPDF

Abstract

Abstract The Hubbard model constitutes one of the most celebrated theoretical frameworks of condensed-matter physics. It describes strongly correlated phases of interacting quantum particles confined in a lattice potential. For bosons, in the last two decades the Hubbard Hamiltonian has been deeply scrutinised in the regime of short-range on-site interactions. On the other hand, extensions to longer-range off-site couplings between neighbouring lattice sites have remained mostly elusive experimentally. Entering this regime constitutes a well identified research frontier where quantum matter phases can spontaneously break the lattice symmetry. Here we unveil one of such phases, precisely the long-sought-after checkerboard solid. It is accessed by confining semiconductors dipolar excitons in a two-dimensional square lattice. The exciton checkerboard is signalled by a strongly minimised compressibility at half-filling of the lattice sites, in quantitative agreement with theoretical expectations. Our observations thus highlight that dipolar excitons enable controlled implementations of extended Bose-Hubbard Hamiltonians.

DOI
10.1038/s41586-022-05123-z

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Abstract The Hubbard model constitutes one of the most celebrated theoretical frameworks of condensed-matter physics. It describes strongly correlated phases of interacting quantum particles confined in a lattice potential. For bosons, in the last two decades the Hubbard Hamiltonian has been deeply scrutinised in the regime of short-range on-site interactions. On the other hand, extensions to longer-range off-site couplings between neighbouring lattice sites have remained mostly elusive experimentally. Entering this regime constitutes a well identified research frontier where quantum matter phases can spontaneously break the lattice symmetry. Here we unveil one of such phases, precisely the long-sought-after checkerboard solid. It is accessed by confining semiconductors dipolar excitons in a two-dimensional square lattice. The exciton checkerboard is signalled by a strongly minimised compressibility at half-filling of the lattice sites, in quantitative agreement with theoretical expectations. Our observations thus highlight that dipolar excitons enable controlled implementations of extended Bose-Hubbard Hamiltonians.
In condensed-matter physics, electronic Mott insulators have triggered considerable research due to their intricate relation with high-temperature superconductors. However, unlike atomic systems for which Mott phases were recently shown for both bosonic and fermionic species, the fingerprint of a Mott phase implemented with bosons is yet to be found in the solid state. Here we unveil such signature by emulating the Bose-Hubbard hamiltonian with semiconductor excitons confined in a two-dimensional lattice. The exciton fluid is characterised by strong repulsive dipolar interactions. These mostly constrain the system to behave classically, but nevertheless allow for a very narrow parameter space where two Mott phases are formed, with either one or two excitons per lattice site. Our ability to program the lattice geometry explored by excitons then paves the way towards quantum simulations of long-sought many-body phases such as supersolids.
Enriching condensed-matter systems with quantum optical phenomena currently drives intense research efforts, particularly to introduce collective quantum correlations. Here we access this paradigm, by confining dipolar excitons in a nanoscopic lattice where long-range hopping, and nearest-neighbour dipolar repulsions, dress the Bose-Hubbard Hamiltonian. Long-range hopping is evidenced by the spontaneous buildup of many-body sub-radiance, signalled by an algebraic slowdown of excitons radiative dissipation. In addition, we observe a threshold increase of temporal coherence for dipolar quantum solids only. It suggests that excitons condense in a single sub-radiant state for Mott-like phases. These combine then spatial order and collectively extended coherence, in a single degree of freedom. Our study unveils that nanoscopic exciton arrays provide a unique platform to design new frontiers of strongly-correlated lattice models with long-range correlations.
In condensed-matter physics, long-range correlations introduce quantum states of matter that challenge intuition. For example, supersolids combine density order that manifests as symmetry-breaking spatial arrangement, and frictionless superfluid flow. However, supersolids have proven to only exist under very stringent conditions, with evidence limited to a few spontaneously fragmented superfluids observed in the weakly-interacting regime. Here, we demonstrate a framework to realize crystalline supersolids in the strong interaction regime, by confining dipolar bosons in a lattice with long-range hopping. We show that dipolar excitons realize this lattice model. At fractional lattice fillings of one quarter, one third and one half we observe mesoscopic quantum crystals across around 100 sites that spontaneously break the lattice translational symmetry. At the same time, coherent long-range hopping induces off-diagonal long-range order such that the exciton solids are superfluids. Our numerical methods quantitatively confirm that supersolidity builds up in the ground-state of the lattice Hamiltonian.
Confined indirect excitons in a two-dimensional magnetic lattice are promoted to simulate condensed matter systems. Excitonic particles are magnetically trapped so that a sufficient cooling mechanism can allow the trapped clouds of indirect excitons to experience the Bose-Einstein condensation phase transition. Thus, a long­ range spatial coherence can be resolved causing an inherited phase-locked across all of the coupled sites (single traps). Using an external magnetic bias field a mutual tunneling can adiabatically be exchanged between sites in which case the underline physics of Bose-Hubbard model can be explored such as Mott-insulator and Josephson Effect.
We consider a minimal model to describe the quantum phases of ultracold dipolar bosons in two-dimensional square optical lattices. The model is a variation of the extended Bose-Hubbard model and apt to study the quantum phases arising from the variation in the tilt angle $\ensuremath{\theta}$ of the dipolar bosons. At low tilt angles, ${0}^{\ensuremath{\circ}}\ensuremath{\leqslant}\ensuremath{\theta}\ensuremath{\lesssim}{25}^{\ensuremath{\circ}}$, the ground states of the system are phases with checkerboard order, which can be either checkerboard supersolids or checkerboard density waves. For high tilt angles, ${35}^{\ensuremath{\circ}}\ensuremath{\lesssim}\ensuremath{\theta}\ensuremath{\lesssim}{55}^{\ensuremath{\circ}}$, phases with striped order of the supersolid or density wave are preferred. In the intermediate domain, ${25}^{\ensuremath{\circ}}\ensuremath{\lesssim}\ensuremath{\theta}\ensuremath{\lesssim}{35}^{\ensuremath{\circ}}$, an emulsion or superfluid phase intervenes the transition between the checkerboard and the striped phases. The attractive interaction dominates at $\ensuremath{\theta}\ensuremath{\gtrsim}{55}^{\ensuremath{\circ}}$, which renders the system unstable, and there is a density collapse. For our studies we use Gutzwiller mean-field theory to obtain the quantum phases and the phase boundaries. In addition, we calculate the phase boundaries between an incompressible and a compressible phase of the system by considering second-order perturbation analysis of the mean-field theory. The analytical results, where applicable, are in excellent agreement with the numerical results. In our study, the incompressible phases have an average occupancy per site $\ensuremath{\rho}\ensuremath{\le}1$, but the compressible phases can have $\ensuremath{\rho}>1$.