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arXiv:2201.01317 · Physical review. B./Physical review. B

Subgap two-particle spectral weight in disordered s -wave superconductors: Insights from mode coupling approach

Prathyush Poduval, Abhisek Samanta, Prashant Kumar Gupta, Nandini Trivedi, Rajdeep Sensarma

Published Aug 30, 2022• 0 citations
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Abstract

We study the two-particle spectral functions and collective modes of weakly disordered superconductors using a disordered attractive Hubbard model on a square lattice. We show that the disorder-induced scattering between collective modes leads to a finite subgap spectral weight in the long-wavelength limit. In general, the spectral weight is distributed between the phase and the Higgs channels, but as we move towards half filling the Higgs contribution dominates. The inclusion of the density fluctuations lowers the frequency at which this mode occurs and results in the phase channel gaining a larger contribution to this subgap mode. Near half filling, the proximity of the system to the charge density wave instability leads to strong fluctuations of the effective disorder at the commensurate wave vector ($[\ensuremath{\pi},\ensuremath{\pi}]$). We develop an analytical mode coupling approach where the pure Goldstone mode in the long-wavelength limit couples to the collective mode at $[\ensuremath{\pi},\ensuremath{\pi}]$. This provides insight into the location and distribution of the two-particle spectral weights between the Higgs and the phase channels.

DOI
10.1103/physrevb.106.064512

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We study the two-particle spectral functions and collective modes of weakly disordered superconductors using a disordered attractive Hubbard model on a square lattice. We show that the disorder-induced scattering between collective modes leads to a finite subgap spectral weight in the long-wavelength limit. In general, the spectral weight is distributed between the phase and the Higgs channels, but as we move towards half filling the Higgs contribution dominates. The inclusion of the density fluctuations lowers the frequency at which this mode occurs and results in the phase channel gaining a larger contribution to this subgap mode. Near half filling, the proximity of the system to the charge density wave instability leads to strong fluctuations of the effective disorder at the commensurate wave vector ([\ensuremathπ,\ensuremathπ][\ensuremath{\pi},\ensuremath{\pi}][\ensuremathπ,\ensuremathπ]). We develop an analytical mode coupling approach where the pure Goldstone mode in the long-wavelength limit couples to the collective mode at [\ensuremathπ,\ensuremathπ][\ensuremath{\pi},\ensuremath{\pi}][\ensuremathπ,\ensuremathπ]. This provides insight into the location and distribution of the two-particle spectral weights between the Higgs and the phase channels.
The two-dimensional attractive Hubbard model is studied in the weak-to-intermediate-coupling regime by employing a nonperturbative approach. It is shown that this approach is in quantitative agreement with Monte Carlo calculations for both single-particle and two-particle quantities. Both the density of states and the single-particle spectral weight show a pseudogap at the Fermi energy below some characteristic temperature T∗,{T}^{*},T∗, also in good agreement with quantum Monte Carlo calculations. The pseudogap is caused by critical pairing fluctuations in the low-temperature renormalized classical regime $(\ensuremath{\Elzxh}\ensuremath{\omega}<{k}_{B}T)$ of the two-dimensional system. With increasing temperature the spectral weight fills in the pseudogap instead of closing it, and the pseudogap appears earlier in the density of states than in the spectral function. Small temperature changes around T∗{T}^{*}T∗ can modify the spectral weight over frequency scales much larger than temperature. Several qualitative results for the s-wave case should remain true for d-wave superconductors.
We discuss the density-density response functions and the collective excitation spectrum for the extended Hubbard model with on-site attraction and arbitrary electron density, in the superconducting ground state.For the short-range intersite interaction we find the sound wave-like modes with the velocity interpolating smoothly between the weak (v 2Zt, |UD <2Zt) and strong coupling (v > 2Zt) limits.The latter agrees with the results obtained from an effective pseudospin Hamiltonian valid in the strong coupling limit.In the weak coupling regime, we obtain that apart from a commensurate charge density wave instability, an increase in the intersite Coułomb repulsion can give rise to a charge density wave incommensurate with the lattice period, away from half-frlling.The ground state phase diagram for 2D square lattice, including singlet superconducting ground state, electronic droplet formation, and charge density waves is determined.It is also shown that the energy of collective excitations evolves smoothly from weak to strong coupling limit for a 2D lattice, in the case of a long-range Coulomb interaction.Finally, the mode coupling effects in the frequency behavior of the density-density response functions are analyzed.
The superfluid properties of attractive Hubbard model in dice lattice are investigated. It is found that three superfluid order parameters increase as the interaction increases. When the filling factor falls into the flat band, due to the infinite large density of states, the resultant superfluid order parameters are proportional to interaction strength, which is in striking contrast with the exponentially small counterparts in usual superfluid (or superconductor). When the interaction is weak, and the filling factor is near the bottom of the lowest band (or the top of highest band), the superfluid density is determined by the effective mass of the lowest (or highest) single-particle band. When the interaction is strong and filling factor is small, the superfluid density is inversely proportional to interaction strength, which is related to effective mass of tightly bound pairs. In the strong interaction limit and finite filling, the asymptotic behaviors of superfluid density can be captured by a parabolic function of filling factor. Furthermore, when the filling is in flat band, the superfluid density shows a logarithmic singularity as the interaction approaches zero. In addition, there exist three undamped collective modes for strong interactions. The lowest excitation is gapless phonon, which is characterized by the total density oscillations. The two others are gapped Leggett modes, which correspond relative density fluctuations between sublattices. The collective modes are also reflected in the two-particle spectral functions by sharp peaks. Furthermore, it is found that the two-particle spectral functions satisfy an exact sum-rule, which is directly related to the filling factor (or density of particle). The sum-rule of the spectral functions may be useful to distinguish between the hole-doped and particle-doped superfluid (superconductor) in experiments.
The auxiliary boson method and 1/N expansion are applied to the solution of the Hubbard model in the U = ∞\infty∞ limit, in functional integral form. The zero order term in the expansion gives the mean-field result of non-interacting enhanced mass quasiparticles, and the next order gives Gaussian fluctuations around the mean-field value, representing effective interactions between the quasiparticles. From the density-density correlation function, the collective mode indicates a very different behavior away from and close to half filling. The superconducting instability is examined to 1/$N\sp2$ order from the dominant double collective mode exchange. For a parabolic band, there is a p-wave triplet instability. But for a 2D square lattice, there is no superconducting pairing to this order. The effects of disorder on this system are also investigated. For moderate filling, the specific heat and scattering rate have the same results as predicted in the weakly interacting theories. Close to half-filling, the specific heat and scattering rate show a much sharper temperature and energy dependence.
By use of a diagrammatic method we determine the density-density response functions in the random-phase approximation (RPA) and the collective-excitation spectrum for the extended Hubbard model with on-site attraction and arbitrary electron density, in the superconducting ground state. The energy of the collective modes, given by the poles of these response functions, is found to be a linear function of the wave vector (for small k and short-range intersite interaction) with the velocity interpolating smoothly between the weak- (\ensuremath{\propto}2zt, \ensuremath{\Vert}U\ensuremath{\Vert}\ensuremath{\ll}2zt) and strong-coupling (\ensuremath{\propto}zt2{\mathit{zt}}^{2}zt2/\ensuremath{\Vert}U\ensuremath{\Vert}, \ensuremath{\Vert}U\ensuremath{\Vert}\ensuremath{\gg}2zt) limits. The latter agrees with the results obtained from an effective pseudospin Hamiltonian valid in the strong-coupling limit. The numerical analysis for a two-dimensional (2D) square lattice shows the occurrence of a rotonlike minima near the zone boundary. In the weak-coupling regime we find that apart from a commensurate charge-density-wave (CDW) instability, an increase in the intersite Coulomb repulsion can give rise to a CDW incommensurate with the lattice period, away from half-filling. The resulting phase diagram for the 2D square lattice, including a singlet superconducting ground state, electronic-droplet formation, and CDW's, is determined. Finally, the effects of a long-range Coulomb interaction are analyzed briefly and it is shown that the energy of collective excitations evolves smoothly from the weak- to the strong-coupling limit for a 2D lattice.
Understanding competing instabilities in systems with correlated fermions remains one of the holy grails of modern condensed matter physics. Among the fermionic lattice models used to this effect, the extended Hubbard model occupies a prime place due to the potential relevance of its repulsive and attractive versions for both electronic materials and artificial systems. Using the recently introduced multichannel fluctuating field approach, we address the interplay of fluctuations in the charge density wave, sss-wave superconducting, and phase separation channels in the attractive extended Hubbard model. Despite the fact that this model has been intensively studied for decades, our approach allows us to identify a phase that has not been analyzed before and which is characterized by the coexistence of collective sss-wave superconducting and phase separation fluctuations. Our findings resonate with previous observations of interplaying phase separation and superconducting phases in electronic systems, most importantly in high-temperature superconductors.