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arXiv:2112.14082 · Physical Review A

Coherent control of a local phonon in trapped ions using dynamical decoupling

Ryutaro Ohira, Shota Kume, Kenji Toyoda

Published Oct 4, 2022• 4 citations
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Abstract

In this article, we present a dynamical decoupling (DD) technique to coherently control the dynamics of a single local phonon in trapped ions. A $2\ensuremath{\pi}$ rotation at a motional sideband transition flips the sign of the relevant local-phonon state, resulting in cancellation of the phonon dynamics. In this work, we implement DD using resonant blue-sideband pulses to control the hopping of a single local phonon between two ${^{40}\mathrm{Ca}}^{+}$ ions in a linear Paul trap. Our proposed DD technique can be used to engineer coupling between local-phonon modes.

DOI
10.1103/physreva.106.042603

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quant-pharXiv:2603.01585•Mar 3, 2026
In this article, we present a dynamical decoupling (DD) technique to coherently control the dynamics of a single local phonon in trapped ions. A 2\ensuremathπ2\ensuremath{\pi}2\ensuremathπ rotation at a motional sideband transition flips the sign of the relevant local-phonon state, resulting in cancellation of the phonon dynamics. In this work, we implement DD using resonant blue-sideband pulses to control the hopping of a single local phonon between two 40Ca+{^{40}\mathrm{Ca}}^{+}40Ca+ ions in a linear Paul trap. Our proposed DD technique can be used to engineer coupling between local-phonon modes.
When molecular ions are trapped together with atomic ions in a Paul trap, their dipole moment couples the molecular rotation to the joint vibrational motion of the particles in the trap. To leverage this coupling for quantum control, a rotational transition in the molecule should be resonant with one of the ion crystal vibrational modes. Focusing on the example of singly charged thorium fluoride molecular ions, cotrapped with two ytterbium ions, we determine the conditions for resonant dipole-phonon coupling, fully accounting for the molecular hyperfine structure. We identify several choices for resonant coupling and discuss its detection using sideband-resolved laser spectroscopy and measurements of decoherence.
This thesis extends the recently reported ground state sideband cooling of the axial motion of a single ion to a broader frequency range of the axial motion, the radial motion and ion crystals. Once cold, coherent control of these different configurations is demonstrated. The experimental work in this thesis uses 40Ca+ ions that can be coherently addressed on a narrow linewidth optical transition at 729 nm. The technique of axialization that resonantly couples the two radial modes of motion is used to enhance laser Doppler cooling leading to mean phonon occupation numbers in the low hundreds for both modes. The sideband cooling technique is then used to simultaneously cool both the motional modes to within one phonon of the ground state for the first time evers. Sideband cooling is then also employed to cool the axial modes of many ion Coulomb crystals in two different configurations. For two ions in a 1D chain, motional occupation numbers of nbar_COM=0.30(4) and nbar_B=0.07(3) are achieved. For two ions in a planar 2D configuration the result for the two modes are nbar_T=nbar_COM<0.1. This technique is scaled up to demonstrate ground state occupation of up to 10 ions in the planar configuration. The axial mode of motion of a single motion is used to characterise the coherent addressing capabilities in our system through optical and motional Ramsey spectroscopy. We observe optical coherence times of 1.78(4) ms and motional coherence times of 590(12) ms. Dynamical decoupling techniques are shown to extend these coherence times. Furthermore, basic decoherence models are validated in high-lying non-thermal motional states that are prepared by a sideband heating technique. Progress towards entangling gates is demonstrated using a bichromatic laser beam to prepare non-classical states of motion.
We demonstrate the implementation of a spin qubit with a single 40 Ca + ion in a micro ion trap. The qubit is encoded in the Zeeman ground state levels m J = +1/2 and m J = −1/2 of the S 1/2 state of the ion. We show sideband cooling close to the vibrational ground state and demonstrate the initialization and readout of the qubit levels with 99.5% efficiency. We employ a Raman transition close to the S 1/2 –P 1/2 resonance for coherent manipulation of the qubit. We observe single qubit rotations with 96% fidelity and gate times below 5 µs. Rabi oscillations on the blue motional sideband are used to extract the phonon number distribution. The dynamics of this distribution is analysed to deduce the trap-induced heating rate of 0.3(1) phonons ms −1 .
We present a theoretical model for realizing squeezed lasing in a trapped-ion system without relying on engineered baths or tailored dissipative reservoirs. Our approach leverages the intrinsic ion-phonon interactions, where two trapped ions, each interacting with a shared vibrational mode, are driven on both red- and blue-sideband transitions. This enables the creation of a squeezed state of motion through the dynamic coupling between the ions' internal states and the phonon mode. Unlike traditional methods that require bath engineering, our model demonstrates that squeezed lasing can be achieved through a direct manipulation of ion-phonon interactions, with no external reservoirs required. We explore the steady-state behavior of the system, analyzing the onset of lasing, gain-loss balance, and the role of the squeezing parameter in shaping the phonon field's statistical properties. Furthermore, we show how external coherent drives can stabilize phase coherence and achieve controlled quadrature squeezing, offering a simple yet effective method for achieving squeezed lasing in quantum mechanical systems. Our findings provide new insights into the realization of squeezed states in phonon-based systems, with potential applications in quantum metrology and information processing.
From subatomic particles to macromolecules, quantum mechanics has a deep impact in understanding the interactions and nature of such constituents of matter. The paradoxical observations of entanglement in quantum systems is used in quantum computations. Ion traps are among the leading platforms which provide clean and highly controllable quantum systems. This thesis presents the study of quantum coherence aiming to devise and test coherent control with trapped ions in a Penning trap. Our apparatus contains one or more calcium ions that are confined in space using DC electric and magnetic fields. Doppler cooling and resolved sideband cooling of trapped ions are carried out to perform high fidelity quantum control. The ions are prepared in their motional ground state via a multi-stage resolved sideband cooling technique. The cooling methods are first verified through simulations. The axial mean phonon numbers for a single ion are measured to be 0.03 ± 0.01 and 0.012 ± 0.009 at 187 kHz and 420 kHz axial frequencies, respectively. The heating rate is measured to be 2.5 ± 0.5 phonons/s, which is consistent with the previous measurements in our system. Similarly, the radial motional modes of a single ion are cooled to 〈n_+ 〉<0.4 and 〈n_- 〉<0.6 from mean phonon numbers corresponding to each mode of around 100. Preliminary studies are carried out of the axial motional modes of a 1D chain and 2D planar crystals, extending sideband cooling to small ICC's in a Penning trap. Coherent control is examined in our system and the optical coherence time and motional coherence time are estimated to be approximately 1 ms and 0.5 s, respectively. Furthermore, a single ion is prepared outside the Lamb-Dicke regime via a sideband heating technique and coherent studies are performed in such a regime via a laser beam.
The quantum phonon laser state is a vibrational state generated by phonon coherent amplification based on quantum mechanics. Its core is coherent excitation and manipulation of phonon quantum states by controlling phonon dynamics. This technology breaks classical limits of traditional phonon lasers, offering new methods for quantum information. Previous research on quantum phonon lasers focused on quantum van der Pol oscillators. As typical nonlinear quantum systems, they show significant value in trapped-ion systems. These breakthroughs extend nonlinear dynamics into the quantum domain and provide platforms for exploring quantum nonlinear phenomena. Although realized in two-ion systems, practical applications remain challenging. This paper explores how a single trapped ion generates quantum phonon laser states using a three-level model. By solving the quantum master equation numerically, steady-state characteristics are analyzed, focusing on quantum statistics including the Wigner function and second-order correlation function. An experimental scheme is proposed based on a single trapped 40Ca+ ion, using bichromatic blue-sideband and red-sideband lasers to generate quantum phonon laser states. By introducing the characteristic function of motional states, precise quantum state tomography is achieved. Additionally, a two-level model discusses the phonon laser threshold effect. However, the three-level model shows significantly different thresholds and more accurately describes the quantum phonon laser's physical mechanisms.