Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2112.11608 · Physical Review A

Universal model of strong coupling at the nonlinear resonance in open cavity-QED systems

Mikhail D. Tokman, Maria Erukhimova, Qianfan Chen, Alexey A. Belyanin

Published May 10, 2022• 3 citations
arXivHTMLPDF

Abstract

Many molecular, quantum-dot, and optomechanical nanocavity-QED systems demonstrate strong nonlinear interactions between electrons, photons, and phonon (vibrational) modes. We show that such systems can be described by a universal model in the vicinity of the nonlinear resonance involving all three degrees of freedom. We solve the nonperturbative quantum dynamics in the strong-coupling regime of the nonlinear resonance, taking into account quantization, dissipation, and fluctuations of all fields. We find analytic solutions for quantum states in the rotating-wave approximation which demonstrate tripartite quantum entanglement once the strong-coupling regime is reached. We show how the strong coupling at the nonlinear resonance modifies photon emission and vibrational spectra, and how the observed spectra can be used to extract information about relaxation rates and the nonlinear coupling strength in specific systems.

DOI
10.1103/physreva.105.053707

Related papers

Generation and dynamics of entangled fermion–photon–phonon states in nanocavities

Mikhail D. Tokman, Maria Erukhimova, University Wang +2 more

We develop the analytic theory describing the formation and evolution of entangled quantum states for a fermionic quantum emitter coupled simultaneously to a quantized electromagnetic field in a nanocavity and quantized phonon or mechanical vibrational modes. The theory is applicable to a broad range of cavity quantum optomechanics problems and emerging research on plasmonic nanocavities coupled to single molecules and other quantum emitters. The optimal conditions for a tripartite entanglement are realized near the parametric resonances in a coupled system. The model includes dissipation and decoherence effects due to coupling of the fermion, photon, and phonon subsystems to their dissipative reservoirs within the stochastic evolution approach, which is derived from the Heisenberg-Langevin formalism. Our theory provides analytic expressions for the time evolution of the quantum state and observables and the emission spectra. The limit of a classical acoustic pumping and the interplay between parametric and standard one-photon resonances are analyzed.

De Gruyter eBooks•May 25, 2021•1 citation

Impact of the phonon environment on the nonlinear quantum-dot cavity QED. II. Analytical approach

L. S. Sirkina, Egor A. Muljarov

The effect of phonons on a nonlinear optical response of a quantum dot-cavity system in quantum strong coupling regime can be accounted for by a fully analytical treatment, provided that the exciton-phonon dynamics is much faster than the exciton-cavity dynamics. Modern experiments involving semiconductor quantum dots embedded in optical microcavities typically meet this criterion. We find that, for a relatively small exciton-cavity coupling, the effect of phonons is concentrated mainly in the polaron shift of the exciton frequency and reduction of exciton-cavity coupling by the Huang-Rhys factor. We have generalized this result to an arbitrary optical nonlinearity and demonstrated a good agreement with the exact solution in a wide range of temperatures. This generalization provides access to higher rungs of the Jaynes-Cummings ladder, where exact numerical approaches are impractical or even impossible. At larger coupling strengths and low temperatures, our approximation is also in good agreement with the exact solution, which makes it a very useful tool for addressing the phonon contribution to the coherent dynamics of a nonlinear optical system. We demonstrate our results for third-order optical polarization with varying observation time and delay time between excitation pulses in the form of two-dimensional spectra. These spectra provide useful information about the coherent coupling between the exciton and the cavity modes. The presented analytical approach is also compared with another useful approximation, having the form of a matrix product, which is a special case of the asymptotically exact solution in the limit of a short phonon memory time.

arXiv:2306.16579•Jun 28, 2023•0 citations

Exploring unresolved sideband, optomechanical strong coupling using a single atom coupled to a cavity

Lukas Neumeier, Darrick E Chang

A major trend within the field of cavity QED is to boost the interaction strength between the cavity field and the atomic internal degrees of freedom of the trapped atom by decreasing the mode volume of the cavity. In such systems, it is natural to achieve strong atom-cavity coupling, where the coherent interaction strength exceeds the cavity linewidth, while the linewidth exceeds the atomic trap frequency. While most work focuses on coupling of photons to the internal degrees of freedom, additional rich dynamics can occur by considering the atomic motional degree of freedom as well. In particular, we show that such a system is a natural candidate to explore an interesting regime of quantum optomechanics, where the zero-point atomic motion yields a cavity frequency shift larger than its linewidth (so-called single-photon optomechanical strong coupling), but simultaneously where the motional frequency cannot be resolved by the cavity. We show that this regime can result in a number of remarkable phenomena, such as strong entanglement between the atomic wave function and the scattering properties of single incident photons, or an anomalous mechanism where the atomic motion can significantly heat up due to single-photon scattering, even if the atom is trapped tightly within the Lamb-Dicke limit.

arXiv:1804.02024•New Journal of Physics•Jul 19, 2018•14 citations

Generation and dynamics of entangled fermion-photon-phonon states in nanocavities

Mikhail D. Tokman, Maria Erukhimova, Yongrui Wang +2 more

We develop the analytic theory describing the formation and evolution of entangled quantum states for a fermionic quantum emitter coupled to a quantized electromagnetic field in a nanocavity and quantized phonon or mechanical vibrational modes. The theory is applicable to a broad range of cavity quantum optomechanics problems and emerging research on plasmonic nanocavities coupled to single molecules and other quantum emitters. The optimal conditions for a tri-state entanglement are realized near the parametric resonances in a coupled system. The model includes decoherence effects due to coupling of the fermion, photon, and phonon subsystems to their dissipative reservoirs within the stochastic evolution approach, which is derived from the Heisenberg-Langevin formalism. Our theory provides analytic expressions for the time evolution of the quantum state and observables, and the emission spectra. The limit of a classical acoustic pumping and the interplay between parametric and standard one-photon resonances are analyzed.

arXiv:2007.02159•Jul 4, 2020•0 citations

Nonlinearities in the strong coupling regime of the Tavis-Cummings model: from multi-photon resonances to bistability

András Dombi, András Vukics, P. Domokos

In the strong coupling regime of cavity QED where the characteristic damping rates are orders of magnitude below the coherent coupling, resolved multi-photon resonances can be observed for strong enough driving strength. In a certain frequency range, the external coherent drive field hits multi-photon resonances which correspond to very high order transitions that cannot be excited at the given power of the driving field. We found that in this range the cavity field evolves into a robust semiclassical solution which is the mixture of the vacuum and an excited quasi-classical state. The system is reminiscent of optical bistability, however, here a single atom produces a telegraph signal for the outgoing intensity by switching between two states with large photon number difference. We calculate this behavior also for the Tavis-Cummings model representing three qubits in an existing circuit QED experimental setting.

•Apr 30, 2014•0 citations

Impact of the phonon environment on the nonlinear quantum-dot–cavity QED: Path-integral approach

L. S. Sirkina, Egor A. Muljarov

We demonstrate a strong influence of the phonon environment on the coherent dynamics of the quantum dot (QD)-cavity system in the quantum strong coupling regime. This regime is implemented in the nonlinear QD-cavity QED and can be reliably measured by heterodyne spectral interferometry. We present a semianalytic asymptotically exact path integral-based approach to the nonlinear optical response of this system, which includes two key ingredients: Trotter's decomposition and linked-cluster expansion. Applied to the four-wave-mixing optical polarization, this approach provides access to different excitation and measurement channels, as well as to higher-order optical nonlinearities and quantum correlators. Furthermore, it allows us to extract useful analytic approximations and analyze the nonlinear optical response in terms of quantum transitions between phonon-dressed states of the anharmonic Jaynes-Cummings (JC) ladder. Being well described by these approximations at low temperatures and small exciton-cavity coupling, the exact solution deviates from them for stronger couplings and higher temperatures, demonstrating remarkable non-Markovian effects, spectral asymmetry, and strong phonon renormalization of the JC ladder.

arXiv:2306.17722•Physical review. B./Physical review. B•Sep 28, 2023•5 citations
Many molecular, quantum-dot, and optomechanical nanocavity-QED systems demonstrate strong nonlinear interactions between electrons, photons, and phonon (vibrational) modes. We show that such systems can be described by a universal model in the vicinity of the nonlinear resonance involving all three degrees of freedom. We solve the nonperturbative quantum dynamics in the strong-coupling regime of the nonlinear resonance, taking into account quantization, dissipation, and fluctuations of all fields. We find analytic solutions for quantum states in the rotating-wave approximation which demonstrate tripartite quantum entanglement once the strong-coupling regime is reached. We show how the strong coupling at the nonlinear resonance modifies photon emission and vibrational spectra, and how the observed spectra can be used to extract information about relaxation rates and the nonlinear coupling strength in specific systems.
We develop the analytic theory describing the formation and evolution of entangled quantum states for a fermionic quantum emitter coupled simultaneously to a quantized electromagnetic field in a nanocavity and quantized phonon or mechanical vibrational modes. The theory is applicable to a broad range of cavity quantum optomechanics problems and emerging research on plasmonic nanocavities coupled to single molecules and other quantum emitters. The optimal conditions for a tripartite entanglement are realized near the parametric resonances in a coupled system. The model includes dissipation and decoherence effects due to coupling of the fermion, photon, and phonon subsystems to their dissipative reservoirs within the stochastic evolution approach, which is derived from the Heisenberg-Langevin formalism. Our theory provides analytic expressions for the time evolution of the quantum state and observables and the emission spectra. The limit of a classical acoustic pumping and the interplay between parametric and standard one-photon resonances are analyzed.
The effect of phonons on a nonlinear optical response of a quantum dot-cavity system in quantum strong coupling regime can be accounted for by a fully analytical treatment, provided that the exciton-phonon dynamics is much faster than the exciton-cavity dynamics. Modern experiments involving semiconductor quantum dots embedded in optical microcavities typically meet this criterion. We find that, for a relatively small exciton-cavity coupling, the effect of phonons is concentrated mainly in the polaron shift of the exciton frequency and reduction of exciton-cavity coupling by the Huang-Rhys factor. We have generalized this result to an arbitrary optical nonlinearity and demonstrated a good agreement with the exact solution in a wide range of temperatures. This generalization provides access to higher rungs of the Jaynes-Cummings ladder, where exact numerical approaches are impractical or even impossible. At larger coupling strengths and low temperatures, our approximation is also in good agreement with the exact solution, which makes it a very useful tool for addressing the phonon contribution to the coherent dynamics of a nonlinear optical system. We demonstrate our results for third-order optical polarization with varying observation time and delay time between excitation pulses in the form of two-dimensional spectra. These spectra provide useful information about the coherent coupling between the exciton and the cavity modes. The presented analytical approach is also compared with another useful approximation, having the form of a matrix product, which is a special case of the asymptotically exact solution in the limit of a short phonon memory time.
A major trend within the field of cavity QED is to boost the interaction strength between the cavity field and the atomic internal degrees of freedom of the trapped atom by decreasing the mode volume of the cavity. In such systems, it is natural to achieve strong atom-cavity coupling, where the coherent interaction strength exceeds the cavity linewidth, while the linewidth exceeds the atomic trap frequency. While most work focuses on coupling of photons to the internal degrees of freedom, additional rich dynamics can occur by considering the atomic motional degree of freedom as well. In particular, we show that such a system is a natural candidate to explore an interesting regime of quantum optomechanics, where the zero-point atomic motion yields a cavity frequency shift larger than its linewidth (so-called single-photon optomechanical strong coupling), but simultaneously where the motional frequency cannot be resolved by the cavity. We show that this regime can result in a number of remarkable phenomena, such as strong entanglement between the atomic wave function and the scattering properties of single incident photons, or an anomalous mechanism where the atomic motion can significantly heat up due to single-photon scattering, even if the atom is trapped tightly within the Lamb-Dicke limit.
We develop the analytic theory describing the formation and evolution of entangled quantum states for a fermionic quantum emitter coupled to a quantized electromagnetic field in a nanocavity and quantized phonon or mechanical vibrational modes. The theory is applicable to a broad range of cavity quantum optomechanics problems and emerging research on plasmonic nanocavities coupled to single molecules and other quantum emitters. The optimal conditions for a tri-state entanglement are realized near the parametric resonances in a coupled system. The model includes decoherence effects due to coupling of the fermion, photon, and phonon subsystems to their dissipative reservoirs within the stochastic evolution approach, which is derived from the Heisenberg-Langevin formalism. Our theory provides analytic expressions for the time evolution of the quantum state and observables, and the emission spectra. The limit of a classical acoustic pumping and the interplay between parametric and standard one-photon resonances are analyzed.
In the strong coupling regime of cavity QED where the characteristic damping rates are orders of magnitude below the coherent coupling, resolved multi-photon resonances can be observed for strong enough driving strength. In a certain frequency range, the external coherent drive field hits multi-photon resonances which correspond to very high order transitions that cannot be excited at the given power of the driving field. We found that in this range the cavity field evolves into a robust semiclassical solution which is the mixture of the vacuum and an excited quasi-classical state. The system is reminiscent of optical bistability, however, here a single atom produces a telegraph signal for the outgoing intensity by switching between two states with large photon number difference. We calculate this behavior also for the Tavis-Cummings model representing three qubits in an existing circuit QED experimental setting.
We demonstrate a strong influence of the phonon environment on the coherent dynamics of the quantum dot (QD)-cavity system in the quantum strong coupling regime. This regime is implemented in the nonlinear QD-cavity QED and can be reliably measured by heterodyne spectral interferometry. We present a semianalytic asymptotically exact path integral-based approach to the nonlinear optical response of this system, which includes two key ingredients: Trotter's decomposition and linked-cluster expansion. Applied to the four-wave-mixing optical polarization, this approach provides access to different excitation and measurement channels, as well as to higher-order optical nonlinearities and quantum correlators. Furthermore, it allows us to extract useful analytic approximations and analyze the nonlinear optical response in terms of quantum transitions between phonon-dressed states of the anharmonic Jaynes-Cummings (JC) ladder. Being well described by these approximations at low temperatures and small exciton-cavity coupling, the exact solution deviates from them for stronger couplings and higher temperatures, demonstrating remarkable non-Markovian effects, spectral asymmetry, and strong phonon renormalization of the JC ladder.