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arXiv:2112.10635 · Optics Letters

From superradiance to subradiance: exploring the many-body Dicke ladder

Antoine Glicenstein, Giovanni Ferioli, Antoine Browaeys, Igor Ferrier-Barbut

Published Feb 17, 2022• 29 citations
arXivHTMLPDF

Abstract

We report a time-resolved study of collective emission in dense ensembles of two-level atoms. We compare, on the same sample, the buildup of superradiance and subradiance from the ensemble when driven by a strong laser. This allows us to measure the dynamics of the population of superradiant and subradiant states as a function of time. In particular, we demonstrate the buildup in time of subradiant states through superradiant dynamics. This illustrates the dynamics of the many-body density matrix of superradiant ensembles of two-level atoms when departing from the ideal conditions of Dicke superradiance, in which symmetry forbids the population of subradiant states.

DOI
10.1364/ol.451903

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We report a time-resolved study of collective emission in dense ensembles of two-level atoms. We compare, on the same sample, the buildup of superradiance and subradiance from the ensemble when driven by a strong laser. This allows us to measure the dynamics of the population of superradiant and subradiant states as a function of time. In particular, we demonstrate the buildup in time of subradiant states through superradiant dynamics. This illustrates the dynamics of the many-body density matrix of superradiant ensembles of two-level atoms when departing from the ideal conditions of Dicke superradiance, in which symmetry forbids the population of subradiant states.
The collective spontaneous emission of many atoms is significantly different from that of a single atom, depending on the geometry and the phase correlation of atomic ensembles. However, experimental observation of arbitrary superradiant and subradiant states of atoms remains challenging due to the difficulties in both preparation and detection of those states. Here we report the time-resolved observation of superradiance from a timed Dicke state in a momentum-space superradiance lattice of Bose-Einstein condensates, which enables an in situ measurement of the coherent lattice dynamics involving both superradiant and subradiant states. The long-lasting oscillation in the superradiant emission is contributed by population transport from the subradiant states in the superradiance lattice. This work paves the way to prepare and observe subradiant states, which has promising applications in quantum information processing.
We report the experimental observation of a superradiant emission emanating from an elongated dense ensemble of laser cooled two-level atoms, with a radial extent smaller than the transition wavelength. In the presence of a strong driving laser, we observe that the system is superradiant along its symmmetry axis. This occurs even though the driving laser is orthogonal to the superradiance direction. This superradiance modifies the spontaneous emission, and, resultantly, the Rabi oscillations. We also investigate Dicke superradiance in the emission of an almost fully inverted system as a function of the atom number. The experimental results are in qualitative agreement with ab-initio, beyond-mean-field calculations.
The collective behavior of ensembles of atoms has been studied in-depth since the seminal paper of Dicke [R. H. Dicke, Phys. Rev. 93, 99 (1954)], where he demonstrated that a group of emitters in collective states is able to radiate with increased intensity and modified decay rates in particular directions, a phenomenon which he called superradiance. Here, we show that the fundamental setup of two atoms coupled to a single-mode cavity can be distinctly exceeding the free-space superradiant behavior, a phenomenon which we call hyperradiance. The effect is accompanied by strong quantum fluctuations and surprisingly arises for atoms radiating out-of-phase, an alleged non-ideal condition, where one expects subradiance. We are able to explain the onset of hyperradiance in a transparent way by a photon cascade taking place among manifolds of Dicke states with different photon numbers under particular out-of-phase coupling conditions. The theoretical results can be realized with current technology and thus should stimulate future experiments.
Collectivity in ensembles of atoms gives rise to effects like super- and subradiance. While superradiance is well studied and experimentally accessible, subradiance remains elusive since it is difficult to track experimentally as well as theoretically. Here we present a new type of phase transition in the resonantly driven, open Dicke model that leads to a deterministic generation of subradiant states. At the transition the system switches from a predominantly superradiant to a predominantly subradiant state. Counterintuitively, the cavity decay is the crucial parameter for subradiant state generation and not the individualizing process of spontaneous decay. The observed effect is thus a cavity assisted generation of subradiant quantum coherences. Clear experimental signatures for the effect are presented and entanglement properties are discussed. Letting the system relax into the ground state generates a cascade of dark Dicke states, with dark state populations up to unity. Furthermore we introduce a collectivity measure that allows to quantify collective behaviour.
Recent works have shown that collective single photon spontaneous emission from an ensemble of N resonant two-level atoms is a rich field of study. Superradiance describes emission from a completely symmetric state of N atoms, with a single excited atom prepared with a given phase, for instance imprinted by an external laser. Instead, subradiance is associated with the emission from the remaining N−1 asymmetric states, with a collective decay rate less than the single-atom value. Here, we discuss the properties of the orthonormal basis of symmetric and asymmetric states and the entanglement properties of superradiant and subradiant states.
Recent advances in generating well controlled dense arrangements of individual atoms in free space have generated interest in understanding how the extended nature of these systems influences superradiance phenomena. Here, we provide an in-depth analysis on how space-dependent light shifts and decay rates induced by dipole-dipole interactions modify the steady-state properties of coherently driven arrays of quantum emitters. We characterize the steady-state phase diagram, with particular focus on the radiative properties in the steady state. Interestingly, we find that diverging from the well-established Dicke paradigm of equal all-to-all interactions significantly modifies the emission properties. In particular, the prominent quadratic scaling of the radiated light intensity with particle number in the steady state—a hallmark of steady-state Dicke superradiance—is entirely suppressed, resulting in only linear scaling with particle number. We show that this breakdown of steady-state superradiance occurs due to the emergence of additional dissipation channels that populate not only superradiant states but also subradiant ones. The additional contribution of subradiant dark states in the dynamics leads to a divergence in the time scales needed to achieve steady states. Building on this, we further show that measurements taken at finite times for extended atom ensembles reveal properties closely mirroring the idealized Dicke scenario. Published by the American Physical Society 2024