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arXiv:2112.09905 · Optics

New Evidence for a Nonclassical Behavior of Laser Multimode Light

Michael V. Lebedev, A. A. Demenev, A.L. Parakhonsky, O. V. Misochko

Published Jan 29, 2022• 1 citation
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Abstract

In this work, we present new experimental evidence of a nonclassical behavior of a multimode Fabry–Perot (FP) semiconductor laser by the measurements of intensity correlation functions. Due to the multimode quantum state occurrence, instead of expected correlations between the intensities of the laser modes (a semiclassical theory), their anticorrelations were revealed.

DOI
10.3390/opt3010006

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In this work, we present new experimental evidence of a nonclassical behavior of a multimode Fabry–Perot (FP) semiconductor laser by the measurements of intensity correlation functions. Due to the multimode quantum state occurrence, instead of expected correlations between the intensities of the laser modes (a semiclassical theory), their anticorrelations were revealed.
In this work, temporal correlations of radiation intensities of a multimode Fabry-Perot (FP) semiconductor laser are studied. Second- and third-order intensity correlation functions are measured both for the multimode FP laser and a pulsed Ti: Sapphire (TiSp) laser. Triple correlators of the latter demonstrate an ordinary product of double correlators (the classic case). The behavior of the multimode laser is more complex and can indicate the quantum nature of optical field correlations. We follow a specific phenomenological formula for calculation of the triple temporal correlator.
High-harmonic generation is a light up-conversion process occurring in a strong laser field, leading to coherent bursts of extreme ultrashort broadband radiation [Lewenstein , Phys. Rev. A , 2117 (1994)]. As a new perspective, we propose that ultrafast strong-field electronic or photonic processes such as high-harmonic generation can potentially generate nonclassical states of light well before the decoherence of the system occurs [Gorlach , Nat. Commun. , 4598 (2020); Stammer ., Phys. Rev. Lett. , 123603 (2022)]. This could address fundamental challenges in quantum technology such as scalability, decoherence, or the generation of massively entangled states [Lewenstein , Luca Argenti Michael Chini, 27 (2024)]. Here, we report experimental evidence of the nonclassical nature of the harmonic emission in several semiconductors excited by a femtosecond infrared laser. By investigating single- and double-beam intensity cross-correlation [Loudon, Rep. Prog. Phys. , 913 (1980)], we measure characteristic nonclassical features in the single-photon statistics. We observe two-mode squeezing in the generated harmonic radiation, which depends on the laser intensity that governs the transition from super-Poissonian to Poissonian photon statistics. The measured violation of the Cauchy-Schwarz inequality realizes a direct test of multipartite entanglement in high-harmonic generation [Wasak, Phys. Rev. A , 033616 (2014)]. This result is supported by the theory of multimodal detection and the Hamiltonian from which the effective squeezing modes of the harmonics can be derived [Gonoskov , Phys. Rev. B , 125110 (2024); Christ New J. Phys. , 033027 (2011)]. With this work, we show experimentally that high-harmonic generation is a new quantum bosonic platform that intrinsically produces nonclassical states of light with unique features such as multipartite broadband entanglement or multimode squeezing. The source operates at room temperature, using standard semiconductors and a standard commercial fiber laser, opening up new routes for the quantum industry, such as optical quantum computing, communication, and imaging. Published by the American Physical Society 2024
We derive a quantum macroscopic model for a multimode semiconductor laser, starting from a complete microscopic description. Nonlinear gain terms describing saturation and mode–mode interaction are obtained by a suitable treatment of the spectral hole burning in the distribution of carriers. In the case in which there are two neighbouring active longitudinal modes above threshold and for quiet pumping, we calculate the spectrum of the total intensity fluctuations at zero frequency. For moderate pumping level the nonlinear gain terms do not reduce the degree of anticorrelation between modes, leaving the squeezing in total intensity unchanged with respect to the single-mode case. Only for very high pumping does the nonlinear gain suppression become relevant, and the total intensity noise is increased.
Multimode nonclassical states of light are an essential resource in quantum computation with continuous variables, for example, in cluster state computation. We report in this Letter the first experimental evidence of a multimode nonclassical frequency comb in a femtosecond synchronously pumped optical parametric oscillator. In addition to a global reduction of its quantum intensity fluctuations, the system features quantum correlations between different parts of its frequency spectrum. This allows us to show that the frequency comb is composed of several uncorrelated eigenmodes having specific spectral shapes, two of them at least being squeezed, and to characterize their spectral shapes.