Multiple emitters coherently interacting with an electromagnetic mode give rise to collective effects such as correlated decay and coherent exchange interaction, depending on the separation of the emitters. By diagonalizing the effective non-Hermitian many-body Hamiltonian we reveal the complex-valued eigenvalue spectrum encoding the decay and interaction characteristics. We show that there are significant differences in the emerging collective effects for an array of interacting anharmonic oscillators compared to those of two-level systems and harmonic oscillators. The bosonic decay rate of the most superradiant state increases linearly as a function of the filling factor and exceeds that of two-level systems in magnitude. Furthermore, with bosonic systems, dark states are formed at each filling factor. These are in strong contrast with two-level systems, where the maximal superradiance is observed at half-filling and with larger filling factors superradiance diminishes and no dark states are formed. As an experimentally relevant setup of bosonic waveguide QED, we focus on arrays of transmon devices embedded inside a rectangular waveguide. Specifically, we study the setup of two transmon pairs realized experimentally in Zanner et al. [Nat. Phys. 18, 538 (2022)] and show that it is necessary to consider transmons as bosonic multilevel emitters to accurately recover correct collective effects for the higher excitation manifolds.
Multiple emitters coherently interacting with an electromagnetic mode give rise to collective effects such as correlated decay and coherent exchange interaction, depending on the separation of the emitters. By diagonalizing the effective non-Hermitian many-body Hamiltonian we reveal the complex-valued eigenvalue spectrum encoding the decay and interaction characteristics. We show that there are significant differences in the emerging collective effects for an array of interacting anharmonic oscillators compared to those of two-level systems and harmonic oscillators. The bosonic decay rate of the most superradiant state increases linearly as a function of the filling factor and exceeds that of two-level systems in magnitude. Furthermore, with bosonic systems, dark states are formed at each filling factor. These are in strong contrast with two-level systems, where the maximal superradiance is observed at half-filling and with larger filling factors superradiance diminishes and no dark states are formed. As an experimentally relevant setup of bosonic waveguide QED, we focus on arrays of transmon devices embedded inside a rectangular waveguide. Specifically, we study the setup of two transmon pairs realized experimentally in Zanner et al. [Nat. Phys. 18, 538 (2022)] and show that it is necessary to consider transmons as bosonic multilevel emitters to accurately recover correct collective effects for the higher excitation manifolds.
When multiple quantum emitters couple to a common electromagnetic environment, interference in their collective radiative dynamics gives rise to superradiance and subradiance. In regimes where coherent interactions and collective dissipation compete, the microscopic many-body dynamics and quantum correlations among the emitters that underlie superradiance and subradiance are theoretically challenging and remain experimentally elusive, even though collective emission has been observed in many physical systems. Here, we realize a superconducting qubit array coupled to a common microwave waveguide that mediates collective dissipation, with simultaneous access to coherent interactions and microscopic measurements of many-body dynamics. Engineered qubit-waveguide couplings with tunable amplitude and phase enable control of collective interference and the resulting super- and subradiant states. Leveraging site-resolved control and readout, we directly observe the microscopic decay dynamics of multi-qubit states across different excitation manifolds and track the evolution of populations and tunable quantum correlations. We reveal collective decay in regimes beyond the ideal Dicke model, where strong qubit-qubit interactions stabilize superradiance and subradiance against local dephasing and reshape decay pathways through spatially and spectrally structured many-body eigenstates. Our results establish a flexible platform for exploring collective phenomena in many-body quantum optics and driven-dissipative approaches to robust quantum information processing.
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
Superradiance, the enhanced collective emission of light from a coherent ensemble of quantum systems, has been typically studied in atomic ensembles. In this work we study the enhanced emission of energy from coherent ensembles of harmonic oscillators. We show that it should be possible to observe harmonic oscillator superradiance in a variety of physical platforms such as waveguide arrays in integrated photonics and resonator arrays in circuit QED. We find general conditions specifying when emission is superradiant and subradiant and find that superradiant, subradiant and dark states take the form of multimode squeezed coherent states and highly entangled multimode Fock states. The intensity, two-mode correlations and fraction of quanta trapped in the system after decay are calculated for a range of initial states including multimode Fock, squeezed, coherent and thermal states. In order to explore these effects, the Law and Eberly protocol [C. K. Law and J. H. Eberly, Phys. Rev. Lett. 76, 1055 (1996)] is generalized to prepare highly entangled multimode Fock states in circuit QED.
Abstract This work introduces a theoretical framework to model the collective dynamics of quantum emitters in highly non-Markovian environments, interacting through the exchange of photons with significant retardations. The formalism consists on a set of coupled delay differential equations for the emitter’s raising/lowering operators σ i ± , supplemented by input–output relations that describe the field mediating the interactions. These equations capture the dynamics of both linear (bosonic) and nonlinear (two-level) emitter arrays. It is exact in some limits—e.g. bosonic emitters or generic systems with up to one collective excitation—and can be integrated to provide accurate results for larger numbers of photons. These equations support a study of collective spontaneous emission of emitter arrays in open waveguide-QED environments. This study uncovers an effect we term cascaded super- and sub-radiance, characterized by light-cone-limited propagation and increasingly correlated photon emission across distant emitters. The collective nature of this dynamics for two-level systems is evident both in the enhancement of collective emission rates, as well as in a superradiant burst with a faster than linear growth. While these effects should be observable in existing circuit QED devices or slight generalizations thereof, the formalism put forward in this work can be extended to model other systems such as network of quantum emitters or the generation of correlated photon states.
We consider a pair of identical two-level atoms interacting with a scalar field in one dimension, separated by a distance x21. We obtain collective decaying states, belonging to a complex spectral representation of the Hamiltonian. The imaginary parts of the eigenvalues give the decay rates, and the real parts give the average energy of the collective states. In one dimension there is strong interference between the fields emitted by the atoms, producing cooperative effects even when the atoms are far apart. The decay rates and the energy oscillate with the distance x21. Depending on x21, the decay rates will either decrease, vanish, or increase as compared with the one-atom decay rate. We have sub- and superradiance at periodic intervals. Our model may be used to study two-cavity electron waveguides. The vanishing of the collective decay rates then suggests the possibility of obtaining stable configurations, where an electron is trapped inside the two cavities.
Waveguide quantum electrodynamics studies photon-mediated interactions of quantum emitters in a one-dimensional radiation channel. Although signatures of such interactions have been observed previously in a variety of physical systems, observation of coherent cooperative dynamics has been obscured by radiative decay of atoms into the waveguide. Employing transmon qubits as artificial atoms coupled to a microwave coplanar waveguide, here we observe dynamical oscillations in an open system where a designated probe qubit interacts with an entangled dark state of an array of qubits which effectively traps radiation as an atomic cavity. The qubit-cavity system is shown to achieve a large cooperativity of C=172 due to collective enhancement of photon-mediated interactions, entering the strong coupling regime. The quantum coherence of the dark state cavity is also explored through its nonlinear response at the single-excitation level. With realistic refinements, this system is suitable for studying the many-body dynamics of large (N>10) quantum spin chains, synthesizing highly non-classical radiation fields on demand, and implementing universal quantum logic operations with high fidelity on information encoded within decoherence-free subspaces.