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arXiv:2112.05747

Transport in the emergent Bose liquid: Bad metal, strange metal, and weak insulator, all in one system

Zeng, Tao, Anthony Hegg, Zou, Long, Shengtao Jiang, Wei Ku

Published Dec 10, 2021• 2 citations
arXivHTMLPDF

Abstract

Non-saturating high-temperature resistivity ("bad metal"), T-linear low-temperature resistivity ("strange metal"), and a crossover to activation-free growth of the resistivity in the low-temperature limit ("weak insulator") are among the most exotic behaviors widely observed in many strongly correlated materials for decades that defy the standard Fermi liquid description of solids. Here we investigate these puzzling behaviors by computing temperature-dependent optical conductivity of an emergent Bose liquid and find that it reproduces all the unexplained features of the experiments, including a featureless continuum and a well-known mid-infrared peak. Amazingly and with physically intuitive mechanisms, the corresponding doping- and temperature-dependent resistivity displays the bad metal and strange metal simultaneously and sometimes weak insulating behaviors as well. The unification of all these non-Fermi liquid behaviors in a single model suggests that a new quantum state of matter, namely the emergent Bose liquid, will guide the development of the next generation of solid state physics.

DOI
10.48550/arxiv.2112.05747

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Non-saturating high-temperature resistivity ("bad metal"), T-linear low-temperature resistivity ("strange metal"), and a crossover to activation-free growth of the resistivity in the low-temperature limit ("weak insulator") are among the most exotic behaviors widely observed in many strongly correlated materials for decades that defy the standard Fermi liquid description of solids. Here we investigate these puzzling behaviors by computing temperature-dependent optical conductivity of an emergent Bose liquid and find that it reproduces all the unexplained features of the experiments, including a featureless continuum and a well-known mid-infrared peak. Amazingly and with physically intuitive mechanisms, the corresponding doping- and temperature-dependent resistivity displays the bad metal and strange metal simultaneously and sometimes weak insulating behaviors as well. The unification of all these non-Fermi liquid behaviors in a single model suggests that a new quantum state of matter, namely the emergent Bose liquid, will guide the development of the next generation of solid state physics.
Metallic quantum states coined strange metal (SM), with robust linear-TTT resistivity, have been widely observed in many quantum materials under strong electron correlations, ranging from high-Tc{T}_{c}Tc​ cuprate superconductors and organic superconductors to twisted multilayer graphene and MoTe2/WSe2{\mathrm{MoTe}}_{2}/{\mathrm{WSe}}_{2}MoTe2​/WSe2​ superlattices. Despite decades of intensive studies, the mystery of SM still defies any sensible theoretical explanation and has been a key puzzle in modern condensed matter physics. Here, we solve a doped Mott insulator model called an Ising-Kondo lattice, which includes static spin fluctuation. With Monte Carlo simulation, the Ising-Kondo lattice unambiguously exhibits SM phenomena accompanied with quantum critical scaling in observables, e.g., resistivity, susceptibility, and specific heat. A closer look at SM reveals the breakdown of Landau's Fermi liquid theory without any symmetry breaking, i.e., the violation of Luttinger theorem. Our paper reveals that the long-overlooked static fluctuations in literature may play an essential role in non-Fermi liquid behaviors in correlated electron systems.
Quantum simulations are quickly becoming an indispensable tool for studying particle transport in correlated lattice models. One of the central topics in the study of transport is bad-metal behavior, characterized by the direct-current resistivity linear in temperature. In the fermionic Hubbard model, optical conductivity has been studied extensively, and a recent optical lattice experiment demonstrated bad-metal behavior in qualitative agreement with theory. Far less is known about transport in the bosonic Hubbard model. We investigate the conductivity in the Bose-Hubbard model and focus on the regime of strong interactions and high temperatures. We use numerically exact calculations for small lattice sizes. At weak tunneling, we find multiple peaks in the optical conductivity that stem from the Hubbard bands present in the many-body spectrum. This feature slowly washes out as the tunneling rate gets stronger. At high temperature, we identify a regime of TTT-linear resistivity, as expected. When the interactions are very strong, the leading inverse-temperature coefficient in conductivity is proportional to the tunneling amplitude. As the tunneling becomes stronger, this dependence takes quadratic form. At very strong coupling and half filling, we identify a separate linear resistivity regime at lower temperature, corresponding to the hard-core boson regime. Additionally, we unexpectedly observe that at half filling, in a big part of the phase diagram, conductivity is an increasing function of the coupling constant before it saturates at the hard-core-boson result. We explain this feature based on the analysis of the many-body energy spectrum and the contributions to conductivity of individual eigenstates of the system.
Strongly correlated materials, where electron-electron interactions dominate, display a range of important yet poorly understood phenomena including high-temperature superconductivity and exotic magnetism. Many such materials also feature unusual ``strange-metal'' transport, corresponding to unexpected temperature dependence of the resistivity. The authors show that, due to band-structure nesting and a bounded spectrum, even a weakly interacting system can display resistivity signatures that are typically associated with such strange metals. Their results are particularly important for interpreting recent cold-atom experiments which explore transport in the Fermi Hubbard model.
Recent progress in extremely correlated Fermi liquid theory (ECFL) and the dynamical mean field theory (DMFT) enables us to accurately compute in the $d\ensuremath{\rightarrow}\ensuremath{\infty}$ limit the resistivity of the $t\ensuremath{-}J$ model after setting $J\ensuremath{\rightarrow}0$. This is also the $U=\ensuremath{\infty}$ Hubbard model. Since JJJ is set to zero, our study isolates the dynamical effects of the single occupation constraint enforced by the projection operator originally introduced by Gutzwiller. We study three densities n=.75,.8,.85n=.75,.8,.85n=.75,.8,.85 that correspond to a range between the overdoped and optimally doped Mott insulating state. We delineate four distinct regimes separated by three crossovers, which are characterized by different behaviors of the resistivity $\ensuremath{\rho}$. We find at the lowest temperature TTT a Gutzwiller correlated Fermi liquid regime with $\ensuremath{\rho}\ensuremath{\propto}{T}^{2}$ extending up to an effective Fermi temperature that is dramatically suppressed from the noninteracting value by the proximity to half filling, $n\ensuremath{\sim}1$. This is followed by a Gutzwiller correlated strange metal regime with $\ensuremath{\rho}\ensuremath{\propto}(T\ensuremath{-}{T}_{0})$, i.e., a linear resistivity extrapolating back to $\ensuremath{\rho}=0$ at a positive T0{T}_{0}T0​. At a higher temperature scale this crosses over into the bad metal regime with $\ensuremath{\rho}\ensuremath{\propto}(T+{T}_{1})$, i.e., a linear resistivity extrapolating back to a finite resistivity at T=0T=0T=0 and passing through the Ioffe-Regel-Mott value where the mean free path is a few lattice constants. This regime finally gives way to the high TTT metal regime, where we find $\ensuremath{\rho}\ensuremath{\propto}T$, i.e., a linear resistivity extrapolating back to zero at T=0T=0T=0. The present work emphasizes the first two, i.e., the two lowest temperature regimes, where the availability of an analytical ECFL theory is of help in identifying the changes in related variables entering the resistivity formula that accompanies the onset of linear resistivity, and the numerically exact DMFT helps to validate the results. We also examine thermodynamical variables such as the magnetic susceptibility, compressibility, heat capacity, and entropy and correlate changes in these with the change in resistivity. This exercise casts valuable light on the nature of charge and spin correlations in the Gutzwiller correlated strange metal regime, which has features in common with the physically relevant strange metal phase seen in strongly correlated matter.
Many strongly correlated systems exhibit strange metallic behavior in certain parameter regimes characterized by anomalous transport properties that are irreconcilable with a Fermi-liquid-like description in terms of quasiparticles. The Hubbard model is a standard theoretical starting point to examine the properties of such systems and also exhibits non-Fermi-liquid behavior in simulations. Here we analytically study the two-dimensional hole-doped Hubbard model in the large UUU limit, first identifying a doping-induced percolation transition in the low-energy sector occurring at a definite critical doping pc{p}_{c}pc​ depending on lattice structure. Using the critical properties near this transition we rewrite the Hubbard Hamiltonian and motivate a low-energy lattice-independent large-NNN model with distinct non-Fermi-liquid properties. We show that this model has linear-in-TTT resistivity with doping-dependent slope maximized at p=pcp={p}_{c}p=pc​ and power-law optical conductivity ${\ensuremath{\sim}|\ensuremath{\omega}|}^{\ensuremath{-}2/3}$. Though the parameters used in developing this theory mean it cannot be directly applied to the cuprate superconductors, we nevertheless reproduce several important phenomena observed in their strange metal phase and also predict these same qualitative behaviors to manifest in other lattices near concrete hole dopings.
A long-standing mystery of fundamental importance in correlated electron physics is to understand strange non-Fermi liquid metals that are seen in diverse quantum materials. A striking experimental feature of these metals is a resistivity that is linear in temperature (T). In this Letter we ask what it takes to obtain such non-Fermi liquid physics down to zero temperature in a translation invariant metal. If in addition the full frequency (ω) dependent conductivity satisfies ω/T scaling, we argue that the T-linear resistivity must come from the intrinsic physics of the low energy fixed point. Combining with earlier arguments that compressible translation invariant metals are "ersatz Fermi liquids" with an infinite number of emergent conserved quantities, we obtain powerful and practical conclusions. We show that there is necessarily a diverging susceptibility for an operator that is odd under inversion and time reversal symmetries, and has zero crystal momentum. We discuss a few other experimental consequences of our arguments, as well as potential loopholes, which necessarily imply other exotic phenomena.