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arXiv:2112.03128 · Journal of Physics A Mathematical and Theoretical

Broken-axisymmetry state and magnetic state diagram of spin-1 condensate through the prism of quadrupole degrees of freedom

M. S. Bulakhov, A. S. Peletminskii, S. V. Peletminskiǐ, Yu. V. Slyusarenko

Published Sep 8, 2022• 2 citations
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Abstract

Abstract We theoretically study a weakly interacting gas of spin-1 atoms with Bose–Einstein condensate in external magnetic field within the Bogoliubov approach. To this end, in contrast to previous studies, we employ the general Hamiltonian, which includes both spin and quadrupole exchange interactions as well as the couplings of the spin and quadrupole moment with the external magnetic field (the linear and quadratic Zeeman terms). The latter is responsible for the emergence of the broken-axisymmetry state. We also reexamine ferromagnetic, quadrupolar, and paramagnetic states employing the proposed Hamiltonian. For all magnetic states, we find the relevant thermodynamic characteristics such as magnetization, quadrupole moment, thermodynamic potential. We also obtain three-branch excitation spectrum of the broken-axisymmetry state. We show that this state can be prepared at three different regimes of applied magnetic field. Finally, we present the magnetic state diagrams for each regime of realizing the broken-axisymmetry state.

DOI
10.1088/1751-8121/ac9098

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Abstract We theoretically study a weakly interacting gas of spin-1 atoms with Bose–Einstein condensate in external magnetic field within the Bogoliubov approach. To this end, in contrast to previous studies, we employ the general Hamiltonian, which includes both spin and quadrupole exchange interactions as well as the couplings of the spin and quadrupole moment with the external magnetic field (the linear and quadratic Zeeman terms). The latter is responsible for the emergence of the broken-axisymmetry state. We also reexamine ferromagnetic, quadrupolar, and paramagnetic states employing the proposed Hamiltonian. For all magnetic states, we find the relevant thermodynamic characteristics such as magnetization, quadrupole moment, thermodynamic potential. We also obtain three-branch excitation spectrum of the broken-axisymmetry state. We show that this state can be prepared at three different regimes of applied magnetic field. Finally, we present the magnetic state diagrams for each regime of realizing the broken-axisymmetry state.
Abstract We obtain and justify a many-body Hamiltonian of pairwise interacting spin-1 atoms, which includes eight generators of the SU(3) group associated with spin and quadrupole degrees of freedom. It is shown that this Hamiltonian is valid for non-local interaction potential, whereas for local interaction specified by s -wave scattering length, the Hamiltonian should be bilinear in spin operators only (of the Heisenberg type). We apply the obtained Hamiltonian to study the ground-state properties and single-particle excitations of a weakly interacting gas of spin-1 atoms with Bose–Einstein condensate (BEC) taking into account the quadrupole degrees of freedom. It is shown that the system under consideration can be in ferromagnetic, quadrupole, and paramagnetic phases. The corresponding phase diagram is constructed and discussed. The main characteristics such as the density of the grand thermodynamic potential, condensate density, and single-particle excitation spectra modified by quadrupole degrees of freedom are determined in different phases.
We study the ground-state phases for a mixture of two atomic spin-1 Bose-Einstein condensates in the presence of a weak magnetic (BBB) field. The ground state is found to contain a broken-axisymmetry (BA) phase due to competitions among intraspecies and interspecies spin-exchange interactions and the linear Zeeman shifts. This is in contrast to the case of a single-species spin-1 condensate, where the axisymmetry breaking results from competitions among the linear and quadratic Zeeman shifts and the intraspecies ferromagnetic interaction. All other remaining ground-state phases for the mixture are found to preserve axisymmetry. We further elaborate on the ground-state phase diagram and calculate the Bogoliubov excitation spectra of the phases. For the BA phase, there exist three Goldstone modes that attempt to restore the broken U(1) and SO(2) symmetries.
We study experimentally the equilibrium phase diagram of a spin-1 Bose-Einstein condensate with antiferromagnetic interactions, in a regime where spin and spatial degrees of freedom are decoupled. For a given total magnetization mz{m}_{z}mz​, we observe for low magnetic fields an ``antiferromagnetic'' phase where atoms condense in the $m=\ifmmode\pm\else\textpm\fi{}1$ Zeeman states, and occupation of the m=0m=0m=0 state is suppressed. Conversely, for large enough magnetic fields, a phase transition to a ``broken-axisymmetry'' phase takes place: The m=0m=0m=0 component becomes populated and rises sharply above a critical field Bc(mz){B}_{c}({m}_{z})Bc​(mz​). This behavior results from the competition between antiferromagnetic spin-dependent interactions (dominant at low fields) and the quadratic Zeeman energy (dominant at large fields). We compare the measured Bc{B}_{c}Bc​ as well as the global shape of the phase diagram with mean-field theory, and find good quantitative agreement.
We have numerically solved the low-energy excitation spectra of ferromagnetic Bose-Einstein condensates subject to dipolar interparticle interactions. The system is assumed to be harmonically confined by purely optical means, thereby maintaining the spin degree of freedom of the condensate order parameter. Using a zero-temperature spin-1 model, we solve the Bogoliubov excitations for different spin textures, including a spin-vortex state in the absence of external magnetic fields and a rapidly rotating polarized spin texture in a finite homogeneous field. In particular, we consider the effect of dipolar interactions on excitations characteristic of ferromagnetic condensates. The energies of spin waves and magnetic quadrupole modes are found to increase rapidly with the dipolar coupling strength, whereas the energies of density oscillations change only slightly.
We provide the general arguments that quantum atomic gases of interacting high-spin atoms represent a physical system in which the multipole (hidden) degrees of freedom may be manifested. Their manifestation occurs when the interatomic interaction is of non-local type. For a local interaction described by the s-wave scattering length, the multipole degrees of freedom do not reveal themselves. To illustrate our findings, we theoretically examine the phenomenon of Bose–Einstein condensation in an interacting gas of spin-1 atoms in an external magnetic field. This study is based on the SU(2) invariant Hamiltonian, which has a bilinear structure in the spin and quadrupole operators along with the scalar term. It is shown that depending on the conditions imposed on the interaction amplitudes (stability conditions), the ground state of the system may exhibit three different phases: quadrupolar, ferromagnetic, and paramagnetic. The basic thermodynamic characteristics affected by hidden degrees of freedom are found for all phases.