Among the best known quantities obtainable from photon correlation measurements are the g ( m ) correlation functions. Here, we introduce a new procedure to evaluate these correlation functions based on higher-order factorial cumulants C F, m that integrate over the time dependence of the correlation functions, that is, summarize the available information at different time spans. In a systematic manner, the information content of higher-order correlation functions as well as the distribution of photon waiting times is taken into account. Our procedure greatly enhances the sensitivity for probing correlations and, moreover, is robust against a limited counting efficiency and time resolution in experiment. It can be applied even in case g ( m ) is not accessible at short time spans. We use the new evaluation scheme to analyze the photon emission of a plasmonic cavity coupled to a single quantum dot. We derive criteria that must hold if the system can be described by a generic Jaynes–Cummings model. A violation of the criteria can be explained by the presence of an additional excited quantum dot state.
Among the best known quantities obtainable from photon correlation measurements are the g ( m ) correlation functions. Here, we introduce a new procedure to evaluate these correlation functions based on higher-order factorial cumulants C F, m that integrate over the time dependence of the correlation functions, that is, summarize the available information at different time spans. In a systematic manner, the information content of higher-order correlation functions as well as the distribution of photon waiting times is taken into account. Our procedure greatly enhances the sensitivity for probing correlations and, moreover, is robust against a limited counting efficiency and time resolution in experiment. It can be applied even in case g ( m ) is not accessible at short time spans. We use the new evaluation scheme to analyze the photon emission of a plasmonic cavity coupled to a single quantum dot. We derive criteria that must hold if the system can be described by a generic Jaynes–Cummings model. A violation of the criteria can be explained by the presence of an additional excited quantum dot state.
High-order photon correlations of light fields are important for characterizing the quantum nature. Since Hanbury Brown and Twiss conducted the pioneering experiments in the 1950s, the HBT effect has inspired extensive research on high-order photon correlation in quantum optics, quantum information, and quantum imaging. The Single-photon counting module is one of the most widely used single-photon detectors. Due to its high detection efficiency and low dark counts in the visible and near-infrared region, it is reasonably chosen for basic research on quantum mechanics. Many researches have demonstrated that the maximum value of second-order photon correlation g(2)(τ) at zero delay (τ = 0) can be used to distinguish different light fields. Therefore, the HBT scheme containing two single photon detectors have been widely used in many advanced studies, such as space interference, ghost imaging, single photon detection with high efficiency, etc. However, higher-order photon correlations g(n) (n > 2) can reveal more measurable characteristics of light fields, such as information about the non-Gaussian scattering process, the skewness and kurtosis of photon number distribution, etc. When the extended HBT scheme is used to measure higher-order photon correlations, the experimental conditions including quantum efficiency and background noise greatly affect the photon correlation measurement. The influences of the counting rate and resolution time of the detection system on the measurements are also very important and cannot be ignored. Therefore, the comprehensive considering of various influence factors is necessary for accurately measuring the high-order photon correlations and also a challenge. In this paper, we present a method based on double Hanbury Brown-Twiss scheme for the accurate measuring of high-order photon correlations g(n) (n > 2). The system consists of four single photon counting modules and is used to detect and analyze the joint distribution probability of temporal photon correlation. Considering the effects of the background noise and overall efficiency, theoretically, we analyze the correlations of the third- and fourth-order photon with the incident light intensity, squeezing parameter and photon number respectively for thermal state, coherent state, squeezed vacuum state, and Fock state. Meanwhile, experimentally we study the influences of resolution time and counting rate on correlations of the coherent state and thermal state with third- and fourth-order photon. On condition that the resolution time is 210 ns and the counting rate is 80 kc/s, the correlations of third and fourth-order photon with the thermal state at zero time delay are accurately measured, and the relative statistical deviations of the measured vales from the theoretical values are 0.3% and 0.8%, respectively. In addition, the third- and fourth-order photon correlations of the thermal state at different delay times are also observed. It is demonstrated that the high-order photon correlations of light fields are measured accurately by comprehensively analyzing various influencing factors. This technique provides a promising and useful tool to investigate quantum correlated imaging and quantum coherence of light fields.
Quantum mechanically indistinguishable particles such as photons may show collective behavior. Therefore, an appropriate description of a light field must consider the properties of an assembly of photons instead of independent particles. We have studied multiphoton correlations up to fourth order in the single-mode emission of a semiconductor microcavity in the weak and strong coupling regimes. The counting statistics of single photons were recorded with picosecond time resolution, allowing quantitative measurement of the few-photon bunching inside light pulses. Our results show bunching behavior in the strong coupling case, which vanishes in the weak coupling regime as the cavity starts lasing. In particular, we verify the n factorial prediction for the zero-delay correlation function of n thermal light photons.
We study, in theory and experiment, the quantum properties of correlated light fields measured with click-counting detectors providing incomplete information on the photon statistics. We establish a correlation parameter for the conditional statistics, and we derive the corresponding nonclassicality criteria for detecting conditional quantum correlations. Classical bounds for Pearson's correlation parameter are formulated that allow us, once they are violated, to determine nonclassical correlations via the joint statistics. On the one hand, we demonstrate nonclassical correlations in terms of the joint click statistics of light produced by a parametric down-conversion source. On the other hand, we verify quantum correlations of a heralded, split single-photon state via the conditional click statistics together with a generalization to higher-order moments. We discuss the performance of the presented nonclassicality criteria to successfully discern joint and conditional quantum correlations. Remarkably, our results are obtained without making any assumptions on the response function, quantum efficiency, and dark-count rate of photodetectors.
The time dynamics of spin-injected, electrically contacted quantum dots were investigated with a focus on the time evolution of photon statistics. Photon statistics can provide insights into whether the device functions as an effective single-photon emitter or exhibits higher-order emissions. Through these investigations, we found that the shape of the electrical excitation pulse has a direct impact on photon statistics. Specifically, the rising edge of the pulse corresponds to a significantly higher number of higher-order photon states, which decay much faster than single photons associated with the falling edge of the electrical pulse. This relationship implies that the pulse shape can be tailored to optimize the device as either a better single-photon source or a generator of higher-order photon states, with potential applications in creating deterministic higher-order photon Fock states. The ability to easily modify the pulse shape is a unique feature of electrically excited quantum dots.
We measure second- and third-order temporal coherences, g((2))(τ) and g((3))(τ1,τ2), of an optically excited single-photon source: an InGaAs quantum dot in a microcavity pedestal. Increasing the optical excitation power leads to an increase in the measured count rate, and also an increase in multi-photon emission probability. We show that standard measurements of g((2)) provide limited information about this multi-photon probability, and that more information can be gained by simultaneously measuring g((3)). Experimental results are compared with a simple theoretical model to show that the observed antibunchings are consistent with an incoherent addition of two sources: 1) an ideal single-photon source that never emits multiple photons and 2) a background cavity emission having Poissonian photon number statistics. Spectrally resolved cross-correlation measurements between quantum-dot and cavity modes show that photons from these two sources are largely uncorrelated, further supporting the model. We also analyze the Hanbury Brown-Twiss interferometer implemented with two or three "click" detectors, and explore the conditions under which it can be used to accurately measure g((2))(τ) and g((3))(τ1,τ2).
We present a theoretical analysis of the intensity correlation functions for the spontaneous emission from a planar ensemble of self-assembled quantum dots. Using the quantum jump approach, we numerically simulate the evolution of the system and construct photon-photon delay time statistics that approximates the second-order correlation functions of the field. The form of this correlation function in the case of collective emission from a highly homogeneous ensemble qualitatively differs from that characterizing an ensemble of independent emitters (inhomogeneous ensemble of uncoupled dots). The signatures of collective emission are observed also in the case of an inhomogeneous but sufficiently strongly coupled ensemble. Different forms of the correlation functions are observed in the intensity autocorrelations and in cross correlations between various spectral ranges, revealing the quantum state projection associated with the detection event and the subsequent interaction-induced redistribution of occupations. The predicted effect of collective dynamics on the correlation functions appears under various excitation conditions. Thus, we show that the second-order correlation function of the emitted field provides a sensitive test of cooperative effects.