Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2112.01952 · Physical review. B./Physical review. B

Isothermal and adiabatic magnetization processes of the spin- 12 Heisenberg model on an anisotropic triangular lattice

Katsuhiro Morita

Published Feb 22, 2022• 7 citations
arXivHTMLPDF

Abstract

In this study, we investigate the magnetic susceptibility, entropy, and isothermal magnetization curve of the spin-1/2 Heisenberg model on an anisotropic triangular lattice using the orthogonalized finite-temperature Lanczos method. In addition, we investigate the adiabatic magnetization curve and magnetocaloric effect. We estimate these physical quantities with sufficient accuracy in the thermodynamic limit, except at low temperatures. We observe a 1/3 magnetization plateau in the isothermal magnetization process, whereas the plateau is observed to have a slope in the adiabatic process. We show that the magnetocaloric effect can be used to detect the signature of phase transitions. We believe that these results will be useful for understanding the magnetism of anisotropic triangular lattice compounds through a comparison with experimental results in the future.

DOI
10.1103/physrevb.105.064428

Related papers

Spin-1/2 XXZ Heisenberg cupolae: magnetization process and related enhanced magnetocaloric effect

Katarína Karľová

The magnetization curves and magnetocaloric effect during the adiabatic demagnetization of antiferromagnetic spin-1/2 XXZ Heisenberg clusters with the shape of Johnson's solids (triangular cupola, square cupola and pentagonal cupola) are investigated using the exact numerical diagonalization for different values of the exchange anisotropy ranging in between the Ising and fully isotropic limit. It is demonstrated that spin-1/2 XXZ Heisenberg cupolae display, in comparison with their Ising counterparts, at least one more magnetization plateau. The novel magnetization plateaux extends over a wider range of the magnetic fields with increasing of a quantum part of the XXZ exchange coupling at the expense of the original plateaux present in the limiting Ising case. It is shown that the spin-1/2 XXZ Heisenberg triangular and pentagonal cupolae exhibit an enhanced magnetocaloric effect in the vicinity of zero magnetic field, which makes these magnetic systems promising refrigerants for cooling down to ultra-low zero temperatures.

arXiv:2002.06907•Condensed Matter Physics•Dec 1, 2020•6 citations

Magnetothermal properties of the Heisenberg-Ising orthogonal-dimer chain with triangular XXZ clusters

Vadim Ohanyan, A. Honecker

We study a spin-1/2 model with triangular $XXZ$ clusters on the orthogonal-dimer chain in the presence of an external magnetic field. First, we discuss the case where the triangular clusters are coupled via intermediate ``classical'' Ising spins. Diagonalization of the triangular $XXZ$ clusters yields the exact ground states; finite-temperature properties are computed exactly by an additional transfer-matrix step. A detailed analysis reveals a large variety of ground states at magnetization $M$ equal to fractions 0, $1/4$, and $1/2$ of the saturation magnetization $M=1$. Some of these ground states break translational symmetry spontaneously and give rise to doubling of the unit cell. In a second part, we present complementary numerical data for the spin-1/2 Heisenberg model on the orthogonal-dimer chain. We analyze several examples of $T=0$ magnetization curves, entropy as a function of temperature $T$ and magnetic field, and the associated magnetic cooling rate. Comparison of the two models shows that in certain situations the simplified exactly solvable model yields a qualitatively or sometimes even quantitatively accurate description of the more challenging quantum model, including a case which may be relevant to experimental observations of an enhanced magnetocaloric effect in the two-dimensional compound SrCu${}_{2}$(BO${}_{3}$)${}_{2}$.

arXiv:1203.4741•Physical Review B•Aug 9, 2012•42 citations

Thermodynamics of anisotropic triangular magnets with ferro- and antiferromagnetic exchange

Burkhard Schmidt, Peter Thalmeier

We investigate thermodynamic properties like specific heat c V and susceptibility χ in anisotropic J 1 – J 2 triangular quantum spin systems ( ). As a universal tool we apply the finite temperature Lanczos method (FTLM) based on exact diagonalization of finite clusters with periodic boundary conditions. We use clusters up to N = 28 sites where the thermodynamic limit behavior is already stably reproduced. As a reference we also present the full diagonalization of a small eight-site cluster. After introducing model and method we discuss our main results on c V ( T ) and . We show the variation of peak position and peak height of these quantities as function of control parameter . We demonstrate that maximum peak positions and heights in Néel phase and spiral phases are strongly asymmetric, much more than in the square lattice J 1 – J 2 model. Our results also suggest a tendency to a second side maximum or shoulder formation at lower temperature for certain ranges of the control parameter. We finally explicitly determine the exchange model of the prominent triangular magnets Cs 2 CuCl 4 and Cs 2 CuBr 4 from our FTLM results.

arXiv:1506.09104•New Journal of Physics•Jul 22, 2015•37 citations

Ising versus Potts criticality in low-temperature magnetothermodynamics of a frustrated spin- 12 Heisenberg triangular bilayer

Jozef Strečka, Katarína Karľová, Vasyl Baliha +1 more

Low-temperature magnetization curves and thermodynamics of a frustrated spin-$\frac{1}{2}$ Heisenberg triangular bilayer with the antiferromagnetic intradimer interaction and either ferromagnetic or antiferromagnetic interdimer interaction are investigated in a highly frustrated parameter region, where localized many-magnon eigenstates provide the most dominant contribution to magnetothermodynamics. Low-energy states of the highly frustrated spin-$\frac{1}{2}$ Heisenberg triangular bilayer can be accordingly found from a mapping correspondence with an effective triangular-lattice spin-$\frac{1}{2}$ Ising model in a field. A description based on the effective Ising model implies that the frustrated Heisenberg triangular bilayer with the ferromagnetic interdimer coupling displays in a zero-temperature magnetization curve discontinuous magnetization jump, which is reduced upon increasing of temperature until a continuous field-driven phase transition from the Ising universality class is reached at a certain critical temperature. The frustrated Heisenberg triangular bilayer with the antiferromagnetic interdimer coupling contrarily exhibits multistep magnetization curve with intermediate plateaus at $\frac{1}{3}$ and $\frac{2}{3}$ of the saturation magnetization, whereas discontinuous magnetization jumps observable at zero temperature change to continuous field-driven phase transitions from the universality class of three-state Potts model at sufficiently low temperatures. Exact results and Monte Carlo simulations of the effective Ising model are confronted with full exact diagonalization data for the Heisenberg triangular bilayer in order to corroborate these findings.

arXiv:1807.08042•Physical review. B./Physical review. B•Nov 21, 2018•7 citations

Magnetization plateaus and enhanced magnetocaloric effect of a spin-1/2 Ising-Heisenberg and Heisenberg double sawtooth ladder with four-spin interaction

Hamid Arian Zad, Vadim Ohanyan, Azam Zoshki +1 more

The ground state, entropy, and magnetic Grüneisen parameter of the antiferromagnetic spin-1/2 Ising-Heisenberg model on a double sawtooth ladder are rigorously investigated using the classical transfer-matrix technique. The model includes the XXZ interaction between the interstitial Heisenberg dimers, the Ising coupling between nearest-neighbor spins of the legs and rungs, and additional cyclic four-spin Ising term in each square plaquette. For a particular value of the cyclic four-spin exchange, we found in the ground-state phase diagram of the Ising-Heisenberg ladder a quadruple point, at which four different ground states coexist together. During an adiabatic demagnetization process, a fast cooling accompanied with an enhanced magnetocaloric effect can be detected near this quadruple point. The ground-state phase diagram of the Ising-Heisenberg ladder is confronted with the zero-temperature magnetization process of the purely quantum Heisenberg ladder, which is calculated by using exact diagonalization based on the Lanczos algorithm for a finite-size ladder of 24 spins and the density-matrix renormalization group simulations for a finite-size ladder with up to 96 spins. Some indications of the existence of intermediate magnetization plateaus in the magnetization process of the full Heisenberg model for a small but nonzero four-spin Ising coupling were found. The DMRG results reveal that the quantum Heisenberg double sawtooth ladder exhibits some quantum Luttinger spin-liquid phase regions that are absent in the Ising-Heisenberg counterpart model. Except this difference, the magnetic behavior of the full Heisenberg model is quite analogous to its simplified Ising-Heisenberg counterpart and, hence, may bring insight into the fully quantum Heisenberg model from rigorous results for the Ising-Heisenberg model.

arXiv:2307.03855•Physical review. E•Oct 19, 2023•9 citations

Unveiling Magnetic Frustration via the Elastocaloric Effect

Eric C. Andrade, Pedro M. Cônsoli, Matthias Vojta C

Motivated by experimental progress in pressure and strain tuning of quantum materials, we examine the thermodynamic response of frustrated magnets to uniaxial strain. Specifically, we study Ising and Heisenberg models on spatially anisotropic triangular (and, for the Ising model, also kagome) lattices. We determine the entropy as a function of temperature and strain, and use it to compute the elastic Grüneisen ratio $η$. The Ising models can be strain-tuned into and out of classical spin-liquid phases, and we show that $η$ can become arbitrarily large at low temperature $T$ near the point of maximal frustration, a universal hallmark of an extensive ground-state entropy. In contrast, the spin-$1/2$ Heisenberg model is moderately frustrated and displays multiple $T=0$ phase transitions. These transitions dominate $η$ at low $T$ while the intermediate-$T$ behavior is similar to that of the Ising model. We discuss the extent to which the elastic Grüneisen ratio can be used to deduce the phase diagram, and we connect our results to recent experiments on triangular-lattice magnets.

arXiv:2605.15274•May 14, 2026•0 citations
In this study, we investigate the magnetic susceptibility, entropy, and isothermal magnetization curve of the spin-1/2 Heisenberg model on an anisotropic triangular lattice using the orthogonalized finite-temperature Lanczos method. In addition, we investigate the adiabatic magnetization curve and magnetocaloric effect. We estimate these physical quantities with sufficient accuracy in the thermodynamic limit, except at low temperatures. We observe a 1/3 magnetization plateau in the isothermal magnetization process, whereas the plateau is observed to have a slope in the adiabatic process. We show that the magnetocaloric effect can be used to detect the signature of phase transitions. We believe that these results will be useful for understanding the magnetism of anisotropic triangular lattice compounds through a comparison with experimental results in the future.
The magnetization curves and magnetocaloric effect during the adiabatic demagnetization of antiferromagnetic spin-1/2 XXZ Heisenberg clusters with the shape of Johnson's solids (triangular cupola, square cupola and pentagonal cupola) are investigated using the exact numerical diagonalization for different values of the exchange anisotropy ranging in between the Ising and fully isotropic limit. It is demonstrated that spin-1/2 XXZ Heisenberg cupolae display, in comparison with their Ising counterparts, at least one more magnetization plateau. The novel magnetization plateaux extends over a wider range of the magnetic fields with increasing of a quantum part of the XXZ exchange coupling at the expense of the original plateaux present in the limiting Ising case. It is shown that the spin-1/2 XXZ Heisenberg triangular and pentagonal cupolae exhibit an enhanced magnetocaloric effect in the vicinity of zero magnetic field, which makes these magnetic systems promising refrigerants for cooling down to ultra-low zero temperatures.
We study a spin-1/2 model with triangular XXZXXZXXZ clusters on the orthogonal-dimer chain in the presence of an external magnetic field. First, we discuss the case where the triangular clusters are coupled via intermediate ``classical'' Ising spins. Diagonalization of the triangular XXZXXZXXZ clusters yields the exact ground states; finite-temperature properties are computed exactly by an additional transfer-matrix step. A detailed analysis reveals a large variety of ground states at magnetization MMM equal to fractions 0, 1/41/41/4, and 1/21/21/2 of the saturation magnetization M=1M=1M=1. Some of these ground states break translational symmetry spontaneously and give rise to doubling of the unit cell. In a second part, we present complementary numerical data for the spin-1/2 Heisenberg model on the orthogonal-dimer chain. We analyze several examples of T=0T=0T=0 magnetization curves, entropy as a function of temperature TTT and magnetic field, and the associated magnetic cooling rate. Comparison of the two models shows that in certain situations the simplified exactly solvable model yields a qualitatively or sometimes even quantitatively accurate description of the more challenging quantum model, including a case which may be relevant to experimental observations of an enhanced magnetocaloric effect in the two-dimensional compound SrCu2{}_{2}2​(BO3{}_{3}3​)2{}_{2}2​.
We investigate thermodynamic properties like specific heat c V and susceptibility χ in anisotropic J 1 – J 2 triangular quantum spin systems ( ). As a universal tool we apply the finite temperature Lanczos method (FTLM) based on exact diagonalization of finite clusters with periodic boundary conditions. We use clusters up to N = 28 sites where the thermodynamic limit behavior is already stably reproduced. As a reference we also present the full diagonalization of a small eight-site cluster. After introducing model and method we discuss our main results on c V ( T ) and . We show the variation of peak position and peak height of these quantities as function of control parameter . We demonstrate that maximum peak positions and heights in Néel phase and spiral phases are strongly asymmetric, much more than in the square lattice J 1 – J 2 model. Our results also suggest a tendency to a second side maximum or shoulder formation at lower temperature for certain ranges of the control parameter. We finally explicitly determine the exchange model of the prominent triangular magnets Cs 2 CuCl 4 and Cs 2 CuBr 4 from our FTLM results.
Low-temperature magnetization curves and thermodynamics of a frustrated spin-12\frac{1}{2}21​ Heisenberg triangular bilayer with the antiferromagnetic intradimer interaction and either ferromagnetic or antiferromagnetic interdimer interaction are investigated in a highly frustrated parameter region, where localized many-magnon eigenstates provide the most dominant contribution to magnetothermodynamics. Low-energy states of the highly frustrated spin-12\frac{1}{2}21​ Heisenberg triangular bilayer can be accordingly found from a mapping correspondence with an effective triangular-lattice spin-12\frac{1}{2}21​ Ising model in a field. A description based on the effective Ising model implies that the frustrated Heisenberg triangular bilayer with the ferromagnetic interdimer coupling displays in a zero-temperature magnetization curve discontinuous magnetization jump, which is reduced upon increasing of temperature until a continuous field-driven phase transition from the Ising universality class is reached at a certain critical temperature. The frustrated Heisenberg triangular bilayer with the antiferromagnetic interdimer coupling contrarily exhibits multistep magnetization curve with intermediate plateaus at 13\frac{1}{3}31​ and 23\frac{2}{3}32​ of the saturation magnetization, whereas discontinuous magnetization jumps observable at zero temperature change to continuous field-driven phase transitions from the universality class of three-state Potts model at sufficiently low temperatures. Exact results and Monte Carlo simulations of the effective Ising model are confronted with full exact diagonalization data for the Heisenberg triangular bilayer in order to corroborate these findings.
The ground state, entropy, and magnetic Grüneisen parameter of the antiferromagnetic spin-1/2 Ising-Heisenberg model on a double sawtooth ladder are rigorously investigated using the classical transfer-matrix technique. The model includes the XXZ interaction between the interstitial Heisenberg dimers, the Ising coupling between nearest-neighbor spins of the legs and rungs, and additional cyclic four-spin Ising term in each square plaquette. For a particular value of the cyclic four-spin exchange, we found in the ground-state phase diagram of the Ising-Heisenberg ladder a quadruple point, at which four different ground states coexist together. During an adiabatic demagnetization process, a fast cooling accompanied with an enhanced magnetocaloric effect can be detected near this quadruple point. The ground-state phase diagram of the Ising-Heisenberg ladder is confronted with the zero-temperature magnetization process of the purely quantum Heisenberg ladder, which is calculated by using exact diagonalization based on the Lanczos algorithm for a finite-size ladder of 24 spins and the density-matrix renormalization group simulations for a finite-size ladder with up to 96 spins. Some indications of the existence of intermediate magnetization plateaus in the magnetization process of the full Heisenberg model for a small but nonzero four-spin Ising coupling were found. The DMRG results reveal that the quantum Heisenberg double sawtooth ladder exhibits some quantum Luttinger spin-liquid phase regions that are absent in the Ising-Heisenberg counterpart model. Except this difference, the magnetic behavior of the full Heisenberg model is quite analogous to its simplified Ising-Heisenberg counterpart and, hence, may bring insight into the fully quantum Heisenberg model from rigorous results for the Ising-Heisenberg model.
Motivated by experimental progress in pressure and strain tuning of quantum materials, we examine the thermodynamic response of frustrated magnets to uniaxial strain. Specifically, we study Ising and Heisenberg models on spatially anisotropic triangular (and, for the Ising model, also kagome) lattices. We determine the entropy as a function of temperature and strain, and use it to compute the elastic Grüneisen ratio ηηη. The Ising models can be strain-tuned into and out of classical spin-liquid phases, and we show that ηηη can become arbitrarily large at low temperature TTT near the point of maximal frustration, a universal hallmark of an extensive ground-state entropy. In contrast, the spin-1/21/21/2 Heisenberg model is moderately frustrated and displays multiple T=0T=0T=0 phase transitions. These transitions dominate ηηη at low TTT while the intermediate-TTT behavior is similar to that of the Ising model. We discuss the extent to which the elastic Grüneisen ratio can be used to deduce the phase diagram, and we connect our results to recent experiments on triangular-lattice magnets.