The modern scientific method is critically dependent on precision measurements of physical parameters. A classic example is the measurement of the optical phase enabled by optical interferometry, where the error on the measured phase is conventionally bounded by the so-called Heisenberg limit. To achieve phase estimation at the Heisenberg limit, it has been common to consider protocols based on highly complex N00N states of light. However, despite decades of research and several experimental explorations, there has been no demonstration of deterministic phase estimation with N00N states reaching the Heisenberg limit or even surpassing the shot noise limit. Here we use a deterministic phase estimation scheme based on a source of Gaussian squeezed vacuum states and high-efficiency homodyne detection to obtain phase estimates with an extreme sensitivity that significantly surpasses the shot noise limit and even beats the conventional Heisenberg limit as well as the performance of a pure N00N state protocol. Using a high-efficiency setup with a total loss of about 11%, we achieve a Fisher information of 15.8(6) rad^{-2} per photon-a significant increase in performance compared to state of the art and beyond an ideal six photon N00N state scheme. This work represents an important achievement in quantum metrology, and it opens the door to future quantum sensing technologies for the interrogation of light-sensitive biological systems.
The modern scientific method is critically dependent on precision measurements of physical parameters. A classic example is the measurement of the optical phase enabled by optical interferometry, where the error on the measured phase is conventionally bounded by the so-called Heisenberg limit. To achieve phase estimation at the Heisenberg limit, it has been common to consider protocols based on highly complex N00N states of light. However, despite decades of research and several experimental explorations, there has been no demonstration of deterministic phase estimation with N00N states reaching the Heisenberg limit or even surpassing the shot noise limit. Here we use a deterministic phase estimation scheme based on a source of Gaussian squeezed vacuum states and high-efficiency homodyne detection to obtain phase estimates with an extreme sensitivity that significantly surpasses the shot noise limit and even beats the conventional Heisenberg limit as well as the performance of a pure N00N state protocol. Using a high-efficiency setup with a total loss of about 11%, we achieve a Fisher information of 15.8(6) rad^{-2} per photon-a significant increase in performance compared to state of the art and beyond an ideal six photon N00N state scheme. This work represents an important achievement in quantum metrology, and it opens the door to future quantum sensing technologies for the interrogation of light-sensitive biological systems.
Quantum metrology exploits quantum correlations to perform measurements with precision higher than can be achieved with classical approaches [1]. Photonic approaches promise transformative advances in the family of interferometric phase measurement techniques, a vital toolset used to precisely determine quantities including distance, velocity, acceleration and materials properties. Without quantum enhancement, the precision limit in optical phase sensing (i.e. the minimum uncertainty) is the shot noise limit (SNL): 1/sqrt(N) where N is the number of resources (e.g. photons) used. Entangled photons promise sensitivity surpassing the shot noise limit achievable with classical probes. The maximally phase-sensitive state is the NOON state [2], a path-entangled state of definite photon number N. Despite theoretical proposals stretching back decades [3], no measurement using such photonic (i.e. definite photon number) states has unconditionally surpassed the shot noise limit: by contrast, all such demonstrations employed postselection to discount photon loss in the source, interferometer or detectors. Here, we use the state of art single photon generation and detection technology to respectively make and measure a two-photon NOON state, and use it to perform unconditional phase sensing beyond the shot noise limit — that is, without artificially correcting for loss or any other source of imperfection [4]. We performed a two-photon NOON state polarisation interferometry measurement on a birefringent test phase. We use photons generated from a high-heralding-efficiency, high purity source of telecom-wavelength photon pairs [5], and we employ high efficiency superconducting photon detectors. Unlike previous experiments, our apparatus does not require postselection to achieve phase uncertainty below that achievable in an ideal, lossless classical interferometer. Our results show a clear violation (for a range of phases) of the stringent SNL Fisher-information bound, F_{SNL} = 2.09635, that takes into account the information in unrecorded trials arising from loss and higher order terms — making our demonstration unconditional. We also performed a direct phase sensing measurement and observed phase uncertainties more than 10 standard deviations below the SNL [4]. Our results enable quantum-enhanced phase measurements at low photon flux and open the door to the next generation of optical quantum metrology advances. References [1] V. Giovannetti, S. Lloyd, and L. Maccone, “Advances in quantum metrology,” Nat. Photon. 5, 222–229 (2011). [2] J. P. Dowling, “Quantum optical metrology–the lowdown on high-N00N states,” Contemp. Phys. 49, 125–143 (2008). [3] R. Demkowicz-Dobrzanski, M. Jarzyna, and J. Kołodynski, “Quantum limits in optical interferometry,” Prog. Opt. 60, 345–435 (2015). [4] S. Slussarenko, M. M.Weston, H. M. Chrzanowski, L. K. Shalm, V. B. Verma, S.W. Nam, and G. J. Pryde, “Unconditional violation of the shot noise limit in photonic quantum metrology,” Nat. Photon. 11, 700-703 (2017). [5] M. M. Weston, H. M. Chrzanowski, S. Wollmann, A. Boston, J. Ho, L. K. Shalm, V. B. Verma, M. S. Allman, S. W. Nam, R. B. Patel, S. Slussarenko, and G. J. Pryde, “Efficient and pure femtosecond-pulse length source of polarization-entangled photons,” Opt. Express 24, 10,869–10,879 (2016).
Quantum-enhanced interferometers utilize non-classical states of light in order to surpass the limitations imposed by classical physics on phase measurement sensitivity and resolution. We review key scientific developments in this growing field of research and derive fundamental metrology concepts, namely the Cram\'{e}r-Rao bound and the Fisher information, which are used to analyze the metrological performance of quantum states of light. We propose a supersensitive quantum interferometry protocol that can be amplified to the macroscopic realm (i.e. the mean number of photons of the probe state can reach approximately 100,000 photons) using contemporary techniques of spontaneous parametric down conversion. The parity measurement on the output field asymptotically saturates the quantum Cram\'{e}r-Rao bound, which scales like the Heisenberg limit. We uncover the role of photon statistics on phase sensitivity and rule out the necessity of mode entanglement for quantum-enhanced interferometry. Based on these insights we outline a practical metrology technique (independent of mode entanglement) that measures a phase delay of a single-mode anti-squeezing operation. This scheme can also be scaled macroscopically using contemporary techniques and is shown to significantly surpass the shot-noise limit (SNL) in the presence of realistic losses. Finally, the physical resources that enable quantum-enhanced interferometry is studied by analyzing the quantum Fisher information (QFI) using the first quantization and the second quantization formalisms of quantum mechanics. It is shown that increasing the intra-mode correlations of an interferometer (as quantified by the second order Glauber coherence function) can be conducive to attaining a quantum advantage in phase estimation; whereas, introducing mode entanglement can reduce phase sensitivity. Using the first quantization description, we derive a formula for the QFI that shows explicitly how the Heisenberg scaling term depends on particle entanglement.
The quantum statistical fluctuations of electromagnetic fields establish a limit, known as the shot-noise limit, on the sensitivity of optical measurements performed with classical technologies. However, quantum technologies are not constrained by this shot-noise limit. In this regard, the possibility of using every photon produced by quantum sources of light to estimate small physical parameters, beyond the shot-noise limit, constitutes one of the main goals of quantum optics. Here, we experimentally demonstrate a scalable protocol for quantum-enhanced optical phase estimation across a broad range of phases, with neither pre- nor post-selected measurements. This is achieved through the efficient design of a source of spontaneous parametric downconversion in combination with photon-number-resolving detection. The robustness of two-mode squeezed vacuum states against loss allows us to outperform schemes based on N00N states, in which the loss of a single photon is enough to remove all phase information from a quantum state. In contrast to other schemes that rely on N00N states or conditional measurements, the sensitivity of our technique could be improved through the generation and detection of high-order photon pairs. This unique feature of our protocol makes it scalable. Our work is important for quantum technologies that rely on multiphoton interference such as quantum imaging, boson sampling, and quantum networks.
The use of quantum resources can provide measurement precision beyond the shot noise limit (SNL). The task of ab initio optical phase measurement-the estimation of a completely unknown phase-has been experimentally demonstrated with precision beyond the SNL, and even scaling like the ultimate bound, the Heisenberg limit (HL), but with an overhead factor. However, existing approaches have not been able-even in principle-to achieve the best possible precision, saturating the HL exactly. Here we demonstrate a scheme to achieve true HL phase measurement, using a combination of three techniques: entanglement, multiple samplings of the phase shift, and adaptive measurement. Our experimental demonstration of the scheme, with photonic qubits and N = 3 photon-passes, achieves a precision that is within 4% of the HL, surpassing the best precision theoretically achievable with simpler techniques. This work represents a fundamental achievement of the ultimate limits of metrology, and the scheme can be extended to higher N and other physical systems.
We propose a high-precision phase estimation scheme in a hybrid interferometer by synergistically combining a Kerr nonlinear phase shifter and multi-photon subtraction operations. Using a coherent state and a vacuum state as input resources, we systematically evaluate the phase sensitivity via homodyne detection and analyze the quantum Fisher information as well as the quantum Cramér-Rao bound under both ideal and lossy conditions. Our results show that the joint integration of Kerr nonlinearity and multi-photon subtraction yields remarkable advantages over either technique used alone. The proposed scheme enables the phase sensitivity to surpass the standard quantum limit, exceed the conventional Heisenberg scaling (1/N), and approach the super-Heisenberg scaling (1/N2)-a direct consequence of Kerr nonlinearity. More precisely, the super-Heisenberg scaling $\propto $ 1/N2 is the ultimate precision limit permitted by the k=2 Kerr nonlinearity and does not violate the fundamental Heisenberg limit for linear phase accumulation. Even under moderate internal photon loss, the system maintains high precision and exhibits enhanced robustness to decoherence. The Kerr nonlinearity introduces an intensity-dependent phase shift proportional to the squared photon number, while multi-photon subtraction tailors non-Gaussian states to strengthen phase information extraction. Compared with existing schemes based on hybrid interferometers or SU(1,1) interferometers, our architecture achieves superior precision and stronger loss resilience. All components are experimentally accessible with current quantum optical technologies. This work provides a promising route for practical high-precision quantum metrology and quantum sensing.
The ultimate precision of phase estimation is limited by the Heisenberg scaling Δϕ0=K/N, where K∼1 is a numerical prefactor and N is the mean number of photons interacting with the phase shifting object(s). However, achieving this fundamental limit often comes at the cost of an extremely narrow high-sensitive range, rendering schemes impractical. We analyze the precision limits of phase measurements in single- and two-arm optical interferometers with input Gaussian states. We consider two detection methods: conventional homodyne measurement and non-Gaussian threshold detection that saturates the quantum Cramér-Rao bound. We characterize the performance by two complementary metrics: the peak sensitivity Δϕ0 and the width δϕ of the high-sensitivity range. We demonstrate that Heisenberg scaling is attainable in all configurations considered. However, we reveal that δϕ strongly depends on K. We derive an approximate analytic expression that describes this trade-off. We show also that the two-arm interferometer with antisymmetrically squeezed inputs exhibits exceptional performance, simultaneously achieving Heisenberg-limited sensitivity and a broad high-sensitivity range δϕ=π/2.