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arXiv:2110.15888 · PRX Quantum

Nonequilibrium Quantum Thermodynamics of a Particle Trapped in a Controllable Time-Varying Potential

Qiongyuan Wu, Luca Mancino, Matteo Carlesso, Mario Arnolfo Ciampini, Lorenzo Magrini, Nikolai Kiesel, Mauro Paternostro

Published Feb 8, 2022• 11 citations
arXivHTMLPDF

Abstract

Many advanced quantum techniques feature non-Gaussian dynamics, and the ability to manipulate the system in that domain is the next stage in many experiments.One example of meaningful non-Gaussian dynamics is that of a double-well potential.Here we study the dynamics of a levitated nanoparticle undergoing the transition from a harmonic potential to a double well in a realistic setting, subjected to both thermalization and localization.We characterize the dynamics of the nanoparticle from a thermodynamic point of view, investigating the dynamics with the Wehrl entropy production and its rates.Furthermore, we investigate coupling regimes where the the quantum effect and thermal effect are of the same magnitude, and look at suitable squeezing of the initial state that provides the maximum coherence.The effects and the competitions of the unitary and the dissipative parts onto the system are demonstrated.We quantify the requirements to relate our results to a bonafide experiment with the presence of the environment, and discuss the experimental interpretations of our results in the end.

DOI
10.1103/prxquantum.3.010322

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Many advanced quantum techniques feature non-Gaussian dynamics, and the ability to manipulate the system in that domain is the next stage in many experiments.One example of meaningful non-Gaussian dynamics is that of a double-well potential.Here we study the dynamics of a levitated nanoparticle undergoing the transition from a harmonic potential to a double well in a realistic setting, subjected to both thermalization and localization.We characterize the dynamics of the nanoparticle from a thermodynamic point of view, investigating the dynamics with the Wehrl entropy production and its rates.Furthermore, we investigate coupling regimes where the the quantum effect and thermal effect are of the same magnitude, and look at suitable squeezing of the initial state that provides the maximum coherence.The effects and the competitions of the unitary and the dissipative parts onto the system are demonstrated.We quantify the requirements to relate our results to a bonafide experiment with the presence of the environment, and discuss the experimental interpretations of our results in the end.
Non-equilibrium thermodynamics can provide strong advantages when compared to more standard equilibrium situations. Here, we present a general framework to study its application to concrete problems, which is valid also beyond the assumption of a Gaussian dynamics. We consider two different problems: 1) the dynamics of a levitated nanoparticle undergoing the transition from an harmonic to a double-well potential; 2) the transfer of a quantum state across a double-well potential through classical and quantum protocols. In both cases, we assume that the system undergoes to decoherence and thermalisation. In case 1), we construct a numerical approach to the problem and study the non-equilibrium thermodynamics of the system. In case 2), we introduce a new figure of merit to quantify the efficiency of a state-transfer protocol and apply it to quantum and classical versions of such protocols.
We propose to optimally control the harmonic potential of a levitated nanoparticle to quantum delocalize its center-of-mass motional state to a length scale orders of magnitude larger than the quantum zero-point motion. Using a bang-bang control of the harmonic potential, including the possibility of inverting it, the initial ground-state-cooled levitated nanoparticle coherently expands to large scales and then contracts to the initial state in a time-optimal way. We show that this fast loop protocol can be used to enhance force sensing as well as to dramatically boost the entangling rate of two weakly interacting nanoparticles. We parameterize the performance of the protocol, and therefore the macroscopic quantum regime that could be explored, as a function of displacement and frequency noise in the nanoparticle's center-of-mass motion. This noise analysis accounts for the sources of decoherence relevant to current experiments.
We develop the theory describing the quantum coupled dynamics of the center-of-mass motion of a nanoparticle and an ensemble of ions co-trapped in a dual-frequency linear Paul trap. We first derive analytical expressions for the motional frequencies and classical trajectories of both nanoparticle and ions. We then derive a quantum master equation for the ion-nanoparticle system and quantify the sympathetic cooling of the nanoparticle motion enabled by its Coulomb coupling to a continuously Doppler-cooled ion. We predict that motional cooling down to sub-kelvin temperatures is achievable in state-of-the-art experiments even in the absence of motional feedback and in the presence of micromotion. We then extend our analysis to an ensemble of NNN ions, predicting a linear increase of the cooling rate as a function of NNN and motional cooling of the nanoparticle down to tenths of millikelvin in current experimental platforms. Our work establishes the theoretical toolbox needed to explore the ion-assisted preparation of non-Gaussian motional states of levitated nanoparticles.
Optomechanics with levitated nanoparticles is a promising way to combine very different types of quantum non-Gaussian aspects induced by continuous dynamics in a nonlinear or time-varying potential with the ones coming from discrete quantum elements in dynamics or measurement. First, it is necessary to prepare quantum non-Gaussian states using both methods. The nonlinear and time-varying potentials have been widely analyzed for this purpose. However, feasible preparation of provably quantum non-Gaussian states in a single mechanical mode using discrete photon detection has not been proposed yet for optical levitation. We explore pulsed optomechanical interactions combined with non-linear photon detection techniques to approach mechanical Fock states and confirm their quantum non-Gaussianity. We also predict the conditions under which the optomechanical interaction can induce multiple-phonon addition processes, which are relevant for nnn-phonon quantum non-Gaussianity. The practical applicability of quantum non-Gaussian states for sensing phase-randomized displacements is shown. Besides such applications, generating quantum non-Gaussian states of levitated nanoparticles can help to study fundamental questions of quantum thermodynamics, and macroscopic quantum effects.
The Brownian motion of a quantum particle in a harmonic confining potential and coupled to harmonic quantum thermal bath is exactly solvable. Though this system presents at high temperatures a pedagogic example to explain the laws of thermodynamics, it is shown that at low enough temperatures the stationary state is non-Gibbsian due to an entanglement with the bath. In physical terms, this happens when the cloud of bath modes around the particle starts to play a nontrivial role, namely, when the bath temperature T is smaller than the coupling energy. Indeed, equilibrium thermodynamics of the total system, particle plus bath, does not imply standard equilibrium thermodynamics for the particle itself at low T. Various formulations of the second law are found to be invalid at low T. First, the Clausius inequality can be violated, because heat can be extracted from the zero point energy of the cloud of bath modes. Second, when the width of the confining potential is suddenly changed, there occurs a relaxation to equilibrium during which the entropy production is partly negative. In this process the energy put on the particle does not relax monotonically, but oscillates between particle and bath, even in the limit of strong damping. Third, for nonadiabatic changes of system parameters the rate of energy dissipation can be negative, and, out of equilibrium, cyclic processes are possible which extract work from the bath. Conditions are put forward under which perpetuum mobility of the second kind, having one or several work extraction cycles, enter the realm of condensed matter physics. Fourth, it follows that the equivalence between different formulations of the second law (e.g., those by Clausius and Thomson) can be violated at low temperatures. These effects are the consequence of quantum entanglement in the presence of the slightly off-equilibrium nature of the thermal bath, and become important when the characteristic quantum time scale variant Planck's over 2pi /k(B)T is larger than or comparable to other time scales of the system. They show that there is no general consensus between standard thermodynamics and quantum mechanics. The known agreements occur only due to the weak coupling limit, which does not pertain to low temperatures. Experimental setups for testing the effects are discussed.
Abstract Optomechanics with levitated nanoparticles is a promising way to combine very different types of quantum non-Gaussian aspects induced by continuous dynamics in a nonlinear or time-varying potential with the ones coming from discrete quantum elements in dynamics or measurement. First, it is necessary to prepare quantum non-Gaussian states using both methods. The nonlinear and time-varying potentials have been widely analyzed for this purpose. However, feasible preparation of provably quantum non-Gaussian states in a single mechanical mode using discrete photon detection has not been proposed yet for optical levitation. We explore pulsed optomechanical interactions combined with non-linear photon detection techniques to approach mechanical Fock states and confirm their quantum non-Gaussianity. We also predict the conditions under which the optomechanical interaction can induce multiple-phonon addition processes, which are relevant for n-phonon quantum non-Gaussianity. The practical applicability of quantum non-Gaussian states for sensing phase-randomized displacements is shown. Besides such applications, generating quantum non-Gaussian states of levitated nanoparticles can help to study fundamental questions of quantum thermodynamics, and macroscopic quantum effects.