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arXiv:2110.15673 · Physical review. B./Physical review. B

Comparing the influence of Floquet dynamics in various Kitaev-Heisenberg materials

Pascal Strobel, Maria Daghofer

Published Feb 24, 2022• 14 citations
arXivHTMLPDF

Abstract

In this paper we examine the possibility of Floquet engineering in the three candidate Kitaev materials ${\mathrm{Na}}_{2}{\mathrm{IrO}}_{3}$, $\ensuremath{\alpha}\text{\ensuremath{-}}{\mathrm{Li}}_{2}{\mathrm{IrO}}_{3}$, and $\ensuremath{\alpha}\text{\ensuremath{-}}{\mathrm{RuCl}}_{3}$. We derive an effective Floquet Hamiltonian and give an approximation for heating processes arising from doublon holon propagation. This suggests that compounds with stronger Hund's rule coupling are less prone to heating. We then investigate the impact of light frequency and amplitude on magnetic interaction terms up to third nearest neighbor and find that third neighbor Heisenberg coupling ${J}_{3}$ is very susceptible to tuning by circularly polarized light. Finally, we discuss uses of linear polarized light in selectively tuning single bond directions.

DOI
10.1103/physrevb.105.085144

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In this paper we examine the possibility of Floquet engineering in the three candidate Kitaev materials Na2IrO3{\mathrm{Na}}_{2}{\mathrm{IrO}}_{3}Na2​IrO3​, \ensuremathα\ensuremath-Li2IrO3\ensuremath{\alpha}\text{\ensuremath{-}}{\mathrm{Li}}_{2}{\mathrm{IrO}}_{3}\ensuremathα\ensuremath-Li2​IrO3​, and \ensuremathα\ensuremath-RuCl3\ensuremath{\alpha}\text{\ensuremath{-}}{\mathrm{RuCl}}_{3}\ensuremathα\ensuremath-RuCl3​. We derive an effective Floquet Hamiltonian and give an approximation for heating processes arising from doublon holon propagation. This suggests that compounds with stronger Hund's rule coupling are less prone to heating. We then investigate the impact of light frequency and amplitude on magnetic interaction terms up to third nearest neighbor and find that third neighbor Heisenberg coupling J3{J}_{3}J3​ is very susceptible to tuning by circularly polarized light. Finally, we discuss uses of linear polarized light in selectively tuning single bond directions.
Magnetic exchange couplings can be tuned by coupling to periodic light, where the frequency and amplitude are typically varied: a process known as Floquet engineering. The polarization of the light is also important, and in this paper, we show how different polarizations, including several types of unpolarized light, can tune the exchange couplings in distinct ways. Using unpolarized light, for example, it is possible to tune the material without breaking either time-reversal or any lattice symmetries. To illustrate these effects generically, we consider single-band Hubbard models at half-filling on the honeycomb, square and triangular lattices. We derive the effective Heisenberg spin models to fourth order in perturbation theory for arbitrary fixed polarizations, and several types of unpolarized light that preserve time-reversal and lattice symmetries. Coupling these models to periodic light tunes first, second, and third neighbor exchange couplings, as well as ring exchange terms on the square and triangular lattices. Circularly polarized light induces chiral fields for the honeycomb and triangular lattices, which favors noncoplanar magnetism and potential chiral spin liquids. We discuss how to maximize the enhancement of the couplings without inducing heating.
Abstract In recent years, there has been an intense search for materials realizing the Kitaev quantum spin liquid model. A number of edge-shared compounds with strong spin-orbit coupling, such as RuCl3 and iridates, have been proposed to realize this model. Nevertheless, an effective spin Hamiltonian derived from the microscopic model relevant to these compounds generally contains terms that are antagonistic toward the quantum spin liquid. This is consistent with the fact that the zero magnetic field ground state of these materials is generally magnetically ordered. It is a pressing issue to identify protocols to drive the system to the limit of the Kitaev quantum spin model. In this work, we propose Floquet engineering of these Kitaev quantum magnets by coupling materials to a circularly polarized laser. We demonstrate that all the magnetic interactions can be tuned in situ by the amplitude and frequency of the laser, hence providing a route to stabilize the Kitaev quantum spin liquid phase.
We consider driving multiorbital Mott insulators using laser radiation. We derive general expressions for periodically driven spin-orbital models using time-dependent perturbation theory in the strong interaction limit. We show that the effective exchange interactions of the Floquet spin-orbital Hamiltonian are highly tunable via variations of the frequency, amplitude, and polarization of the laser. We also take the effect of a finite bandwidth of excitations into account and study possible heating effects. We further apply our formalism to orthorhombic titanates YTiO_{3} and LaTiO_{3} based on first-principles calculations, and we find that the spin exchange interactions in these compounds can be engineered to a large extent by tuning the frequency and electric-field amplitude of the laser.
Floquet engineering is a powerful tool that drives materials with periodic light. Traditionally, the light is monochromatic, with amplitude, frequency, and polarization varied. We introduce Floquet engineering via unpolarized light built from quasimonochromatic light and show how it can modify strongly correlated systems, while preserving the original symmetries. Different types of unpolarized light can realize different strongly correlated phases As an example, we treat insulating magnetic materials on a triangular lattice and show how unpolarized light can induce a Dirac spin liquid.
We show how second-order Floquet engineering can be employed to realize systems in which many-body localization coexists with topological properties in a driven system. This allows one to implement and dynamically control a symmetry protected topologically ordered qubit even at high energies, overcoming the roadblock that the respective states cannot be prepared as ground states of nearest-neighbor Hamiltonians. Floquet engineering-the idea that a periodically driven nonequilibrium system can effectively emulate the physics of a different Hamiltonian-is exploited to approximate an effective three-body interaction among spins in one dimension, using time-dependent two-body interactions only. In the effective system, emulated topology and disorder coexist, which provides an intriguing insight into the interplay of many-body localization that defies our standard understanding of thermodynamics and into the topological phases of matter, which are of fundamental and technological importance. We demonstrate explicitly how combining Floquet engineering, topology, and many-body localization allows one to harvest the advantages (time-dependent control, topological protection, and reduction of heating, respectively) of each of these subfields while protecting them from their disadvantages (heating, static control parameters, and strong disorder).
We study the interplay of magnetic order and superconductivity in the square-lattice Hubbard model under periodic driving with circularly polarized light. Formulating diagrammatic techniques based on the random-phase approximation in terms of Floquet Green's functions, allows us to analyze fluctuation-driven unconventional pairing for weak to moderate interactions. The interplay of repulsive interactions and photoassisted hopping of electrons gives rise to a rich magnetic phase diagram featuring an antiferromagnetic-to-ferromagnetic transition prior to a Floquet Lifshitz transition. Close to the antiferromagnetic transition, topological d + i d -wave superconductivity prevails in the phase diagram for a wide range of drive parameters. At intermediate- to high-frequency driving near the Floquet Lifshitz transition, superconducting orders are tuned from spin-singlet d -wave to spin-triplet p -wave character, providing an effective protocol for Floquet engineering topological superconductivity.