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arXiv:2110.06902 · PRX Quantum

Controlling Rydberg Excitations Using Ion-Core Transitions in Alkaline-Earth Atom-Tweezer Arrays

A. P. Burgers, Shuo Ma, Sam Saskin, Jack Wilson, Miguel A. Alarcón, Chris H. Greene, Jeff D. Thompson

Published May 6, 2022• 56 citations
arXivHTMLPDF

Abstract

Scalable local control over gate operations is an outstanding challenge in the field of quantum computing and programmable quantum simulation with Rydberg-atom arrays.One approach is to use a global field to excite atoms to the Rydberg state and tune individual atoms in and out of resonance via local light shifts.In this work, we point out that photon-scattering errors from light shifts can be significantly reduced if the light shift is applied to the Rydberg state instead of the ground state, which can be realized in Rydberg states of alkaline-earth atoms using optical transitions in the ion core.As a proof of concept, we experimentally demonstrate global control of Rydberg excitations in an Yb optical-tweezer array via light shifts induced by a laser tuned near the Yb + 6s → 6p 1/2 transition.We also perform detailed spectroscopy of the induced light shift and scattering rates of the 6sns 3 S 1 Rydberg states and reveal the existence of satellite lines where losses from autoionization are strongly suppressed.This work can be readily extended to implement local gate operations in Rydberg-atom arrays.

DOI
10.1103/prxquantum.3.020326

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Coherence time and gate fidelities in Rydberg atom quantum simulators and computers are fundamentally limited by the Rydberg state lifetime. Circular Rydberg states are highly promising candidates to overcome this limitation by orders of magnitude, as they can be effectively protected from decay due to their maximum angular momentum. We report the first realization of alkaline-earth circular Rydberg atoms trapped in optical tweezers, which provide unique and novel control possibilities due to the optically active ionic core. Specifically, we demonstrate creation of very high- n ( n = 79 ) circular states of Sr 88 . We measure lifetimes as long as 2.55 ms at room temperature, which are achieved via cavity-assisted suppression of black-body radiation. We show coherent control of a microwave qubit encoded in circular states of nearby manifolds, and characterize the qubit coherence time via Ramsey and spin-echo spectroscopy. Finally, circular-state tweezer trapping exploiting the Sr + core polarizability is quantified via measurements of the trap-induced light shift on the qubit. Our work opens routes for quantum simulations with circular Rydberg states of divalent atoms, exploiting the emergent toolbox associated with the optically active core ion. Published by the American Physical Society 2024

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Scalable local control over gate operations is an outstanding challenge in the field of quantum computing and programmable quantum simulation with Rydberg-atom arrays.One approach is to use a global field to excite atoms to the Rydberg state and tune individual atoms in and out of resonance via local light shifts.In this work, we point out that photon-scattering errors from light shifts can be significantly reduced if the light shift is applied to the Rydberg state instead of the ground state, which can be realized in Rydberg states of alkaline-earth atoms using optical transitions in the ion core.As a proof of concept, we experimentally demonstrate global control of Rydberg excitations in an Yb optical-tweezer array via light shifts induced by a laser tuned near the Yb + 6s → 6p 1/2 transition.We also perform detailed spectroscopy of the induced light shift and scattering rates of the 6sns 3 S 1 Rydberg states and reveal the existence of satellite lines where losses from autoionization are strongly suppressed.This work can be readily extended to implement local gate operations in Rydberg-atom arrays.
New experimental quantum simulation platforms have recently been implemented with divalent atoms trapped in optical tweezer arrays, with promising performance.The second valence electron also brings about new prospects through the so-called isolated core excitation (ICE).However, autoionization presents a strong limitation to this use.In this study, we propose and demonstrate a new approach to applying a sizable light shift to a Rydberg state with close-to-resonant ICE while avoiding autoionization.In particular, we investigate the ICE of ytterbium atoms in 1 S 0 Rydberg states.Spectroscopic studies of the induced autoionization and the light shift imparted to the Rydberg states are well accounted for with multichannel quantum defect theory.Such control over the inner electron without disturbing the Rydberg electron brings about a new tool for the targeted coherent manipulation of Rydberg states in quantum simulation or quantum computing experiments performed with alkaline-earth atoms.
Neutral atom qubits with Rydberg-mediated interactions are a leading platform for developing large-scale coherent quantum systems. In the majority of experiments to date, the Rydberg states are not trapped by the same potential that confines ground state atoms, resulting in atom loss and constraints on the achievable interaction time. In this Letter, we demonstrate that the Rydberg states of an alkaline earth atom, ytterbium, can be stably trapped by the same red-detuned optical tweezer that also confines the ground state, by leveraging the polarizability of the Yb^{+} ion core. Using the previously unobserved ^{3}S_{1} series, we demonstrate trapped Rydberg atom lifetimes exceeding 100 μs, and observe no evidence of auto- or photoionization from the trap light for these states. We measure a coherence time of T_{2}=59 μs between two Rydberg levels, exceeding the 28 μs lifetime of untrapped Rydberg atoms under the same conditions. These results are promising for extending the interaction time of Rydberg atom arrays for quantum simulation and computing, and are vital to capitalize on the extended Rydberg lifetimes in circular states or cryogenic environments.
Scalable quantum computers and quantum networks require the combination of quantum processing nodes with efficient light-matter interfaces to distribute quantum information in local or long-distance quantum networks. Neutral-atom arrays have both been coupled to Rydberg states to enable high-fidelity quantum gates in universal processing architectures, and to optical cavities to realize interfaces to photons. However, combining these two capabilities and coupling atom arrays to highly excited Rydberg states in the mode of an optical cavity has been an outstanding challenge. Here we present a novel cavity-coupled Rydberg array that achieves this long-standing goal. We prepare, detect, and control individual atoms in a scalable optical tweezer array, couple them strongly to the optical mode of a high-finesse optical cavity and excite them in a controlled way to Rydberg states. We show that high-cooperativity coupling to an optical cavity -- demonstrated via the dispersive shift of the resonance of the cavity in presence of the atoms -- and strong Rydberg interactions -- demonstrated via the collective enhancement of Rydberg coupling in the atomic array -- can be achieved in our setup at the same spatial location. Our presented experimental platform opens the path to several new directions, including the realization of quantum network nodes, quantum simulation of long-range interacting, open quantum systems and photonic-state engineering leveraging high-fidelity Rydberg control.
Neutral atom qubits with Rydberg-mediated interactions are a leading platform for developing large-scale coherent quantum systems. In the majority of experiments to date, the Rydberg states are not trapped by the same potential that confines ground state atoms, resulting in atom loss and constraints on the achievable interaction time. In this work, we demonstrate that the Rydberg states of an alkaline earth atom, ytterbium, can be stably trapped by the same red-detuned optical tweezer that also confines the ground state, by leveraging the polarizability of the Yb+^++ ion core. Using the previously unobserved \tripletS series, we demonstrate trapped Rydberg atom lifetimes exceeding 100 μ100\,μ100μs, and observe no evidence of auto- or photo-ionization from the trap light for these states. We measure a coherence time of T2=59T_2 = 59T2​=59 μμμs between two Rydberg levels, exceeding the 28 μμμs lifetime of untrapped Rydberg atoms under the same conditions. These results are promising for extending the interaction time of Rydberg atom arrays for quantum simulation and computing, and are vital to capitalize on the extended Rydberg lifetimes in circular states or cryogenic environments.
Integrating Rydberg-state control of atom-atom interactions with cavity control of atom-light interactions enables the combination of local entangling operations with photon-mediated long-range coupling, measurement, and communication. Such integration is challenging because electric fields generated by charges on cavity optics and by cavity-stabilizing actuators may disturb Rydberg-state coherence. Here, we couple a Rydberg tweezer array to a high-cooperativity optical cavity, suppressing the electric fields produced by cavity length actuation so that the residual field variation of about 3 mV/cm3~\mathrm{mV/cm}3 mV/cm rms does not limit Rydberg coherence. We demonstrate two capabilities that neither system provides alone. First, we use Purcell-enhanced fluorescence to read out atoms directly in the ground-Rydberg basis within 7.5 μs7.5~μ\mathrm{s}7.5 μs, well within the Rydberg-state lifetime, with ground- and Rydberg-state detection infidelities of 3%3\%3% and 5%5\%5%, respectively, and with low atom loss. Second, we use Rydberg-Rydberg interactions to control collective light-atom scattering into the cavity mode. Specifically, we drive blockaded Rabi oscillations between a state with two ground-state atoms, which scatter collectively with a superradiant or subradiant rate controlled by the atomic positions, and an entangled state with a single Rydberg excitation, which scatters like a single atom. These capabilities open routes toward networked Rydberg processors, mid-circuit measurements in analog quantum simulators, and many-body quantum optics with entangled emitters coupled collectively to light.
Coherence time and gate fidelities in Rydberg atom quantum simulators and computers are fundamentally limited by the Rydberg state lifetime. Circular Rydberg states are highly promising candidates to overcome this limitation by orders of magnitude, as they can be effectively protected from decay due to their maximum angular momentum. We report the first realization of alkaline-earth circular Rydberg atoms trapped in optical tweezers, which provide unique and novel control possibilities due to the optically active ionic core. Specifically, we demonstrate creation of very high- n ( n = 79 ) circular states of Sr 88 . We measure lifetimes as long as 2.55 ms at room temperature, which are achieved via cavity-assisted suppression of black-body radiation. We show coherent control of a microwave qubit encoded in circular states of nearby manifolds, and characterize the qubit coherence time via Ramsey and spin-echo spectroscopy. Finally, circular-state tweezer trapping exploiting the Sr + core polarizability is quantified via measurements of the trap-induced light shift on the qubit. Our work opens routes for quantum simulations with circular Rydberg states of divalent atoms, exploiting the emergent toolbox associated with the optically active core ion. Published by the American Physical Society 2024