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arXiv:2110.06229 · Physical review. B./Physical review. B

Thermal melting of a quantum electron solid in the presence of strong disorder: Anderson localization versus the Wigner crystal

DinhDuy Vu, S. Das Sarma

Published Sep 8, 2022• 6 citations
arXivHTMLPDF

Abstract

We consider the temperature-induced melting of a Wigner solid in one-dimensional (1D) and two-dimensional (2D) lattices of electrons interacting via the long-range Coulomb interaction in the presence of strong disorder arising from charged impurities in the system. The system simulates semiconductor-based 2D electron layers where Wigner crystallization is often claimed to be observed experimentally. Using exact diagonalization and utilizing the inverse participation ratio as well as conductance to distinguish between the localized insulating solid phase and the extended metallic liquid phase, we find that the effective melting temperature may be strongly enhanced by disorder since the disordered crystal typically could be in a localized glassy state incorporating the combined nonperturbative physics of both Anderson localization and Wigner crystallization. This disorder-induced enhancement of the melting temperature may explain why experiments often manage to observe insulating disorder-pinned Wigner solids in spite of the experimental temperature being decisively far above the theoretical melting temperature of the pristine Wigner crystal phase in many cases.

DOI
10.1103/physrevb.106.l121103

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We consider the temperature-induced melting of a Wigner solid in one-dimensional (1D) and two-dimensional (2D) lattices of electrons interacting via the long-range Coulomb interaction in the presence of strong disorder arising from charged impurities in the system. The system simulates semiconductor-based 2D electron layers where Wigner crystallization is often claimed to be observed experimentally. Using exact diagonalization and utilizing the inverse participation ratio as well as conductance to distinguish between the localized insulating solid phase and the extended metallic liquid phase, we find that the effective melting temperature may be strongly enhanced by disorder since the disordered crystal typically could be in a localized glassy state incorporating the combined nonperturbative physics of both Anderson localization and Wigner crystallization. This disorder-induced enhancement of the melting temperature may explain why experiments often manage to observe insulating disorder-pinned Wigner solids in spite of the experimental temperature being decisively far above the theoretical melting temperature of the pristine Wigner crystal phase in many cases.
Critically analyzing recent STM and transport experiments [Z. Ge, et al, arXiv:2510.12009] on 2D electron systems in the presence of random quenched impurities, we argue that the resulting low-density putative "solid" phase reported experimentally is better described as an Anderson solid with the carriers randomly spatially localized by impurities than as a Wigner solid where the carriers form a crystal due to an interaction-induced spontaneous breaking of the translational symmetry. In strongly disordered systems, the resulting solid is amorphous, which is adiabatically connected to the infinite disorder Anderson fixed point rather than the zero disorder Wigner crystal fixed point.
We consider an electron system under conditions of strong Anderson localization, taking into account interelectron long-range Coulomb repulsion. We have established that with the electron density going to zero the Coulomb interaction brings the arrangement of the Anderson localized electrons closer and closer to an ideal (Wigner) crystal lattice, provided the temperature is sufficiently low and the dimension of the system is > 1. The ordering occurs despite the fact that a random spread of the energy levels of the localized one-electron states, exceeding the mean Coulomb energy per electron, renders it impossible the electrons to be self-localized due to their mutual Coulomb repulsion This differs principally the Coulomb ordered Anderson localized electron system (COALES) from Wigner crystal, Wigner glass, and any other ordered electron or hole system that results from the Coulomb self-localization of electrons/holes. The residual disorder inherent to COALES is found to bring about a multi-valley ground-state degeneration akin to that in spin glass. With the electron density increasing, COALES is revealed to turn into Wigner glass or a glassy state of a Fermi-glass type depending on the width of the random spread of the electron levels.
(received; accepted) PACS. 71.10-w – Theories and models for many-electron systems. PACS. 71.27+a – Strongly correlated electron systems. PACS. 73.20.Qt – Electron solids. Abstract. – We consider three spinless fermions free to move on 2d square lattice with periodic boundary conditions and interacting via a U/r Coulomb repulsion. When the Coulomb energy to kinetic energy ratio rs is large, a rigid Wigner molecule is formed. As rs decreases, we show that melting proceeds via an intermediate regime where a floppy two particle molecule coexists with a partially delocalized particle. A simple ansatz is given to describe the ground state of this mesoscopic solid-liquid regime. Ordered arrays of charged particles with long range Coulomb repulsion have been a continuous subject of interest in various branches of physics, including colloidal suspensions, ion rings, atomic-ion Wigner crystals, quantum computers, biophysics, plasmas, electrons deposited on liquid Helium surfaces, charges created in semiconductor or organic field effect devices. These
One-dimensional electron systems interacting with long-range Coulomb forces (quantum wires) show a Wigner crystal structure. We investigate in this paper the transport properties of such a Wigner crystal in the presence of impurities. Contrary to what happens when only short-range interactions are included, the system is dominated by 4kF{\mathit{k}}_{\mathit{F}}kF​ scattering on the impurities. There are two important length scales in such a problem: one is the pinning length above which the (quasi-)long-range order of the Wigner crystal is destroyed by disorder. The other length, ${\ensuremath{\xi}}_{\mathrm{cr}}$, is the length below which Coulomb interactions are not important and the system is behaving as a standard Luttinger liquid with short-range interactions. We obtain the frequency and temperature dependence of the conductivity. We show that such a system is very similar to a classical charge density wave pinned by impurities, but with important differences due to quantum fluctuations and long-range Coulomb interactions. Finally, we discuss our results in comparison with experimental systems.
For intermediate Coulomb energy to Fermi energy ratios rsr_srs​, spinless fermions in a two-dimensional random potential form a new quantum phase, different from the Fermi glass (weakly interacting Anderson localized states) and the Wigner crystal (regular array of charges pinned by the disorder). The intermediate phase is characterized by an ordered flow of persistent currents with a typical value decreasing with excitation energy. Extending finite size scaling analysis to the many body ground state, we find that electron-electron interactions can drive the Fermi glass towards an intermediate metallic phase (Coulomb metal).
Disorder or sufficiently strong interactions can render a metallic state unstable, causing it to turn into an insulating one. Despite the fact that the interplay of these two routes to a vanishing conductivity has been a central research topic, a unifying picture has not emerged so far. Here, we establish that the two-dimensional Falicov-Kimball model, one of the simplest lattice models of strong electron correlation, does allow for the study of this interplay. In particular, we show that this model at particle-hole symmetry possesses three distinct thermodynamic insulating phases and exhibits Anderson localization. The previously reported metallic phase is identified as a finite-size feature due to the presence of weak localization. We characterize these phases by their electronic density of states, staggered occupation, conductivity, and the generalized inverse participation ratio. The implications of our findings for other strongly correlated systems are discussed.