These notes summarize lectures given at the 2019 Les Houches summer school on Quantum Information Machines. They describe and review an application of quantum metrology concepts to searches for ultralight dark matter. In particular, for ultralight dark matter that couples as a weak classical force to a laboratory harmonic oscillator, quantum squeezing benefits experiments in which the mass of the dark matter particle is unknown. This benefit is present even if the oscillatory dark matter signal is much more coherent than the harmonic oscillator that it couples to, as is the case for microwave frequency searches for dark matter axion particles.
These notes summarize lectures given at the 2019 Les Houches summer school on Quantum Information Machines. They describe and review an application of quantum metrology concepts to searches for ultralight dark matter. In particular, for ultralight dark matter that couples as a weak classical force to a laboratory harmonic oscillator, quantum squeezing benefits experiments in which the mass of the dark matter particle is unknown. This benefit is present even if the oscillatory dark matter signal is much more coherent than the harmonic oscillator that it couples to, as is the case for microwave frequency searches for dark matter axion particles.
Precision molecular spectroscopy provides a sensitive detection method for ultralight bosonic dark matter. This wavelike dark matter couples to the Standard Model fundamental constants, modulates the frequencies of the molecular transitions and of the resonances of the optical cavities, and brings oscillations in the laser absorption spectroscopy signals. Spectroscopy experiments with differential detection methods approach the fundamental limitation imposed by quantum noise in photodetection. The use of squeezed light in spectroscopy is addressed here to circumvent this limitation. An experimental setup is proposed for the interrogation of an acetylene transition at 1542 nm with a bright squeezed light field and a homodyne detection scheme. This approach enables measurements using the squeezed quadrature, ensures broadband sensitivity, demonstrates robustness to moderate losses, and provides improved constraints for the couplings of the ultralight bosonic dark matter to the Standard Model in the radiofrequency range.
One of the areas of research of the Superconducting Quantum Systems and Materials (SQMS) center is the application of quantum sensing to fundamental physics searches, demonstrating that quantum sensors can greatly improve the sensitivity of experiments searching for Beyond the Standard Model (BSM) physics, or performing high-precision measurements. Theorists have developed many ideas for BSM physics that would result in interactions that can in principle be detected, but with signals small enough that they haven t been observed yet. In this field, the capability to lower the detector s thermal noise to few or dozens of mK, and to use QIS technologies such as Josephson Parametric Amplifiers and photon counters (in-situ or itinerant) enable us to reach unprecedented sensitivities and faster scan rates. Here is presented an overview of the quantum sensing efforts at SQMS [1], focusing on theoretical advancements and experimental searches for Dark Sector particles (as dark matter candidates and not), gravitational waves, and precision measurements. The experiments conducted, or under preparation, include axion dark matter (DM) [2, 3], dark photon DM searches [4,5], light-shining-through-wall experiments [6], cavity-based searches for high frequency gravitational waves [7], and measurements of the electron magnetic moment [8]. [1] Berlin, A., et al. "Searches for new particles, dark matter, and gravitational waves with SRF cavities." arXiv preprint arXiv:2203.12714 (2022). [2] Giaccone, B., et al. "Design of axion and axion dark matter searches based on ultra high Q SRF cavities." arXiv preprint arXiv:2207.11346 (2022). [3] Braggio, C., et al. "Quantum-enhanced sensing of axion dark matter with a transmon-based single microwave photon counter." arXiv preprint arXiv:2403.02321 (2024). [4] Fan, X., et al. "One-electron quantum cyclotron as a milli-eV dark-photon detector." Physical review letters 129.26 (2022): 261801. [5] Cervantes, R., et al. "Deepest sensitivity to wavelike dark photon dark matter with superconducting radio frequency cavities." Physical Review D 110.4 (2024): 043022. [6] Romanenko, A., et al. "Search for dark photons with superconducting radio frequency cavities." Physical review letters 130.26 (2023): 261801. [7] Berlin, A., et al. "Electromagnetic cavities as mechanical bars for gravitational waves." Physical Review D 108.8 (2023): 084058. [8] Fan, X., et al. "Measurement of the electron magnetic moment." Physical review letters 130.7 (2023): 071801.
Quantum metrology has recently emerged as a powerful approach for dark matter (DM) searches, particularly using nonclassical bosonic states in microwave cavities that are sensitive to weak signals. Nonclassical cat states-macroscopic superpositions of coherent states featuring sub-Planck interference structures-offer promising advantages for high-precision measurements. However, their practical utility in DM search remains unexplored. Here, we report the first experimental application of four-component cat states within a high-quality superconducting microwave cavity to search for dark photons, a potential DM candidate. We demonstrate an 8.1-fold enhancement in the signal photon rate and constrain the dark photon kinetic mixing angle to an unprecedented ε<7.32×10^{-16} near 6.44 GHz (26.6 μeV). By employing a parametric sideband drive to actively tune the cavity frequency, we achieve dark photon searches and background subtraction across multiple frequency bins, yielding a sensitivity at the 10^{-16} level within a 100 kHz bandwidth. Our cat-assisted DM search and frequency-scanning techniques demonstrate substantial improvements over previous results, promising potential implications in quantum-enhanced searches for new physics.
Dark matter is an enduring mystery in our quest to understand the fundamental constituents of our universe. Low mass bosons, such the axion or hidden photon, are compelling dark matter candidates. We leverage their potential interactions with electromagnetic fields, whereby the dark matter (of unknown mass) on rare occasion converts into a single photon, to devise a method of detecting these candidates. Current dark matter searches operating at microwave frequencies use a resonant cavity to coherently accumulate the field sourced by the dark matter and a near standard quantum limited (SQL) linear amplifier to read out the cavity signal. To further increase sensitivity to the dark matter signal and enable future searches, sub-SQL detection techniques are required. In this thesis, I report the development of a novel microwave photon counting technique and a new exclusion limit on hidden photon dark matter. We operate a superconducting qubit to make repeated quantum non-demolition measurements of cavity photons and apply a hidden Markov model analysis to reduce the noise to 15.7 dB below the quantum limit, with overall detector performance limited by a residual background of real photons. With the present device, we perform a hidden photon search and constrain the kinetic mixing angle to less than 1.68 X 10^{-15} in a band around 6.011 GHz (24.86 micro-eV) with an integration time of 8.33 s. This demonstrated noise reduction technique enables future dark matter searches to be sped up by a factor of 1300. By coupling a qubit to an arbitrary quantum sensor, more general sub-SQL metrology is possible with the techniques presented in this work.
Many experiments that interrogate fundamental theories require detectors whose sensitivities are limited by the laws of quantum mechanics.In cavity-based searches for axionic dark matter, vacuum fluctuations in the two quadratures of the cavity electromagnetic field limit the sensitivity to an axion-induced field.In an apparatus designed to partially mimic existing axion detectors, we demonstrate experimentally that such quantum limits can be overcome through the use of squeezed states.By preparing a microwave cavity in a squeezed state and measuring just the squeezed quadrature, we enhance the spectral scan rate by a factor of 2.12 Æ 0.08.This enhancement is in excellent quantitative agreement with a theoretical model accounting for both imperfect squeezing and measurement.
The hypothetical axion particle (of unknown mass) is a leading candidate for dark matter (DM).Many experiments search for axions with microwave cavities, where an axion may convert into a cavity photon, leading to a feeble excess in the output power of the cavity.Recent work [Backes et al., Nature 590, 238 (2021)] has demonstrated that injecting squeezed vacuum into the cavity can substantially accelerate the axion search.Here, we go beyond and provide a theoretical framework to leverage the benefits of quantum squeezing in a network setting consisting of many sensor cavities.By forming a local sensor network, the signals among the cavities can be combined coherently to boost the axion search.Furthermore, injecting multipartite entanglement across the cavities-generated by splitting a squeezed vacuum-enables a global noise reduction.We explore the performance advantage of such a local, entangled sensor network, which enjoys both coherence between the axion signals and entanglement between the sensors.Our analyses are pertinent to next-generation DM-axion searches aiming to leverage a network of sensors and quantum resources in an optimal way.Finally, we assess the possibility of using a more exotic quantum state, the Gottesman-Kitaev-Preskill (GKP) state.Despite a constant-factor improvement in the scan time relative to a single-mode squeezed state in the ideal case, the advantage of employing a GKP state disappears when a practical measurement scheme is considered.