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arXiv:2110.02650 · npj Quantum Information

A chiral one-dimensional atom using a quantum dot in an open microcavity

Nadia O. Antoniadis, Natasha Tomm, Tomasz Jakubczyk, Rüdiger Schott, Sascha R. Valentin, Andreas Dirk Wieck, Arne Ludwig, Richard John Warburton, Alisa Javadi

Published Mar 11, 2022• 23 citations

Abstract

Abstract In a chiral one-dimensional atom, a photon propagating in one direction interacts with the atom; a photon propagating in the other direction does not. Chiral quantum optics has applications in creating nanoscopic single-photon routers, circulators, phase-shifters, and two-photon gates. Here, we implement chiral quantum optics using a low-noise quantum dot in an open microcavity. We demonstrate the non-reciprocal absorption of single photons, a single-photon diode. The non-reciprocity, the ratio of the transmission in the forward-direction to the transmission in the reverse direction, is as high as 10.7 dB. This is achieved by tuning the photon-emitter coupling in situ to the optimal operating condition (β = 0.5). Proof that the non-reciprocity arises from a single quantum emitter lies in the photon statistics—ultralow-power laser light propagating in the diode’s reverse direction results in a highly bunched output (g(2)(0) = 101), showing that the single-photon component is largely removed.

DOI: 10.1038/s41534-022-00545-z

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We investigated the transmission of single and two photons in a one-dimensional waveguide that is coupled with a Kerr micro-ring resonator and a polarized quantum emitter. In both cases, a phase shift occurs, and the non-reciprocal behavior of the system is attributed to the unbalanced coupling between the quantum emitter and the resonator. Our analytical solutions and numerical simulations demonstrate that the nonlinear resonator scattering causes the energy redistribution of the two photons through the bound state. When the system is in the two-photon resonance state, the polarization of the correlated two photons is locked to their propagation direction, leading to non-reciprocity. As a result, our configuration can act as an optical diode.

We report strongly nonreciprocal behavior for quantum dot exciton spins coupled to nanophotonic waveguides under resonant laser excitation. A clear dependence of the transmission spectrum on the propagation direction is found for a chirally coupled quantum dot, with spin up and spin down exciton spins coupling to the left and right propagation directions, respectively. The reflection signal shows an opposite trend to the transmission, which a numerical model indicates is due to direction-selective saturation of the quantum dot. The chiral spin-photon interface we demonstrate breaks reciprocity of the system and opens the way to spin-based quantum optical components such as optical diodes and circulators in a chip-based solid-state environment.

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We study the coherent transport of one or two photons in a one-dimensional waveguide chirally coupled to a nonlinear resonator. Analytic solutions of the one-photon and two-photon scattering is derived. Although the resonator acts as a non-reciprocal phase shifter, light transmission is reciprocal at one-photon level. However, the forward and reverse transmitted probabilities for two photons incident from either the left side or the right side of the nonlinear resonator are nonreciprocal due to the energy redistribution of the two-photon bound state. Hence, the nonlinear resonator acts as an optical diode at two-photon level.