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arXiv:2109.13571 · Physical Review Research

SU(2) hyper-clocks: Quantum engineering of spinor interferences for time and frequency metrology

T. Zanon-Willette, David Wilkowski, R. Lefèvre, А. В. Тайченачев, Valeriy I. Yudin

Published May 13, 2022• 2 citations
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Abstract

In 1949, Ramsey's method [Phys. Rev. 76, 996 (1949)] of separated oscillating fields was elaborated boosting over many decades metrological performances of atomic clocks and becoming the standard technique for very high-precision spectroscopic measurements. A generalization of this interferometric method is presented replacing the two single coherent excitations by arbitrary composite laser pulses. The rotation of the state vector of a two-level system under the effect of a single pulse is described using the Pauli matrices basis of the SU(2) group. It is then generalized to multiple excitation pulses by a recursive Euler-Rodrigues-Gibbs algorithm describing a composition of rotations with different rotation axes. A general analytical formula for the phase shift associated with the clock's interferometric signal is derived. As illustrations, hyper-clocks based on three-pulse and five-pulse interrogation protocols are studied and shown to exhibit nonlinear cubic and quintic sensitivities to residual probe-induced light shifts. The presented formalism is well suited to optimize composite phase shifts produced by tailored quantum algorithms in order to design a new generation of optical frequency standards and robust engineering control of atomic interferences in atomic, molecular, and optical physics with cold matter and antimatter.

DOI
10.1103/physrevresearch.4.023117

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In 1949, Ramsey's method [Phys. Rev. 76, 996 (1949)] of separated oscillating fields was elaborated boosting over many decades metrological performances of atomic clocks and becoming the standard technique for very high-precision spectroscopic measurements. A generalization of this interferometric method is presented replacing the two single coherent excitations by arbitrary composite laser pulses. The rotation of the state vector of a two-level system under the effect of a single pulse is described using the Pauli matrices basis of the SU(2) group. It is then generalized to multiple excitation pulses by a recursive Euler-Rodrigues-Gibbs algorithm describing a composition of rotations with different rotation axes. A general analytical formula for the phase shift associated with the clock's interferometric signal is derived. As illustrations, hyper-clocks based on three-pulse and five-pulse interrogation protocols are studied and shown to exhibit nonlinear cubic and quintic sensitivities to residual probe-induced light shifts. The presented formalism is well suited to optimize composite phase shifts produced by tailored quantum algorithms in order to design a new generation of optical frequency standards and robust engineering control of atomic interferences in atomic, molecular, and optical physics with cold matter and antimatter.
In 1949, Ramsey's method of separated oscillating fields was proposed boosting over many decades metrological performances of atomic clocks and becoming the standard technique for very high precision spectroscopic measurements. A full generalization of this interferometric method is presented replacing the two single coherent excitations by arbitrary composite laser pulses. The rotation of the state vector of a two-level system under the effect of a single pulse is described using the Pauli-spin matrices basis of the SU(2) group. It is then generalized to multiple excitation pulses by a recursive Euler-Rodrigues-Gibbs algorithm describing a composition of rotations with different rotation axes. A general analytical formula for the phase-shift associated with the clock's interferometric signal is derived. As illustrations, hyper-clocks based on three-pulse and five-pulse interrogation protocols are studied and shown to exhibit nonlinear cubic and quintic sensitivities to residual probe-induced light-shifts. The presented formalism is well suited to conceive programmable composite phase-shifts produced by tailored quantum algorithms in order to design a new generation of optical frequency standards, robust qubit and qudit rotations for quantum computation and address new challenges in AMO physics with ultra-high precision laser spectroscopy on cold matter and anti-matter.
A new class of atomic interferences using ultranarrow optical transitions are pushing quantum engineering control to a very high level of precision for the next generation of sensors and quantum gate operations. In such context, we propose a new quantum engineering approach to Ramsey-Bord\'e interferometry introducing multiple composite laser pulses with tailored pulse duration, Rabi field amplitude, frequency detuning and laser phase step. We explore quantum metrology with hyper-Ramsey and hyper-Hahn-Ramsey clocks below the ${10}^{\ensuremath{-}18}$ level of fractional accuracy by fine-tuning control of light excitation parameters leading to spinor interferences protected against light-shift coupled to laser-probe field variation. We review cooperative composite pulse protocols to generate robust Ramsey-Bord\'e, Mach-Zehnder, and double-loop atomic sensors shielded against measurement distortion related to Doppler and light shifts coupled to pulse area errors. Fault-tolerant autobalanced hyperinterferometers are introduced eliminating several technical laser pulse defects that can occur during the entire probing interrogation protocol. Quantum sensors with composite pulses and ultracold atomic sources should offer a new level of high accuracy in the detection of acceleration and rotation inducing phase shifts, a strong improvement in tests of fundamental physics with hyperclocks while paving the way to a new conception of atomic interferometers tracking space-time gravitational waves with very high sensitivity.
Probing an atomic resonance without disturbing it is an ubiquitous issue in physics. This problem is critical in high-accuracy spectroscopy or for the next generation of atomic optical clocks. Ultra-high resolution frequency metrology requires sophisticated interrogation schemes and robust protocols handling pulse length errors and residual frequency detuning offsets. This review reports recent progress and perspective in such schemes, using sequences of composite laser-pulses tailored in pulse duration, frequency and phase, inspired by NMR techniques and quantum information processing. After a short presentation of Rabi technique and NMR-like composite pulses allowing efficient compensation of electromagnetic field perturbations to achieve robust population transfers, composite laser-pulses are investigated within Ramsey's method of separated oscillating fields in order to generate non-linear compensation of probe-induced frequency shifts. Laser-pulses protocols such as hyper-Ramsey, modified hyper-Ramsey, generalized hyper-Ramsey and hybrid schemes as auto-balanced Ramsey spectroscopy are reviewed. These techniques provide excellent protection against both probe induced light-shift perturbations and laser intensity variations. More sophisticated schemes generating synthetic frequency-shifts are presented. They allow to reduce or completely eliminate imperfect correction of probe-induced frequency-shifts even in presence of decoherence due to the laser line-width. Finally, two universal protocols are presented which provide complete elimination of probe-induced frequency shifts in the general case where both decoherence and relaxation dissipation effects are present by using exact analytic expressions for phase-shifts and the clock frequency detuning. These techniques might be applied to atomic, molecular and nuclear frequency metrology, Ramsey-type mass spectrometry as well as precision spectroscopy.
A new generation of atomic sensors using ultra-narrow optical clock transitions and composite pulses are pushing quantum engineering control to a very high level of precision for applied and fundamental physics. Here, we propose a new version of Ramsey-Bord\'e interferometry introducing arbitrary composite laser pulses with tailored pulse duration, Rabi field, detuning and phase-steps. We explore quantum metrology below the 10−1810^{-18}10−18 level of fractional accuracy by a fine tuning control of light excitation parameters protecting ultra-narrow optical clock transitions against residual light-shift coupled to laser-probe field fluctuation. We present, for the first time, new developments for robust hyper Ramsey-Bord\'e and Mach-Zehnder interferometers, where we protect wavepacket interferences against distortion on frequency or phase measurement related to residual Doppler effects and light-shifts coupled to a pulse area error. Quantum matter-wave sensors with composite pulses and ultra-cold sources will offer detection of inertial effects inducing phase-shifts with better accuracy, to generate hyper-robust optical clocks and improving tests of fundamental physics, to realize a new class of atomic interferometers tracking space-time gravitational waves with a very high sensitivity.
The generalised hyper-Ramsey resonance formula originally published in Phys. Rev. A , 92, 023416 (2015) is derived using a Cayley – Klein spinor parametrisation. The shape of the interferometric resonance and the associated composite phase shift are reformulated including all individual laser pulse parameters. Potential robustness of signal contrast and phase-shift of the wave-function fringe pattern can now be arbitrarily explored tracking any shape distortion due to systematic effects from the probe laser. An exact and simple analytical expression describing Ramsey’s method of separated composite oscillating laser fields with quantum state control allows us to accurately simulate all recent clock interrogation protocols under various pulse defects.
Optical clock interrogation protocols, based on laser-pulse spectroscopy, are suffering from probe-induced frequency shifts and their variations induced by laser power. Original Hyper-Ramsey probing scheme, which was proposed to alleviate those issues, does not fully eliminate the shift, especially when decoherence and relaxation by spontaneous emission or collisions are present. We propose to solve the fundamental problem of frequency shifts induced by laser probe by deriving the exact canonical form of a multi-pulse generalized Hyper-Ramsey (GHR) resonance, including decoherence and relaxation. We present a universal interrogation protocol based on composite laser-pulses spectroscopy with phase-modulation eliminating probe-induced frequency shifts at all orders in presence of various dissipative processes. Unlike frequency shifts extrapolation-based methods, a universal interrogation protocol based on ±π/4\pm\pi/4±π/4 and ±3π/4\pm3\pi/4±3π/4 phase-modulated resonances is proposed which does not compromise the stability of the optical clock while maintaining an ultra-robust error signal gradient in presence of substantial uncompensated ac Stark-shifts. Such a scheme can be implemented in two flavours: either by inverting clock state initialization or by pulse order reversal even without a perfect quantum state initialization. This universal interrogation protocol can be applied to atomic, molecular and nuclear frequency metrology, mass spectrometry and to the field of precision spectroscopy. It might be designed using magic-wave induced transitions, two-photon excitation and magnetically-induced spectroscopy or it might even be implemented with quantum logic gate circuit and qubit entanglement.