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arXiv:2109.08058 · Entropy

Quantum Probes for the Characterization of Nonlinear Media

Alessandro Candeloro, Sholeh Razavian, Matteo Piccolini, Berihu Teklu, Stefano Olivares, Matteo G. A. Paris

Published Oct 16, 2021• 50 citations
arXivHTMLPDF

Abstract

Active optical media leading to interaction Hamiltonians of the form H=λ˜(a+a†)ζ represent a crucial resource for quantum optical technology. In this paper, we address the characterization of those nonlinear media using quantum probes, as opposed to semiclassical ones. In particular, we investigate how squeezed probes may improve individual and joint estimation of the nonlinear coupling λ˜ and of the nonlinearity order ζ. Upon using tools from quantum estimation, we show that: (i) the two parameters are compatible, i.e., the may be jointly estimated without additional quantum noise; (ii) the use of squeezed probes improves precision at fixed overall energy of the probe; (iii) for low energy probes, squeezed vacuum represent the most convenient choice, whereas for increasing energy an optimal squeezing fraction may be determined; (iv) using optimized quantum probes, the scaling of the corresponding precision with energy improves, both for individual and joint estimation of the two parameters, compared to semiclassical coherent probes. We conclude that quantum probes represent a resource to enhance precision in the characterization of nonlinear media, and foresee potential applications with current technology.

DOI
10.3390/e23101353

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Active optical media leading to interaction Hamiltonians of the form H=λ˜(a+a†)ζ represent a crucial resource for quantum optical technology. In this paper, we address the characterization of those nonlinear media using quantum probes, as opposed to semiclassical ones. In particular, we investigate how squeezed probes may improve individual and joint estimation of the nonlinear coupling λ˜ and of the nonlinearity order ζ. Upon using tools from quantum estimation, we show that: (i) the two parameters are compatible, i.e., the may be jointly estimated without additional quantum noise; (ii) the use of squeezed probes improves precision at fixed overall energy of the probe; (iii) for low energy probes, squeezed vacuum represent the most convenient choice, whereas for increasing energy an optimal squeezing fraction may be determined; (iv) using optimized quantum probes, the scaling of the corresponding precision with energy improves, both for individual and joint estimation of the two parameters, compared to semiclassical coherent probes. We conclude that quantum probes represent a resource to enhance precision in the characterization of nonlinear media, and foresee potential applications with current technology.
We address the precise characterization of coupling strength of nonlinear media in continuous-variable (CV) quantum systems using coherent and squeezed vacuum states as Gaussian probes, together with their photon-added and photon-subtracted counterparts as non-Gaussian probes. We consider three main classes of nonlinear Hamiltonians, namely quadrature nonlinearities, generalized squeezing and Kerr-type interactions. By analytically evaluating the quantum Fisher information (QFI), we compare the performance of Gaussian and non-Gaussian probes and assess the optimal probe based on the probe parameters, energy resource and non-Gaussianity. Our results are twofold as follows: first, for coherent-state family, the improvement provided by photon addition at fixed coherent amplitude originates mainly from the extra energy carried by the probe and does not provide a genuine metrological resource, since the same precision can be achieved by a Gaussian coherent-state signal of a larger energy, which can be more easily produced. Second, in contrast, photon addition and subtraction become effective resources when applied to already nonclassical states such as squeezed vacuum states. In this case, they lead to a significant enhancement of the QFI, particularly for higher-order interactions. Although Gaussian squeezed states remain optimal at equal energy constraint, photon-added and photon-subtracted squeezed states achieve comparable sensitives with significantly lower squeezing requirements. Since large squeezing level remains experimentally challenging, these non-Gaussian probes offer a practical route towards enhanced estimation of the nonlinear coupling strength within currently accessible squeezing regimes.
We address the characterization of dissipative bosonic channels and show that estimation of the loss rate by Gaussian probes (coherent or squeezed) is improved in the presence of Kerr nonlinearity. In particular, enhancement of precision may be substantial for short interaction time, i.e., for media of moderate size, e.g., biological samples. We analyze in detail the behavior of the quantum Fisher information (QFI), and determine the values of nonlinearity maximizing the QFI as a function of the interaction time and of the parameters of the input signal. We also discuss the precision achievable by photon counting and quadrature measurement and present additional results for truncated, few-photon, probe signals. Finally, we discuss the origin of the precision enhancement, showing that it cannot be linked quantitatively to the non-Gaussianity or the nonclassicality of the interacting probe signal.
Squeezed light has lower quantum noise in amplitude or phase than the quantum noise limit (QNL) of classical light. This enables enhancing sensitivity -- quantified by the signal-to-noise ratio (SNR) -- to beyond the QNL in optical techniques such as spectroscopy, gravitational wave detection, magnetometry and imaging. Precision -- the variance of repeated estimates -- has also been enhanced beyond the QNL using squeezed vacuum to estimate optical phase and transmission. However, demonstrations have been limited to femtowatts of probe power. Here we demonstrate simultaneous precision and sensitivity beyond the QNL for estimating modulated transmission using a squeezed amplitude probe of 0.2 mW average (25 W peak) power. This corresponds to 8 orders of magnitude above the power limitations of previous sub-QNL precision measurements. Our theory and experiment show precision enhancement scales with the amount of squeezing and increases with the resolution bandwidth of detection. We conclude that quantum enhanced precision in estimating a modulated transmission increases when observing dynamics at ∼\sim∼ kHz and above. This opens the way to performing measurements that compete with the optical powers of current classical techniques, but have superior precision and sensitivity beyond the classical limit.
Abstract Nonlinear optics plays a crucial role in science and technology, with applications ranging from spectroscopy to quantum information processing. Therefore, precise estimation of their nonlinear optical parameters is of fundamental importance. Here, we investigate quantum-enhanced sensitivity in the estimation of nonlinear absorption parameters, including saturable absorption (SA) and reverse saturable absorption (RSA). By employing the quantum Fisher information, we quantify the enhancement in sensitivity for estimating transmission ( T ), linear absorption coefficient ( α0\alpha _0α0​ ), saturable intensity ( IsI_sIs​ ), and two-photon absorption coefficient ( β\beta β ) using bright two-mode squeezed states (bTMSS) and applied it to analyze the nonlinear parameters of Pt nanoparticle samples as an example. In addition, we propose an experimental scheme based on an open-aperture Z-scan with bTMSS to realize quantum-enhanced sensitivity. Our findings establish a pathway toward quantum-enhanced estimation of nonlinear optical parameters.
Stark systems in which a linear gradient field is applied across a many-body system have recently been proposed for quantum sensing. Here, we explore sensing capacity of Stark probes, in both single-particle and many-body interacting systems, for estimating nonlinear forms of the gradient fields. Our analysis reveals that, this estimation can achieve super-Heisenberg scaling precision that grows linearly by increasing the nonlinearity. Specifically, we find a universal algebraic relation between the scaling of the precision and the degree of the nonlinearity. This universal behavior remains valid in both single-particle and many-body interacting probes and reflects itself in the properties of the phase transition from an extended to a localized phase, obtained through establishing a comprehensive finite-size scaling analysis. Considering a parabolic gradient potential composed of both linear and nonlinear fields, we used multiparameter estimation methodology to estimate the components of the gradient potential. The phase diagram of the system is determined in terms of both linear and nonlinear gradient fields showing how the nonlocalized phase turns into a localized one as the Stark fields increase. The sensing precision of both linear and nonlinear Stark fields follows the same universal algebraic relation that was found for the case of single parameter sensing. We demonstrate that simple and experimentally available measurements can reach the theoretical precision bounds. Finally, we show that quantum enhanced sensitivity is still achievable even when we incorporate the preparation time of the probe into our resource analysis.
The major problem of multiparameter quantum estimation theory is to find an ultimate measurement scheme to go beyond the standard quantum limits that each quasi-classical estimation measurement is limited by. Although, in some specifics quantum protocols without environmental noise, the ultimate sensitivity of a multiparameter quantum estimation can beat the standard quantum limit. However, the presence of noise imposes limitations on the enhancement of precision due to the inevitable existence of environmental fluctuations. Here, we address the motivation behind the usage of Gaussian quantum resources and their advantages in reaching the standard quantum limits under realistic noise. In this context, our work aims to explore the ultimate limits of precision for the simultaneous estimation of a pair of parameters that characterize the displacement channel acting on Gaussian probes and subjected to open dynamics. More precisely, we focus on a general two-mode mixed squeezed displaced thermal state, after reducing it to various Gaussian probes states, like; a two-mode pure squeezed vacuum, two-mode pure displaced vacuum, two-mode mixed displaced thermal, two-mode mixed squeezed thermal. To study the ultimate estimation precision, we evaluate the upper and bottom bound of HCRB in various cases. We find that when the entangled states, two-mode pure squeezed vacuum and two-mode mixed squeezed thermal, are employed as probes states, the upper and bottom bound of HCRB beats the standard quantum limit in the presence of a noisy environment.