In ultra- and deep-strong cavity quantum electrodynamics (QED) systems, many intriguing phenomena that do not conserve the excitation number are expected to occur. In this paper, we theoretically analyze the optical response of an ultrastrong cavity-QED system in which an atom is coupled to the first and third harmonic modes of a cavity, and report the possibility of deterministic three-photon down-conversion of itinerant photons upon reflection at the cavity. In the conventional parametric down-conversion, a strong input field is needed because of the smallness of the transition matrix elements of the higher-order processes. However, if we use an atom-cavity system in an unprecedentedly strong-coupling region, even a weak field in the linear-response regime is sufficient to cause this rare event involving the fourth-order transitions.
In ultra- and deep-strong cavity quantum electrodynamics (QED) systems, many intriguing phenomena that do not conserve the excitation number are expected to occur. In this paper, we theoretically analyze the optical response of an ultrastrong cavity-QED system in which an atom is coupled to the first and third harmonic modes of a cavity, and report the possibility of deterministic three-photon down-conversion of itinerant photons upon reflection at the cavity. In the conventional parametric down-conversion, a strong input field is needed because of the smallness of the transition matrix elements of the higher-order processes. However, if we use an atom-cavity system in an unprecedentedly strong-coupling region, even a weak field in the linear-response regime is sufficient to cause this rare event involving the fourth-order transitions.
We revisit the superstrong coupling regime of multi-mode cavity quantum electrodynamics (QED), defined to occur when the frequency of vacuum Rabi oscillations between the qubit and the nearest cavity mode exceeds the cavity's free spectral range. A novel prediction is made that the cavity's linear spectrum, measured in the vanishing power limit, can acquire an intricate fine structure associated with the qubit-induced cascades of coherent single-photon down-conversion processes. This many-body effect is hard to capture by a brute-force numerics and it is sensitive to the light-matter coupling parameters both in the infra-red and the ultra-violet limits. We focused at the example case of a superconducting fluxonium qubit coupled to a long transmission line section. The conversion rate in such a circuit QED setup can readily exceed a few MHz, which is plenty to overcome the usual decoherence processes. Analytical calculations were made possible by an unconventional gauge choice, in which the qubit circuit interacts with radiation via the flux/charge variable in the low-/high-frequency limits, respectively. Our prediction of the fine spectral structure lays the foundation for the "strong down-conversion" regime in quantum optics, in which a single photon excited in a non-linear medium spontaneously down-converts faster than it is absorbed.
Interference-induced photon antibunching is investigated for a three-level system coupled to a cavity mode, in which the level scheme is of a lambda type. One of the transitions is weakly coupled to the cavity mode while the other is driven by a control field. Without the control field, i.e. , in the conventional cavity quantum electrodynamics (QED) scheme in the weak coupling regime, photon antibunching can be achieved by carefully choosing the coupling strength and the detuning. This condition can be alleviated by tuning the strength and the frequency of the control field. The condition for the optimal control field that yields photon blockade is derived, and the effects of changing various parameters are investigated. For a given a set of dissipation rates, the atom-cavity coupling strength g needs to be higher than a certain threshold value, although the whole system still remains in the weak coupling regime. A numerical method for finding the optimal parameter regime is proposed.
We propose a new method for frequency conversion of photons which is both versatile and deterministic. We show that a system with two resonators ultrastrongly coupled to a single qubit can be used to realise both single- and multiphoton frequency-conversion processes. The conversion can be exquisitely controlled by tuning the qubit frequency to bring the desired frequency-conversion transitions on or off resonance. Considering recent experimental advances in ultrastrong coupling for circuit QED and other systems, we believe that our scheme can be implemented using available technology.
A single two-level emitter coupled to a single mode of an electromagnetic resonator constitutes the most fundamental instance of light--matter interaction. Realizations of this type of system are investigated in the field of cavity quantum electrodynamics (cavity QED). Particularly important are schemes in which the coupling is strong enough to exceed the spontaneous emission rate as well as cavity damping. In this case, the coherent exchange of excitation between source and photon is the dominating process, providing the unique possibility to deterministically control the quantum evolution of the system. Great progress has recently been accomplished, technologically as well as conceptually, and the focus section in this issue of Journal of Optics B: Quantum and Semiclassical Optics features five articles highlighting important recent developments in the field. Strong coupling between single atoms and the electromagnetic cavity field have been achieved in two distinct regimes, the optical and the microwave region. The latter is represented by the micromaser, a high-Q microwave cavity pumped by a beam of highly excited Rydberg atoms. It has proved to be an almost ideal system for the generation of non-classical field states. A constraint in these experiments is the fact that the field inside the cavity can only be examined indirectly, by analysing the occupation of atoms leaving the cavity. While only two atomic states were previously identified for this purpose, V A Reshetov shows in his article (pages 119--126) that more information on the field may be extracted by taking advantage of the Zeeman substructure of the atomic levels. In the optical domain of cavity QED, by contrast, the state of the resonator field may be probed directly by measuring the light leaking from the cavity using photodetectors. In order to minimize damping, high-quality cavities must be employed. In most optical experiments these are Fabry--Perot resonators with ultra-high reflectivity mirrors, with losses as low as a few parts per million being state of the art. At the same time, the coupling of atoms and photons is enhanced by reducing the length of the cavity, so that strong coupling conditions are reached. A very attractive application of this type of cavity QED setup is the possibility of exerting control over the quantum dynamics of the system. An impressive example is the implementation of quantum feedback, reported in the paper by W P Smith and L A Orozco (pages 127--134). Using information gained from detecting a single photon escaping from the cavity, active feedback is applied to halt the dynamical evolution of the system. This is the first time active feedback has been used to modify the quantum evolution of a system at the single-photon level. The authors discuss how detunings between the subsystems affect the quantum feedback, an issue particularly relevant for ensembles of atoms with a spread in detuning. Perfect quantum feedback in this case requires the use of additional parameters to control the system. The majority of optical cavity QED experiments performed so far have used as a medium atoms traversing the cavity on random trajectories, such as, for example, thermal atomic beams. In this case, the observation of quantum effects is degraded in two ways. The Doppler effect and the finite transit time lead to line broadening, while the spatial structure of the cavity mode results in atoms in different locations experiencing different coupling with the photonic field. J E Reiner et al (pages 135--142) investigate the impact of these effects on quantum fluctuations in their cavity QED system. In order to overcome line broadening, they have developed a continuous cold atomic beam, extracted from a magneto-optical trap. An even better control of broadening effects and fluctuating coupling strength is provided by trapping the atoms inside the cavity and cooling them to temperatures at which their position spread is smaller than the optical wavelength. Much recent activity has been devoted to developing such an ultimate cavity QED system. A Vukics et al (pages 143--153) present a theoretical proposal for dynamically trapping and cooling atoms inside a cavity. By driving the atoms with a standing wave injected from the side of the cavity and by weakly exciting the cavity field itself, they predict three-dimensional trapping of the atom for periods around 1 second, an extremely long time on the typical scale of cavity QED dynamics. The essential component of their scheme is the interference between the two driving fields, determining the temperature of the particle and the stable trapping positions. In the quest for better confinement of radiation, lately, an appealing alternative to the Fabry--Perot cavity has been investigated -- the optical microsphere resonator. A sphere with a diameter of a few tens of microns, it supports so-called whispering gallery modes near its circumference, for which quality factors up to 10 10 have been measured. In order to exploit the correspondingly low field damping rates for cavity QED, a method must be found to couple atomic or solid state emitters to these modes. S Göotzinger et al (pages 154--158) report the coupling of single nanocrystals on the surface of a microsphere through the evanescent field of the mode. Selective excitation of a single nano-emitter was accomplished with a scanning confocal microscope. The system is a promising candidate for cavity QED with single-quantum emitters. The ability to fully control the quantum dynamics of atoms and light is beginning to spawn early applications. The most notable example is quantum information processing. This requires the coherent manipulation of single-quantum systems, which is ideally provided by cavity QED interaction in the strong-coupling limit. The development of practical devices will be among the principal future tasks for research in the field. This will include physical systems, which have not been covered in this issue, such as semiconductors, quantum dots as emitters, or photonic crystals as resonator structures. Cavity QED is therefore guaranteed to remain a vigorous field in the years to come.
When an atom is strongly coupled to a cavity, the two systems can exchange a single photon through a coherent Rabi oscillation. This process enables precise quantum-state engineering and manipulation of atoms and photons in a cavity, which play a central role in quantum information and measurement. Recently, a new regime of cavity QED was reached experimentally where the strength of the interaction between light and artificial atoms (qubits) becomes comparable to the atomic transition frequency or the resonance frequency of the cavity mode. Here we show that this regime can strongly modify the concept of vacuum Rabi oscillations, enabling multiphoton exchanges between the qubit and the resonator. We find that experimental state-of-the-art circuit-QED systems can undergo two- and three-photon vacuum Rabi oscillations. These anomalous Rabi oscillations can be exploited for the realization of efficient Fock-state sources of light and complex entangled states of qubits.
Deterministic single-photon sources are indispensable core devices for quantum information technology, yet high-performance implementation remains a long-standing bottleneck for linear optical quantum computing. We propose a feasible scheme for deterministic single-photon emission based on a △-type three-level atom coupled to a single-mode cavity, driven by two classical external fields, which is adaptable to both strong and ultrastrong cavity-atom coupling regimes. Under continuous-wave driving, the system achieves excellent single-photon characteristics: the normalized equal-time second-order correlation function reaches g(2)(0)∼10−6, with a photon indistinguishability of 98.73% and a state purity of 99.95% in the strong coupling regime, while the ultrastrong coupling regime further suppresses G(2)(0)∼10−8, yielding an indistinguishability of 99.10% and a purity of 99.99%. For pulsed driving in the ultrastrong coupling regime, the source realizes superior performance, with an emission efficiency, indistinguishability, and purity of 99.96%, 98.98%, and 99.99% under resonant conditions, and 100%, 95.91%, and 99.93% under detuned conditions, respectively. The near-ideal optical performance of the proposed scheme provides a viable route for constructing high-quality deterministic single-photon sources, which offers a promising solution to the limitations of conventional single-photon devices and facilitates the further development of quantum information science and fundamental quantum optical research.