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arXiv:2109.01857 · Physical Review A

Distinguishability in quantum interference with multimode squeezed states

V. S. Shchesnovich

Published Jun 2, 2022• 8 citations
arXivHTMLPDF

Abstract

Distinguishability theory is developed for quantum interference of the squeezed vacuum states on unitary linear interferometers. It is found that the entanglement of photon pairs over the Schmidt modes is one of the sources of distinguishability. The distinguishability is quantified by the symmetric part of the internal state of $n$ pairs of photons over the spectral Schmidt modes, whose normalization ${q}_{2n}$ is the probability that $2n$ photons interfere as indistinguishable. For two pairs of photons ${q}_{4}=(1+2\mathbb{P})/3$, where $\mathbb{P}$ is the purity of the squeezed states ($K=1/\mathbb{P}$ is the Schmidt number). For a fixed purity $\mathbb{P}$, the probability ${q}_{2n}$ decreases exponentially fast in $n$. For example, in the experimental Gaussian boson sampling of H.-S. Zhong et al., [Science 370, 1460 (2020)], the achieved purity $\mathbb{P}\ensuremath{\approx}0.938$ for the average number of photons $2n\ensuremath{\ge}43$ gives ${q}_{2n}\ensuremath{\lesssim}0.5$, i.e., close to the middle line between $n$ indistinguishable and $n$ distinguishable pairs of photons. In derivation of all the results, the first-order quantization representation based on the particle decomposition of the Hilbert space of identical bosons serves as an indispensable tool. The approach can be applied also to the generalized (non-Gaussian) squeezed states, such as those recently generated in the three-photon parametric down-conversion.

DOI
10.1103/physreva.105.063703

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Distinguishability theory is developed for quantum interference of the squeezed vacuum states on unitary linear interferometers. It is found that the entanglement of photon pairs over the Schmidt modes is one of the sources of distinguishability. The distinguishability is quantified by the symmetric part of the internal state of nnn pairs of photons over the spectral Schmidt modes, whose normalization q2n{q}_{2n}q2n​ is the probability that 2n2n2n photons interfere as indistinguishable. For two pairs of photons q4=(1+2P)/3{q}_{4}=(1+2\mathbb{P})/3q4​=(1+2P)/3, where P\mathbb{P}P is the purity of the squeezed states (K=1/PK=1/\mathbb{P}K=1/P is the Schmidt number). For a fixed purity P\mathbb{P}P, the probability q2n{q}_{2n}q2n​ decreases exponentially fast in nnn. For example, in the experimental Gaussian boson sampling of H.-S. Zhong et al., [Science 370, 1460 (2020)], the achieved purity P\ensuremath≈0.938\mathbb{P}\ensuremath{\approx}0.938P\ensuremath≈0.938 for the average number of photons 2n\ensuremath≥432n\ensuremath{\ge}432n\ensuremath≥43 gives q2n\ensuremath≲0.5{q}_{2n}\ensuremath{\lesssim}0.5q2n​\ensuremath≲0.5, i.e., close to the middle line between nnn indistinguishable and nnn distinguishable pairs of photons. In derivation of all the results, the first-order quantization representation based on the particle decomposition of the Hilbert space of identical bosons serves as an indispensable tool. The approach can be applied also to the generalized (non-Gaussian) squeezed states, such as those recently generated in the three-photon parametric down-conversion.
Photon distinguishability is a fundamental property manifested in multiphoton interference and one of the main sources of noise in any photonic quantum information processing. In this work, rather than relying on first-quantization methods, we build on a generating-function framework based on the phase-space formalism to characterize the effects of partial distinguishability on the interference of single-mode squeezed states. Our approach goes beyond commonly used models that represent distinguishability via additional noninterfering modes and captures genuine multiphoton interference effects induced by the overlap of the internal state of the photons. This description provides a clear physical account of how distinguishability gives rise to effective noise in Gaussian boson sampling protocols while enabling a systematic investigation of phase effects arising from the overlap of the internal states.
We show that it is possible for completely distinguishable particles to interfere postselectively without operating on, or indeed having any knowledge of, the distinguishing degree of freedom. In particular, we find a family of three-mode spatial interferometers that, upon inputting, say, a red photon in port 1 and a green photon in port 2, produce a state such that when vacuum is detected at one output, the two photons in the other two outputs will pass a HOM test, despite their frequency degree of freedom remaining untouched. In doing so we develop a general approach to distinguishability based on the Schmidt decomposition between particles' "System" and "Label" degrees of freedom, corresponding to what has been called unitary-unitary duality in many-body physics. This also gives insight into the relationship between the first and second quantized pictures, which is useful in bringing other quantum information concepts across from the former to the latter.
This thesis explores the interference of nonclassical states of light, particularly Fock and Gaussian states, in noisy linear interferometers, with applications to quantum information and quantum sensing. Using the phase-space formalism, analytical tools based on generating functions are developed to describe quantum optical interference in a unified way. For multiphoton Fock states, new zero probability events (suppression laws) are identified beyond the previously derived symmetry permutation principle, revealing rich interference structures that is degraded with photon distinguishability. For Gaussian states, the Hafnian-based description of Gaussian Boson Sampling is extended to include partial distinguishability via the overlap matrix of the internal state of the photons. Finally, the link between these interference effects and quantum multiparameter estimation is examined for the simultaneous estimation of phase and loss. This study shows that while probe incompatibility can vanish for optimized non-Gaussian states and some two-mode Gaussian states, at high photon number, measurement incompatibility remains a fundamental constraint even in this limit.
Using tools from quantum information theory, we present a general theory of indistinguishability of identical bosons in experiments consisting of passive linear optics followed by particle number detection. Our results do neither rely on additional assumptions on the input state of the interferometer, such as, for instance, a fixed mode occupation, nor on any assumption on the degrees of freedom that potentially make the particles distinguishable. We identify the expectation value of the projector onto the N-particle symmetric subspace as an operationally meaningful measure of indistinguishability, and derive tight lower bounds on it that can be efficiently measured in experiments. Moreover, we present a consistent definition of perfect distinguishability and characterize the corresponding set of states. In particular, we show that these states are diagonal in the computational basis up to a permutationally invariant unitary. Moreover, we find that convex combinations of states that describe partially distinguishable and perfectly indistinguishable particles can lead to perfect distinguishability, which itself is not preserved under convex combinations.
Quantum interference constitutes one of the sharpest divides between our classical intuition and the weirdness of the quantum world. Whenever there are multiple paths leading to the same outcome, it is the interplay of associated probability amplitudes that determines measurement results. In the double slit experiment, wave-like interference governs the distribution of particles on a detection screen. Extending to multiple particles allows behaviour that cannot be described by a classical wave, such as the bunching of photon pairs in Hong-Ou-Mandel interference. In both these examples, the ability to distinguish the interfering paths leads to degradation of interference and a return to behaviour described by probabilities. Understanding how this transition evolves for larger multiparticle quantum systems is of fundamental interest and also vital for developing photonic quantum technologies that rely on many-photon interference. In this thesis we investigate the role of distinguishability in the interference of three and four independent photons by using polarisation and time delays. For three photons, a new type of collective distinguishing phase appears that goes beyond a pairwise description of the similarity of quantum states. We use nonlinear photon sources and a fibre interferometer to experimentally demonstrate the ability to tune and isolate this phase in interference statistics. Extending to four photons we show that, contrary to intuition from two-photon experiments, the interference of photons prepared in distinguishable states is possible due to a four-particle phase. This is confirmed experimentally using a bulk four-mode interferometer. We then extend our study to include the effects of state impurity in the interference of three photons. New properties of this interference enable diagnosis of realistic experimental imperfections and characterisation tasks impossible using only two photons. Finally, we link discussions of state distinguishability to the group representations underpinning the exchange symmetry of multiparticle wavefunctions.
Abstract These two accompanying papers are concerned with two mode entanglement for systems of identical massive bosons and the relationship to spin squeezing and other quantum correlation effects. Entanglement is a key quantum feature of composite systems in which the probabilities for joint measurements on the composite sub-systems are no longer determined from measurement probabilities on the separate sub-systems. There are many aspects of entanglement that can be studied. This two-part review focuses on the meaning of entanglement, the quantum paradoxes associated with entangled states, and the important tests that allow an experimentalist to determine whether a quantum state—in particular, one for massive bosons is entangled. An overall outcome of the review is to distinguish criteria (and hence experiments) for entanglement that fully utilize the symmetrization principle and the super-selection rules that can be applied to bosonic massive particles. In the first paper (I), the background is given for the meaning of entanglement in the context of systems of identical particles. For such systems, the requirement is that the relevant quantum density operators must satisfy the symmetrization principle and that global and local super-selection rules prohibit states in which there are coherences between differing particle numbers. The justification for these requirements is fully discussed. In the second quantization approach that is used, both the system and the sub-systems are modes (or sets of modes) rather than particles, particles being associated with different occupancies of the modes. The definition of entangled states is based on first defining the non-entangled states—after specifying which modes constitute the sub-systems. This work mainly focuses on the two mode entanglement for massive bosons, but is put in the context of tests of local hidden variable theories, where one may not be able to make the above restrictions. The review provides the detailed arguments necessary for the conclusions of a recent paper, where the question of how to rigorously demonstrate the entanglement of a two-mode Bose–Einstein condensate (BEC) has been examined. In the accompanying review paper (II), we consider spin squeezing and other tests for entanglement that have been proposed for two-mode bosonic systems. We apply the approach of review (I) to determine which tests, and which modifications of the tests, are useful for detecting entanglement in massive bosonic (BEC), as opposed to photonic, systems. Several new inequalities are derived, a theory for the required two-mode interferometry is presented, and key experiments to date are analyzed.