Quantum van der Pol oscillators are driven-dissipative systems displaying quantum synchronization phenomena. When forced by a squeezed drive, the frequency adjusts to half of the forcing displaying multiple preferred phases. Here we analyze the physical origin of this entrained response, establishing a connection with metastability in open quantum systems. We report a dynamical regime characterized by a huge separation of time scales, in which a dynamical mode displays a lifetime that can be orders of magnitude larger than the rest. In this regime, the long-time dynamics is captured by an incoherent process between two metastable states, which correspond to the preferred phases of the synchronized oscillator. In fact, we show that quantum entrainment is here characterized by fluctuations driving an incoherent process between two metastable phases, which ultimately limits its temporal coherence when moving into the quantum regime. Finally, we discuss connections with the phenomena of dissipative phase transitions and transient synchronization in open quantum systems.
Quantum van der Pol oscillators are driven-dissipative systems displaying quantum synchronization phenomena. When forced by a squeezed drive, the frequency adjusts to half of the forcing displaying multiple preferred phases. Here we analyze the physical origin of this entrained response, establishing a connection with metastability in open quantum systems. We report a dynamical regime characterized by a huge separation of time scales, in which a dynamical mode displays a lifetime that can be orders of magnitude larger than the rest. In this regime, the long-time dynamics is captured by an incoherent process between two metastable states, which correspond to the preferred phases of the synchronized oscillator. In fact, we show that quantum entrainment is here characterized by fluctuations driving an incoherent process between two metastable phases, which ultimately limits its temporal coherence when moving into the quantum regime. Finally, we discuss connections with the phenomena of dissipative phase transitions and transient synchronization in open quantum systems.
Recently, several studies have investigated synchronization in quantum-mechanical limit-cycle oscillators. However, the quantum nature of these systems remained partially hidden, since the dynamics of the oscillator's phase was overdamped and therefore incoherent. We show that there exist regimes of underdamped and even quantum-coherent phase motion, opening up new possibilities to study quantum synchronization dynamics. To this end, we investigate the Van der Pol oscillator (a paradigm for a self-oscillating system) synchronized to an external drive. We derive an effective quantum model which fully describes the regime of underdamped phase motion and additionally allows us to identify the quality of quantum coherence. Finally, we identify quantum limit cycles of the phase itself.
Synchronisation has been explored extensively for classical systems from the mid-1600s, and is a phenomenon widely understood in many diverse systems. In the age of technology miniaturisation, there are great incentives to develop an understanding of quantum synchronisation, where quantum fluctuations become the dominant source of noise and non-classical features become important. This thesis considers different types of synchronisation in systems that can display highly non-linear, quantum behaviours. Phase synchronisation for a micromaser coupled to an external drive is initially considered, and it is found that for low photon numbers a semiclassical approximation underestimates phase synchronisation, but a perturbation theory can be accurate for sufficiently weak coupling in either a quantum or semiclassical regime. When a small detuning between the drive and micromaser is introduced, frequency entrainment is also found to exist. Then two micromasers are coupled with each other, in two different configurations, and synchronisation through a relative phase preference is found for each. A semiclassical approximation once again underestimates the phase synchronisation. Entanglement and mutual information are found to behave differently to the relative phase preference depending on each system's parameters. Finally, a mean-field theory is considered for many coupled van der Pol oscillators and micromasers respectively. As the coupling between the oscillators is increased, a critical point is reached and the systems undergo a transition to a phase synchronised state. This bistability appears via a saddle-node bifurcation, and in addition to examining a variety of properties before and after the transition the critical scaling behaviour was investigated close to the transition.
Classical self-sustained oscillators, which generate periodic motion without periodic external forcing, are ubiquitous in science and technology. The realization of nonclassical self-oscillators is an important goal of quantum physics. We here present the experimental implementation of a quantum van der Pol oscillator, a paradigmatic autonomous quantum driven-dissipative system with nonlinear damping, using a single trapped atom. We demonstrate the existence of a quantum limit cycle in phase space in the absence of a drive and the occurrence of quantum synchronization when the nonlinear oscillator is externally driven. We additionally show that synchronization can be enhanced with the help of squeezing perpendicular to the direction of the drive and, counterintuitively, linear dissipation. We also observe the bifurcation to a bistable phase-space distribution for large squeezing. Our results pave the way for the exploration of self-sustained quantum oscillators and their application to quantum technology.
We present a general theory of classical metastability in open quantum systems. Metastability is a consequence of a large separation in timescales in the dynamics, leading to the existence of a regime when states of the system appear stationary, before eventual relaxation toward a true stationary state at much larger times. In this work, we focus on the emergence of classical metastability, i.e., when metastable states of an open quantum system with separation of timescales can be approximated as probabilistic mixtures of a finite number of states. We find that a number of classical features follow from this approximation, for the manifold of metastable states, long-time dynamics between them, and symmetries of the dynamics. Namely, those states are approximately disjoint and thus play the role of metastable phases, the relaxation toward the stationary state is approximated by a classical stochastic dynamics between them, and weak symmetries correspond to their permutations. Importantly, the classical dynamics is observed not only on average but also at the level of individual quantum trajectories: We show that time coarse-grained continuous measurement records can be viewed as noisy classical trajectories, while their statistics can be approximated by that of the classical dynamics. Among others, this explains how first-order dynamical phase transitions arise from metastability. Finally, to verify the presence of classical metastability in a given open quantum system, we develop an efficient numerical approach that delivers the set of metastable phases together with the effective classical dynamics. Since the proximity to a first-order dissipative phase transition manifests as metastability, the theory and tools introduced in this work can be used to investigate such transitions---which occur in the large size limit---through the metastable behavior of many-body systems of moderate sizes accessible to numerics.
We employ a quantum trajectory approach to characterize synchronization and phase-locking between open quantum systems in nonequilibrium steady states. We exemplify our proposal for the paradigmatic case of two quantum Van der Pol oscillators interacting through dissipative coupling. \nWe show the deep impact of synchronization on the statistics of phase-locking indicators and other correlation measures defined for single trajectories, spotting a link between the presence of synchronization and the emergence of large tails in the probability distribution for the entanglement along trajectories. Our results shed new light on fundamental issues regarding quantum synchronization providing new methods for its precise quantification.
Open quantum systems with nearly degenerate energy levels have been shown to exhibit long-lived metastable states in the approach to equilibrium, even when modelled with certain Lindblad-form quantum master equations. This is a result of dramatic separation of timescales due to differences between Liouvillian eigenvalues. These metastable states often have nonzero coherences that die off only in the long-time limit once the system reaches thermal equilibrium. We examine two distinct situations that give rise to this effect: one in which dissipative dynamics couple together states only within a nearly degenerate subspace, and one in which they give rise to jumps over finite-energy splittings, between nearly degenerate subspaces. We find, in each case, that a change of basis can often lead to a representation that more naturally captures the impact of the system-bath interaction than does the energy eigenbasis, revealing that separate timescales are associated with separate processes (e.g., decoherence into a nonenergy eigenbasis, decay of population correlations to the initial state). This approach is paired with the inspection of quantum trajectories, which further provide intuition as to how open system evolution is characterized when coherent oscillations, thermal relaxation, and decoherence all occur simultaneously. Published by the American Physical Society 2024