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arXiv:2108.13738 · Physical Review Letters

Fast Quantum State Tomography in the Nitrogen Vacancy Center of Diamond

Jingfu Zhang, Swathi S. Hegde, Dieter Suter

Published Feb 28, 2023• 16 citations
arXivHTMLPDF

Abstract

Quantum state tomography is the procedure for reconstructing unknown quantum states from a series of measurements of different observables. Depending on the physical system, different sets of observables have been used for this procedure. In the case of spin qubits, the most common procedure is to measure the transverse magnetization of the system as a function of time. Here, we present a different scheme that relies on time-independent observables and therefore does not require measurements at different evolution times, thereby greatly reducing the overall measurement time. To recover the full density matrix, we use a set of unitary operations that transform the density operator elements into the directly measurable observable. We demonstrate the performance of this scheme in the electron-nuclear spin system of the nitrogen vacancy center in diamond.

DOI
10.1103/physrevlett.130.090801

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Quantum state tomography is the procedure for reconstructing unknown quantum states from a series of measurements of different observables. Depending on the physical system, different sets of observables have been used for this procedure. In the case of spin qubits, the most common procedure is to measure the transverse magnetization of the system as a function of time. Here, we present a different scheme that relies on time-independent observables and therefore does not require measurements at different evolution times, thereby greatly reducing the overall measurement time. To recover the full density matrix, we use a set of unitary operations that transform the density operator elements into the directly measurable observable. We demonstrate the performance of this scheme in the electron-nuclear spin system of the nitrogen vacancy center in diamond.
Quantum state tomography (QST) of electron-nuclear spins of nitrogen-vacancy (NV) center in diamond commonly requires a sequence of population flipping operations and frequent calibration of basis states by fluorescence photon-counting. Here, we realize an effective and robust quantum state tomography of electron-nuclear spins based on time-resolved fluorescence, which can enhance the signal-to-noise ratio between different basis states up to 29.6% compared to the photon-counting method. Meanwhile, our method can directly obtain the population of four basis states with only one measurement, which significantly improves the efficiency of tomography. Furthermore, the photon count rate fluctuation of time-resolved fluorescence can be reduced to the standard quantum limit by normalization operation, indicating that the time-resolved method is calibration-free. This method could be easily applied to multi-nuclear spins of NV center in diamond and extended to other solid-state spin systems.
We report on a quantum state characterization method, which we call Rabi-based quantum state tomography (RQST), that we have validated on single-qubit quantum states, in particular on the electron and nuclear spins of a single nitrogen-vacancy (NV) center in diamond, demonstrating high fidelities. The difference of RQST with conventional tomography methods is in the implementation of rotation operators and construction of the density matrix from the measured datasets. We demonstrate efficient quantum state control of the electron spin at room temperature with an average fidelity of 0.995 over more than 40 measurements on different states on the Bloch sphere. Also, we apply the methodology to the dark NV nuclear spin state. The state is read via the electron spin using the C-NOT two-qubit entanglement gate and demonstrates fidelities of the same order.
High fidelity quantum state tomography of electron-14^{14}14N nuclear hybrid spin register in diamond using Rabi oscillations
We report on a new quantum state characterisation method, which we call Rabi-based Quantum State Tomography (RQST), that we have validated on single-qubit quantum states, in particular on the electron and nuclear spins of a single nitrogen-vacancy (NV) centre in diamond, demonstrating high fidelities. The difference of RQST with conventional tomography methods is in the implementation of rotation operators and construction of density matrix from the measured data sets. We demonstrate efficient quantum state control of the electron spin at room temperature with an average fidelity of 0.995 over more than 40 measurements on different states on the Bloch sphere with a maximum fidelity of 0.99992. Also, we apply the methodology to the dark NV nuclear spin state. The state is read via the electron spin using the C-NOT two-qubit entanglement gate and demonstrate fidelities of the same order.
Single-qubit measurements are typically insufficient for inferring arbitrary quantum states of a multiqubit system. We show that, if the system can be fully controlled by driving a single qubit, then utilizing a local random pulse is almost always sufficient for complete quantum-state tomography. Experimental demonstrations of this principle are presented using a nitrogen-vacancy (NV) center in diamond coupled to a nuclear spin, which is not directly accessible. We report the reconstruction of a highly entangled state between the electron and nuclear spin with fidelity above 95% by randomly driving and measuring the NV-center electron spin only. Beyond quantum-state tomography, we outline how this principle can be leveraged to characterize and control quantum processes in cases where the system model is not known.
We present the experimental reconstruction of the Wigner function of an individual electronic spin qubit associated with a nitrogen-vacancy center in diamond at room temperature. This spherical Wigner function contains the same information as the density matrix for arbitrary spin systems. As an example, we exactly characterize the quantum state of a single qubit undergoing a nearly pure dephasing process by the Wigner function. The fidelities and purities during this process are extracted from the experimentally reconstructed Wigner functions, whose dynamics agree with the theoretical prediction.
We present Tomography-NMR, an open-source Python package that reconstructs quantum density matrices from spectroscopic measurement data. The package implements a complete analysis pipeline for two-qubit quantum state tomography based on the product operator formalism: raw time-domain signals are Fourier-transformed into frequency-domain spectra, spectral peak intensities are mapped to expansion coefficients of the density matrix, and the full quantum state is reconstructed. Three integration methods are provided for different use cases: direct peak height measurement and fixed-parameter numerical integration require no theoretical reference and are suited to unknown states, achieving fidelities of approximately 98\% on a benchmark set of known states, while a systematic parameter optimization against a known target state achieves reconstruction fidelities exceeding 99\% for the same benchmark states. While the detailed theoretical framework for quantum state tomography is well established, the practical procedures for extracting density matrices from experimental spectra are often inadequately documented in the literature and obscured within proprietary software. This package addresses that gap by providing a fully transparent, reproducible implementation of every analysis step, from spectral preprocessing to density matrix visualization. The software has been validated on experimentally prepared two-qubit states measured via nuclear magnetic resonance (NMR) spectroscopy of coupled 31^{31}31P nuclei. Average reconstruction fidelities range from 0.975 to 0.995 across a benchmark set of 20 two-qubit states, including the computational basis states, Bell states, and the outputs of three fundamental quantum gates (CNOT, H, and T). Although developed for NMR, the modular architecture facilitates adaptation to other spectroscopic platforms and alternative measurement protocols.