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arXiv:2108.12691

Quantum simulation of an exotic quantum critical point in a two-site charge Kondo circuit

Winston Pouse, Lucas Peeters, Connie L. Hsueh, U. Gennser, A. Cavanna, M. A. Kastner, Andrew K. Mitchell, David Goldhaber‐Gordon

Published Aug 28, 2021• 3 citations
arXivHTMLPDF

Abstract

Tuning a material to the cusp between two distinct ground states can produce exotic physical properties, unlike those in either of the neighboring phases. The prospect of designing a model experimental system to capture such behavior is tantalizing. An array of tunnel-coupled quantum dots, each hosting a local spin, should have an appropriately complex phase diagram, but scaling up from individual dots to uniform clusters or lattices has proven difficult: though each site can be tuned to the same occupancy, each has a different set of localized wavefunctions whose couplings to neighboring sites cannot be made fully uniform. An array of metal nanostructures has complementary strengths and weaknesses: simple electrostatic tuning can make each element behave essentially identically, but intersite coupling is not tunable. In this work, we study a tunable nanoelectronic circuit comprising two coupled hybrid metallic-semiconductor islands, combining the strengths of the two types of materials, and demonstrating the potential for scalability. With two charge states of an island acting as an effective spin-1/2, the new architecture also offers a rich range of coupling interactions, and we exploit this to demonstrate a novel quantum critical point. Experimental results in the vicinity of the critical point match striking theoretical predictions.

DOI
10.48550/arxiv.2108.12691

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Tuning a material to the cusp between two distinct ground states can produce exotic physical properties, unlike those in either of the neighboring phases. The prospect of designing a model experimental system to capture such behavior is tantalizing. An array of tunnel-coupled quantum dots, each hosting a local spin, should have an appropriately complex phase diagram, but scaling up from individual dots to uniform clusters or lattices has proven difficult: though each site can be tuned to the same occupancy, each has a different set of localized wavefunctions whose couplings to neighboring sites cannot be made fully uniform. An array of metal nanostructures has complementary strengths and weaknesses: simple electrostatic tuning can make each element behave essentially identically, but intersite coupling is not tunable. In this work, we study a tunable nanoelectronic circuit comprising two coupled hybrid metallic-semiconductor islands, combining the strengths of the two types of materials, and demonstrating the potential for scalability. With two charge states of an island acting as an effective spin-1/2, the new architecture also offers a rich range of coupling interactions, and we exploit this to demonstrate a novel quantum critical point. Experimental results in the vicinity of the critical point match striking theoretical predictions.
The physical properties of a material tuned to the cusp between two distinct ground states can be quite exotic, and unlike those in either of the neighboring phases. The prospect of capturing such behavior in a simple model is tantalizing; for example, the interplay between heavy fermion physics and magnetic ordering in certain materials is often rationalized in terms of the quantum phase transition in the two-impurity Kondo model. However, this model is oversimplified for the purpose: its quantum critical point does not reflect the distinctive properties of a magnetic lattice surrounded by mobile electrons. In this work, we study a tunable nanoelectronic circuit comprising two coupled charge-Kondo quantum islands, realizing a new model which captures the essence of competition between local and collective screening of magnetic moments. This may have relevance for materials in which collective many-body effects drive lattice coherence. We tune our device to a novel quantum critical point, and show experimentally that deviations as we tune away from this point match non-trivial predictions from the model. This work on the crucial role of inter-island interactions is a necessary first step in scaling up such circuits from individual sites to networks or lattices.
Hybrid metal-semiconductor quantum circuits offer a controlled setting for realizing and probing strongly correlated quantum matter. A largely open question that may be addressed by such simulators is whether coupled critical states can combine into new non-Fermi liquid (NFL) phases. Inspired by the recent realization of a two-site charge-Kondo circuit [W. Pouse \textit{et al.}, \href{https://www.nature.com/articles/s41567-022-01905-4}{Nat. Phys. \textbf{19}, 492 (2023)}], we uncover the fate of coupled Kondo anyons emerging from the two-channel-Kondo critical point at each site. Bosonization and quantum Brownian motion methods yield the full quasiballistic phase diagram and low-temperature transport properties, while numerical renormalization group calculations resolve the complementary weak-coupling limit. Together, these provide a unified description, and reveal robust NFL phases with continuously tunable transport and susceptibility exponents. Stronger inter-site coupling ultimately produces a screened Fermi liquid.
We study the influence of many-body interactions on the transport properties in a two-site charge Kondo circuit recently implemented in a hybrid metal-semiconductor double-quantum dot device [W. Pouse {\it et al.}, Nat. Phys. {\bf 19}, 492 (2023)]. There emerge two principal types of interactions: (i) an intrinsic one, described by the Luttinger liquid model, and (ii) an induced one, which appears due to the coupling of the system to an Ohmic environment. Case (i) could be achieved if the charge Kondo circuit operates in the fractional quantum Hall regime, while case (ii) can be implemented via a finite number of open ballistic channels coupled to both the quantum dots. We demonstrate that the conductance scaling for the case of strong and weak interdot coupling is fully determined by the effective interaction parameter, which is the combination of the fractional filling factor ν=1/mν=1/mν=1/m and the number of transmitting channels. Furthermore, we predict that the fractional filling factor ννν defines a universal Kondo scaling in the vicinity of a special triple quantum critical point featured by the emergence of a Z3\mathbb{Z}_3Z3​ parafermion.
We study the influence of many-body interactions on the transport properties in a two-site charge Kondo circuit recently implemented in a hybrid metal-semiconductor double-quantum dot device [W. Pouse et al., Nat. Phys. 19, 492 (2023)]. There emerge two principal types of interactions: (i) an intrinsic one, described by the Luttinger liquid model, and (ii) an induced one, which appears due to the coupling of the system to an Ohmic environment. Case (i) could be achieved if the charge Kondo circuit operates in the fractional quantum Hall regime, while case (ii) can be implemented via a finite number of open ballistic channels coupled to both the quantum dots. We demonstrate that the conductance scaling for the case of strong and weak interdot coupling is fully determined by the effective interaction parameter, which is the combination of the fractional filling factor $\ensuremath{\nu}=1/m$ and the number of transmitting channels. Furthermore, we predict that the fractional filling factor $\ensuremath{\nu}$ defines a universal Kondo scaling in the vicinity of a special triple-quantum critical point featured by the emergence of a Z3{\mathbb{Z}}_{3}Z3​ parafermion.
We investigate systems comprising chains and rings of quantum dots, coupled to two metallic leads. Such systems allow to study the competition between orbital and spin degrees of freedom in a nanodevice, and the effect this subtle interplay has on two-channel Kondo (2CK) physics. We demonstrate that a rich range of strongly correlated electron behaviour results, with non-Fermi liquid 2CK phases and non-trivial phase transitions accessible. We employ physical arguments and the numerical renormalization group (NRG) technique to analyse these systems in detail, examining in particular both thermodynamic and dynamical properties. When leads are coupled to either end of a chain of dots, we show that the resulting behaviour on low temperature/energy scales can be understood in terms of simpler paradigmatic quantum `impurity' models. An effective low-energy single-spin 2CK model is derived for all odd-length chains, while the behaviour of even-length chains is related fundamentally to that of the classic `two-impurity Kondo' model. In particular, for small interdot coupling, we show that an effective coupling mediated though incipient single-channel Kondo states drives all odd chains to the 2CK fixed point (FP) on the lowest temperature/energy scales. A theory is also developed to describe a phase transition in even chains. We derive an effective channel-anisotropic 2CK model, which indicates that the critical FP of such models must be the 2CK FP. This physical picture is confirmed using NRG for various chain systems. We also examine the effect of local frustration on 2CK physics in mirror-symmetric ring systems. The importance of geometry and symmetry is demonstrated clearly in the markedly different physical behaviour that arises in systems where two leads are either connected to the same dot, or to neighbouring dots. In the latter case, we show for all odd-membered rings that two distinct 2CK phases, with different ground state parities, arise on tuning the interdot couplings. A frustration-induced phase transition thus occurs, the 2CK phases being separated by a novel critical point for which an effective low-energy model is derived. Precisely at the transition, parity mixing of the quasidegenerate local trimer states acts to destabilise the 2CK FPs, and the critical FP is shown to consist of a free pseudospin together with effective single-channel spin quenching. While connecting both leads to the same dot again results in two parity-distinct phases, a simple level-crossing transition now results due to the symmetry of the setup. The proposed geometry also allows access to a novel ferromagnetically-coupled two-channel local moment phase. Driven by varying the interdot couplings and occurring at the point of inherent magnetic frustration, such transitions in ring structures provide a striking example of the subtle interplay between internal spin and orbital degrees of freedom in coupled quantum dot systems, and the resulting effect on Kondo physics.
Charge Kondo circuits consist of metallic islands connected by single-mode quantum point contacts (QPCs). The island's charging energy makes these circuits tunable quantum simulators of various strongly interacting models. Here we propose a circuit that realizes the Kondo effect with effective Luttinger-liquid interactions, and show that it undergoes a localization transition in which the QPC transmission is fully suppressed below a critical value. Experimental signatures include a diverging charge susceptibility and an entropy step. Our findings open a path toward realizing localization transitions in more exotic settings.