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arXiv:2108.10928 · Physical Review Letters

Optical Entanglement of Distinguishable Quantum Emitters

David Levonian, Ralf Riedinger, Bartholomeus Machielse, Erik Knall, Mihir K. Bhaskar, Can M. Knaut, Rivka Bekenstein, Hongkun Park, Marko Lončar, Mikhail D. Lukin

Published May 23, 2022• 23 citations
arXivHTMLPDF

Abstract

Solid-state quantum emitters are promising candidates for the realization of quantum networks, owing to their long-lived spin memories, high-fidelity local operations, and optical connectivity for long-range entanglement. However, due to differences in local environment, solid-state emitters typically feature a range of distinct transition frequencies, which makes it challenging to create optically mediated entanglement between arbitrary emitter pairs. We propose and demonstrate an efficient method for entangling emitters with optical transitions separated by many linewidths. In our approach, electro-optic modulators enable a single photon to herald a parity measurement on a pair of spin qubits. We experimentally demonstrate the protocol using two silicon-vacancy centers in a diamond nanophotonic cavity, with optical transitions separated by 7.4 GHz. Working with distinguishable emitters allows for individual qubit addressing and readout, enabling parallel control and entanglement of both colocated and spatially separated emitters, a key step toward scaling up quantum information processing systems.

DOI
10.1103/physrevlett.128.213602

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Solid-state quantum emitters are promising candidates for the realization of quantum networks, owing to their long-lived spin memories, high-fidelity local operations, and optical connectivity for long-range entanglement. However, due to differences in local environment, solid-state emitters typically feature a range of distinct transition frequencies, which makes it challenging to create optically mediated entanglement between arbitrary emitter pairs. We propose and demonstrate an efficient method for entangling emitters with optical transitions separated by many linewidths. In our approach, electro-optic modulators enable a single photon to herald a parity measurement on a pair of spin qubits. We experimentally demonstrate the protocol using two silicon-vacancy centers in a diamond nanophotonic cavity, with optical transitions separated by 7.4 GHz. Working with distinguishable emitters allows for individual qubit addressing and readout, enabling parallel control and entanglement of both colocated and spatially separated emitters, a key step toward scaling up quantum information processing systems.
Chapter 1 reviews recent advances towards the realization of quantum networks based on atom-like solid-state quantum emitters coupled to nanophotonic devices. Specifically, focus is on experiments involving the negatively charged silicon-vacancy color center in diamond. These emitters combine homogeneous, coherent optical transitions and a long-lived electronic spin quantum memory. Optical and spin properties of this system at cryogenic temperatures and experiments where silicon-vacancy centers are coupled to nanophotonic cavities are discussed. Finally, the chapter discusses experiments demonstrating quantum nonlinearities at the single-photon level and two-emitter entanglement in a single nanophotonic device.
Photon-mediated coupling between distant matter qubits may enable secure communication over long distances, the implementation of distributed quantum computing schemes, and the exploration of new regimes of many-body quantum dynamics. Solid-state quantum emitters coupled to nanophotonic devices represent a promising approach towards these goals, as they combine strong lightmatter interaction and high photon collection efficiencies. However, nanostructured environments introduce mismatch and diffusion in optical transition frequencies of emitters, making reliable photonmediated entanglement generation infeasible. Here we address this long-standing challenge by employing silicon-vacancy color centers embedded in electromechanically deflectable nanophotonic waveguides. This electromechanical strain control enables control and stabilization of optical resonance between two silicon-vacancy centers on the hour timescale. Using this platform, we observe the signature of an entangled, superradiant state arising from quantum interference between two spatially separated emitters in a waveguide. This demonstration and the developed platform constitute a crucial step towards a scalable quantum network with solid-state quantum emitters.
Photon-mediated interactions between quantum systems are essential for realizing quantum networks and scalable quantum information processing. We demonstrate such interactions between pairs of silicon-vacancy (SiV) color centers coupled to a diamond nanophotonic cavity. When the optical transitions of the two color centers are tuned into resonance, the coupling to the common cavity mode results in a coherent interaction between them, leading to spectrally resolved superradiant and subradiant states. We use the electronic spin degrees of freedom of the SiV centers to control these optically mediated interactions. Such controlled interactions will be crucial in developing cavity-mediated quantum gates between spin qubits and for realizing scalable quantum network nodes.
Solid state quantum emitters with electronic spin properties can be entangled using optical interferometric which-path erasure techniques that rely on identical frequencies and linewidths of the emitters. This promises a powerful, fast and scalable platform for quantum technologies. Using current protocols, a pair of emitters embedded in a waveguide interferometer can be deterministically prepared in a maximally entangled state. However, the amount of entanglement diminishes rapidly with increasing separation of the emission lines and variations in the linewidths of the emitters. Solid state emitters such as quantum dots are subject to intrinsic variations in the fabrication process. Therefore, manufacturing the required number of identical emitters on a chip is not scalable. In this Letter, we present a method that uses readily available pairs of entangled photons to entangle solid state emitters with large transition frequency separations and linewidth variations, circumventing the need to fabricate optically identical emitters. We demonstrate a concurrence of C = 0.95 for typical quantum dots using narrowband photon inputs.
Photon-mediated interactions between quantum systems are essential for realizing quantum networks and scalable quantum information processing. We demonstrate such interactions between pairs of silicon-vacancy (SiV) color centers strongly coupled to a diamond nanophotonic cavity. When the optical transitions of the two color centers are tuned into resonance, the coupling to the common cavity mode results in a coherent interaction between them, leading to spectrally-resolved superradiant and subradiant states. We use the electronic spin degrees of freedom of the SiV centers to control these optically-mediated interactions. Our experiments pave the way for implementation of cavity-mediated quantum gates between spin qubits and for realization of scalable quantum network nodes.
Solid-state spin-photon interfaces promise to scale quantum networks through on-chip photonic integration and multiplexed entanglement generation. To date, remote entanglement between integrated emitters has been realized only in cavity-enhanced systems, where fabrication yield and spectral matching remain major obstacles. Here we demonstrate heralded remote entanglement between diamond tin-vacancy spin qubits embedded in separate on-chip waveguides. Combining intrinsically efficient photon emission with a broadband waveguide architecture provides high device yield and obviates the need for spectral matching to cavity modes. We realize coherent optical and spin control and achieve high-visibility two-photon interference. By combining photon-mediated entanglement generation with real-time feedforward, we produce a consistent entangled state independent of the heralding pattern. These results establish waveguide-integrated tin-vacancy centers as a compelling platform for scalable quantum network nodes.